High Cycle-Life Twistocaloric Cooling of Poly-p-Phenylene Benzodioxole Fibers.
elasticocaloric cooling
functional fibers
poly-p-phenylene benzodioxole (PBO)
twistocaloric cooling
Journal
Macromolecular rapid communications
ISSN: 1521-3927
Titre abrégé: Macromol Rapid Commun
Pays: Germany
ID NLM: 9888239
Informations de publication
Date de publication:
Dec 2023
Dec 2023
Historique:
revised:
29
07
2023
received:
01
06
2023
medline:
11
12
2023
pubmed:
13
8
2023
entrez:
12
8
2023
Statut:
ppublish
Résumé
It is an urgent need to develop efficient solid state cooling technologies and materials with high cycle life. Poly-p-phenylene benzodioxole (PBO) is a high performance fiber with excellent mechanical properties. In this work, for the first time, elasto- and twistocaloric cooling of PBO fibers by stretching and twisting of the PBO fiber bundles is reported. The cooling temperature reaches -0.4 and -1.3 K, for fiber stretching and twisting, respectively. A self-coiled PBO fiber achieves maximum cooling of -3.7 K upon stretching by 35% strain, with an exceptionally high cycle life of 200 000 times. During the twisting of the PBO fibers, reversible changes in the intensity of the diffraction peaks in X-ray diffraction patterns are observed. A strain-sensitive color change application is realized by coating a self-coiled PBO fiber with liquid crystallite dyes. This work provides new perspectives for PBO fibers as a high cycle-life solid-state refrigeration material.
Identifiants
pubmed: 37572085
doi: 10.1002/marc.202300318
doi:
Substances chimiques
poly-para-phenylene
0
Cycloparaffins
0
Heterocyclic Compounds
0
Benzodioxoles
0
Types de publication
Journal Article
Langues
eng
Sous-ensembles de citation
IM
Pagination
e2300318Subventions
Organisme : National Key Research and Development Program of China
ID : 2019YFE0119600
Organisme : National Key Research and Development Program of China
ID : 2022YFB3807103
Organisme : National Key Research and Development Program of China
ID : 2022YFA1203304
Organisme : National Natural Science Foundation of China
ID : 52090034
Organisme : National Natural Science Foundation of China
ID : 52225306
Organisme : National Natural Science Foundation of China
ID : 51973093
Organisme : National Natural Science Foundation of China
ID : 51773094
Organisme : Frontiers Science Center for New Organic Matter, Nankai University
ID : 63181206
Organisme : National Special Support Plan for High-Level Talents People
ID : C041800902
Organisme : Science Foundation for Distinguished Young Scholars of Tianjin
ID : 18JCJQJC46600
Organisme : Fundamental Research Funds for the Central Universities
ID : 63171219
Organisme : Operation Huiyan
ID : 62502510601
Informations de copyright
© 2023 Wiley-VCH GmbH.
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