Activation of Solid-State Emission and Photostability through Molecular Confinement: The Case of Triptycene-Fused Quinacridone Dyes.


Journal

Organic letters
ISSN: 1523-7052
Titre abrégé: Org Lett
Pays: United States
ID NLM: 100890393

Informations de publication

Date de publication:
08 Sep 2023
Historique:
medline: 28 8 2023
pubmed: 28 8 2023
entrez: 28 8 2023
Statut: ppublish

Résumé

We report the facile, metal-free convergent synthesis and the characterization of novel quinacridone dyes in which two triptycene units end-cap and sterically confine the quinacridone chromophore. A precise comparison of the confined dyes with their known homologues reveals that the reduction of π-π interactions in triptycene-fused quinacridone dyes compared to classical quinacridone results not only in an increase of solubility and processability but also in an enhancement of fluorescence quantum yield and photostability in the solid state.

Identifiants

pubmed: 37638412
doi: 10.1021/acs.orglett.3c02093
pmc: PMC10496147
doi:

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Pagination

6490-6494

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Auteurs

Giovanni Preda (G)

Department of Chemistry and INSTM, University of Pavia Via Taramelli 12, 27100 Pavia PV, Italy.

Andrea Aricò (A)

Department of Chemistry and INSTM, University of Pavia Via Taramelli 12, 27100 Pavia PV, Italy.

Chiara Botta (C)

SCITEC-CNR, Consiglio Nazionale delle Ricerche, Istituto di Scienze e Tecnologie Chimiche 'G. Natta', Via A. Corti 12, 20133 Milano, Italy.

Davide Ravelli (D)

Department of Chemistry and INSTM, University of Pavia Via Taramelli 12, 27100 Pavia PV, Italy.

Daniele Merli (D)

Department of Chemistry and INSTM, University of Pavia Via Taramelli 12, 27100 Pavia PV, Italy.

Sara Mattiello (S)

Dipartimento di Scienza dei Materiali, Università degli Studi Milano-Bicocca and INSTM, Via R. Cozzi 55, 20125, Milano, Italy.

Luca Beverina (L)

Dipartimento di Scienza dei Materiali, Università degli Studi Milano-Bicocca and INSTM, Via R. Cozzi 55, 20125, Milano, Italy.

Dario Pasini (D)

Department of Chemistry and INSTM, University of Pavia Via Taramelli 12, 27100 Pavia PV, Italy.

Classifications MeSH