Anion-Dependent Reactivity of Mono- and Dinuclear Boron Cations.

Lewis base bond activation boron cation phosphorus

Journal

Chemistry (Weinheim an der Bergstrasse, Germany)
ISSN: 1521-3765
Titre abrégé: Chemistry
Pays: Germany
ID NLM: 9513783

Informations de publication

Date de publication:
21 Nov 2023
Historique:
received: 04 08 2023
medline: 29 8 2023
pubmed: 29 8 2023
entrez: 29 8 2023
Statut: ppublish

Résumé

The dinuclear bis(N-heterocyclic carbene) borane adduct 2 rapidly reacts with tritylium salts at room temperature but the outcome is strongly impacted by the respective counter-ion. Using tritylium tetrakis(perfluoro-tert-butoxy)aluminate affords - depending on the solvent - either the bis(boronium) ion 4 or the hydride-bridged dication 5. In case of tritylium hexafluorophosphate, however, H/F exchange occurs between boron and phosphorus yielding the dinuclear BF

Identifiants

pubmed: 37641815
doi: 10.1002/chem.202302544
doi:

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Pagination

e202302544

Subventions

Organisme : Deutsche Forschungsgemeinschaft
ID : KR4782/3-1

Informations de copyright

© 2023 The Authors. Chemistry - A European Journal published by Wiley-VCH GmbH.

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Auteurs

Alexander Röther (A)

Institute of Inorganic and Analytical Chemistry (IAAC), Friedrich Schiller University Jena, Humboldtstraße 8, 07743, Jena, Germany.

James C Farmer (JC)

Institute of Inorganic and Analytical Chemistry (IAAC), Friedrich Schiller University Jena, Humboldtstraße 8, 07743, Jena, Germany.

Flavio L Portwich (FL)

Institute of Inorganic and Analytical Chemistry (IAAC), Friedrich Schiller University Jena, Humboldtstraße 8, 07743, Jena, Germany.

Helmar Görls (H)

Institute of Inorganic and Analytical Chemistry (IAAC), Friedrich Schiller University Jena, Humboldtstraße 8, 07743, Jena, Germany.

Robert Kretschmer (R)

Institute of Inorganic and Analytical Chemistry (IAAC), Friedrich Schiller University Jena, Humboldtstraße 8, 07743, Jena, Germany.
Jena Center for Soft Matter (JCSM), Friedrich Schiller University Jena, Philosophenweg 7, 07743, Jena, Germany.
Institute of Chemistry, Chemnitz University of Technology, Straße der Nationen 62, 09111, Chemnitz, Germany.

Classifications MeSH