Heterogenous Slippery Surfaces: Enabling Spontaneous and Rapid Transport of Viscous Liquids with Viscosities Exceeding 10 000 mPa s.
SLIPS
directional liquid transport
liquid manipulation
microfluidics
viscosity
wetting and capillary
Journal
Small (Weinheim an der Bergstrasse, Germany)
ISSN: 1613-6829
Titre abrégé: Small
Pays: Germany
ID NLM: 101235338
Informations de publication
Date de publication:
30 Aug 2023
30 Aug 2023
Historique:
revised:
07
08
2023
received:
19
05
2023
medline:
31
8
2023
pubmed:
31
8
2023
entrez:
31
8
2023
Statut:
aheadofprint
Résumé
Superhydrophobic and slippery lubricant-infused surfaces have garnered significant attention for their potential to passively transport low-viscosity liquids like water (1 mPa s). Despite exciting progress, these designs have proven ineffective for transporting high-viscosity liquids such as polydimethylsiloxane (5500 mPa s) due to their inherent limitations imposed by the homogenous surface design, resulting in high viscous drags and compromised capillary forces. Here, a heterogenous water-infused divergent surface (WIDS) is proposed that achieves spontaneous, rapid, and long-distance transport of viscous liquids. WIDS reduces viscous drag by spatially isolating the viscous liquids and surface roughness through its heterogenous, slippery topological design, and generates capillary forces through its heterogenous wetting distributions. The essential role of surface heterogeneity in viscous liquid transport is theoretically and experimentally verified. Remarkably, such a heterogenous paradigm enables transporting liquids with viscosities exceeding 12 500 mPa s, which is two orders of magnitude higher than state-of-the-art techniques. Furthermore, this heterogenous design is generic for various viscous liquids and can be made flexible, making it promising for various systems that require viscous liquid management, such as micropatterning.
Identifiants
pubmed: 37649201
doi: 10.1002/smll.202304218
doi:
Types de publication
Journal Article
Langues
eng
Sous-ensembles de citation
IM
Pagination
e2304218Subventions
Organisme : National Natural Science Foundation of China
ID : 52375442
Organisme : National Natural Science Foundation of China
ID : 51875285
Organisme : Natural Science Foundation of Jiangsu Province
ID : BK20190066
Organisme : Fok Ying Tung Education Foundation
ID : 171045
Organisme : Fok Ying Tung Education Foundation
ID : 20193218210002
Organisme : Fundamental Research Funds for the Central Universities
ID : NT2023010
Organisme : Research Grants Council of Hong Kong
ID : 11213320
Organisme : Research Grants Council of Hong Kong
ID : C1006-20WF
Informations de copyright
© 2023 Wiley-VCH GmbH.
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