3D Assembly of MXene Networks using a Ceramic Backbone with Controlled Porosity.
3D assembly of 2D materials
MXenes
conductive ceramics
porous backbone
supercapacitors
Journal
Advanced materials (Deerfield Beach, Fla.)
ISSN: 1521-4095
Titre abrégé: Adv Mater
Pays: Germany
ID NLM: 9885358
Informations de publication
Date de publication:
03 Sep 2023
03 Sep 2023
Historique:
revised:
14
08
2023
received:
19
05
2023
pubmed:
3
9
2023
medline:
3
9
2023
entrez:
3
9
2023
Statut:
aheadofprint
Résumé
Transition metal carbides (MXenes) are novel 2D nanomaterials with exceptional properties, promising significant impact in applications such as energy storage, catalysis, and energy conversion. A major barrier preventing the widespread use of MXenes is the lack of methods for assembling MXene in 3D space without significant restacking, which degrades their performance. Here, this challenge is successfully overcome by introducing a novel material system: a 3D network of MXene formed on a porous ceramic backbone. The backbone dictates the network's 3D architecture while providing mechanical strength, gas/liquid permeability, and other beneficial properties. Freeze casting is used to fabricate a silica backbone with open pores and controlled porosity. Next, capilary flow is used to infiltrate MXene into the backbone from a dispersion. The system is then dried to conformally coat the pore walls with MXene, creating an interconnected 3D-MXene network. The fabrication approach is reproducible, and the MXene-infiltrated porous silica (MX-PS) system is highly conductive (e.g., 340 S m
Identifiants
pubmed: 37660292
doi: 10.1002/adma.202304757
doi:
Types de publication
Journal Article
Langues
eng
Sous-ensembles de citation
IM
Pagination
e2304757Informations de copyright
© 2023 The Authors. Advanced Materials published by Wiley-VCH GmbH.
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