Is Ethanol Essential for the Lithium-Mediated Nitrogen Reduction Reaction?

ammonia synthesis electrochemistry lithium organic electrolyte electrolysis solid-electrolyte interphase

Journal

ChemSusChem
ISSN: 1864-564X
Titre abrégé: ChemSusChem
Pays: Germany
ID NLM: 101319536

Informations de publication

Date de publication:
22 Nov 2023
Historique:
revised: 03 08 2023
received: 13 07 2023
medline: 8 9 2023
pubmed: 8 9 2023
entrez: 8 9 2023
Statut: ppublish

Résumé

The lithium-mediated nitrogen reduction reaction (Li-NRR) is a promising method for decentralized ammonia synthesis using renewable energy. An organic electrolyte is utilized to combat the competing hydrogen evolution reaction, and lithium is plated to activate the inert N

Identifiants

pubmed: 37681646
doi: 10.1002/cssc.202301011
doi:

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Pagination

e202301011

Subventions

Organisme : Villum Fonden
ID : 9455
Organisme : Innovationsfonden
ID : 9067-00010B

Informations de copyright

© 2023 The Authors. ChemSusChem published by Wiley-VCH GmbH.

Références

U. P. Warehouse, U.S. Geological Survey 2023, http://pubs.er.usgs.gov/publication/mcs2023.
F. R. Service, Science 2018, 10.1126/science.aau7489.
C. Smith, A. K. Hill, L. Torrente-Murciano, Energy Environ. Sci. 2020, 13, 331-344.
F. Fichter, P. Girard, H. Erlenmeyer, Helv. Chim. Acta 1930, 13, 1228-1236.
A. Tsuneto, A. Kudo, T. Sakata, Chem. Lett. 1993, 22, 851-854.
A. Tsuneto, A. Kudo, T. Sakata, J. Electroanal. Chem. 1994, 367, 183-188.
S. Z. Andersen, V. Čolic, S. Yang, J. A. Schwalbe, A. C. Nielander, J. M. McEnaney, K. Enemark-Rasmussen, J. G. Baker, A. R. Singh, B. A. Rohr, M. J. Statt, S. J. Blair, S. Mezzavilla, J. Kibsgaard, P. C. K. Vesborg, M. Cargnello, S. F. Bent, T. F. Jaramillo, I. E. L. Stephens, J. K. Nørskov, I. Chorkendorff, Nature 2019, 570, 403-508.
B. H. R. Suryanto, K. Matuszek, J. Choi, R. Y. Hodgetts, H.-L. Du, J. M. Bakker, C. S. M. Kang, P. V. Cherepanov, A. N. Simonov, D. R. MacFarlane, Science 2021, 372, 1187-1191.
N. Lazousku, Z. J. Schiffer, K. Williams, K. Manthiram, Joule 2019, 3, 1-13.
O. Westhead, M. Spry, A. Bagger, Z. Shen, H. Yadegari, S. Favero, R. Tort, M. Titirici, M. P. Ryan, R. Jervis, Y. Katayama, A. Aguadero, A. Regoutz, A. Grimaud, I. E. L. Stephens, J. Mater. Chem. A 2022.
X. Cai, C. Fu, H. Iriawan, F. Yang, A. Wu, L. Luo, S. Shen, G. Wei, Y. Shao-Horn, J. Zhang, iScience 2021, 24, 103105.
B. H. R. Suryanto, H.-L. Du, D. Wang, D. Chen, J. Chen, A. N. Simonov, D. R. MacFarlane, Nat. Catal. 2019, 2, 290-296.
K. Li, S. Z. Andersen, M. J. Statt, M. Saccocio, V. J. Bukas, K. Kremple, R. Sazinas, J. B. Pedersen, V. Shadravan, Y. Zhou, D. Chakraborty, J. Kibsgaard, P. C. K. Vesborg, J. K. Nørskov, I. Chorkendorff, Science 2021, 374, 1593-1597.
M. Yan, Y. Kawamata, P. S. Baran, Chem. Rev. 2017, 117, 13230-13319.
X.-B. Cheng, R. Zhang, C.-Z. Zhao, F. Wei, J.-G. Zhang, Q. Zhang, Adv. Sci. 2016, 3, 1500213.
E. F. McFarlane, F. C. Tompkins, Trans. Faraday Soc. 1962, 58, 997-1007.
A. R. Singh, B. A. Rohr, J. A. Schwalbe, M. Cargnello, K. Chan, T. F. Jaramillo, I. Chorkendorff, J. K. Nørskov, ACS Catal. 2017, 7, 706-709.
S. Z. Andersen, M. J. Statt, V. J. Bukas, S. G. Shapel, J. B. Pedersen, K. Krempl, M. Saccocio, D. Chakraborty, J. Kibsgaard, P. C. K. Vesborg, J. Nørskov, I. Chorkendorff, Energy Environ. Sci. 2020, 13, 4291-4300.
K. Steinberg, X. Yuan, C. K. Klein, N. Lazouski, M. Mecklenburg, K. Manthiram, Y. Li, Nat. Energy 2022, 8, 138-148.
S. J. Blair, M. Doucet, J. F. Browning, K. Stone, H. Wang, C. Halbert, J. A. Acosta, Z. A. Z. José, N. C. Adam, A. Gallo, T. F. Jaramillo, ACS Energy Lett. 2022, 7, 1939-1946.
N. Lazouski, K. J. Steinberg, M. L. Gala, D. Krishnamurthy, V. Viswanathan, K. Manthiram, ACS Catal. 2022, 12, 5197-5208.
H.-L. Du, K. Matusek, R. Y. Hodgetts, K. N. Dinh, P. V. Cherepanov, J. M. Bakker, D. R. MacFarlane, A. N. Simonov, Energy Environ. Sci. 2023, 16, 1082-1090.
X. Fu, J. B. Pedersen, Y. Zhou, M. Saccocio, S. Li, R. Sazinas, K. Li, S. Z. Andersen, A. Xu, N. H. Deissler, J. B. V. Mygind, C. Wei, J. Kibsgaard, P. C. K. Vesborg, J. K. Nørskov, I. Chorkendorff, Science 2023, 379, 707-712.
A. N. Simonov, D. R. MacFarlane, K. Matuszek, C. K. Nguyen, P. V. Cherepanov, R. Y. Hodgetts, M. Chatti, H.-L. Du, Nature 2022, 609, 722-727.
S. Li, Y. Zhou, K. Li, M. Saccocio, R. Sažinas, S. Z. Andersen, J. B. Pedersen, X. Fu, V. Shadravan, D. Chakraborty, J. Kibsgaard, P. C. K. Vesborg, J. K. Nørskov, I. Chorkendordd, Joule 2022, 6, 2083-2101.
K. Krempl, J. B. Pedersen, J. Kibsgaard, P. C. K. Vesborg, I. Chorkendorff, Electrochem. Commun. 2022, 134, 107186.
Z. J. Schiffer, K. Williams, K. Manthiram, N. Lazouski, Joule 2019, 3, 1127-1139.
G. R. Zhuang, K. Wang, Y. Chen, J. Vac. Sci. Technol. A 1998, 16, 3041-3045.
G. Lunn, E. B. Sansone, J. Chem. Educ. 1994, 11, 972.
K. Krempl, D. Hochfiltzer, F. Cavalca, M. Saccocio, J. Kibsgaard, P. C. K. Vesborg, I. Chorkendorff, ChemElectroChem 2022, 9, e202101713.
D. D. Wagman, W. H. Evans, V. B. Parker, R. H. Schumm, I. Halow, S. M. Bailey, K. L. Churney, R. L. Nuttall, J. Phys. Chem. Ref. 1982, 11, 90-100.
N. Pino, López, J. F. Espinal, J. Mol. Model. 2019, 25, 1-10.
S. A. Cambell, C. Bowes, R. S. McMillan, J. Electroanal. Chem. 1990, 284, 195-204.
G. Sundholm, J. Electroanal. Chem. Interfacial Electrochem. 1971, 31, 265-267.
G. Gritzner, J. Mol. Liq. 2010, 156, 103-108.
A. N. Dey, E. J. Rudd, J. Electrochem. Soc. 1974, 121, 1294-1298.
S. Nakahama, K. Hashimoto, N. Yamazaki, Polym. J. 1973, 4, 437-445.
G. Pruckmayr, P. Dreyfuss, M. P. Dreyfuss, “Polyethers, Tetrahydrofuran, oxetane Polymers”, John Wiley & Sons, 2000, 1-30.
R. Sažinas, S. Z. Andersen, K. Li, M. Saccocio, K. Krempl, J. B. Pedersen, J. Kibsgaard, P. C. K. Vesborg, D. Chakraborty, I. Chorkendorff, RSC Adv. 2021, 11, 31487-31498.
E. J. McShane, P. Benedek, V. A. Niemann, S. J. Blair, G. A. Kamat, A. C. Nielander, T. F. Jaramillo, M. Cargnello, ACS Energy Lett. 2022, 8, 230-235.
R. Tort, O. Westhead, M. Spry, B. J. V. Davies, M. P. Ryan, M.-M. Titirici, I. E. L. Stephens, ACS Energy Lett. 2023, 8, 1003-1009.
J. R. Taylor, “An Introduction to Error Analysis: The Study of Uncertainties in Physical Measurements”, University Science Books, 1982, 90-100.
G. Sauerbrey, Zeitsschrift für Physik 1959, 1294-1298.
D. Aurbach, A. Zaban, J. Electroanal. Chem. 1995, 393, 43-53.
K. Alexander, S. Roslyakov, P. Loginov, Chem. Phys. Lett. 2021, 26, 1-5.
D. D. Wagman, W. H. Evans, V. B. Parker, R. Schumm, I. Halow, S. M. Bailey, K. Churney, R. Nuttall, J. Phys. Chem. Ref. 1982, 11, 90-100.

Auteurs

Jon Bjarke Valbaek Mygind (J)

Department of Physics, Technical University of Denmark, 2800, Kongens Lyngby, Denmark.

Jakob B Pedersen (JB)

Department of Physics, Technical University of Denmark, 2800, Kongens Lyngby, Denmark.

Katja Li (K)

Department of Physics, Technical University of Denmark, 2800, Kongens Lyngby, Denmark.

Niklas H Deissler (NH)

Department of Physics, Technical University of Denmark, 2800, Kongens Lyngby, Denmark.

Mattia Saccoccio (M)

Department of Physics, Technical University of Denmark, 2800, Kongens Lyngby, Denmark.

Xianbiao Fu (X)

Department of Physics, Technical University of Denmark, 2800, Kongens Lyngby, Denmark.

Shaofeng Li (S)

Department of Physics, Technical University of Denmark, 2800, Kongens Lyngby, Denmark.

Rokas Sažinas (R)

Department of Physics, Technical University of Denmark, 2800, Kongens Lyngby, Denmark.

Suzanne Z Andersen (SZ)

Department of Physics, Technical University of Denmark, 2800, Kongens Lyngby, Denmark.

Kasper Enemark-Rasmussen (K)

Department of Chemistry, Technical University of Denmark, Kongens Lyngby, Denmark.

Peter C K Vesborg (PCK)

Department of Physics, Technical University of Denmark, 2800, Kongens Lyngby, Denmark.

Jakob Doganli-Kibsgaard (J)

Department of Physics, Technical University of Denmark, 2800, Kongens Lyngby, Denmark.

Ib Chorkendorff (I)

Department of Physics, Technical University of Denmark, 2800, Kongens Lyngby, Denmark.

Classifications MeSH