Nonmetallic-Bonding Fe-Mn Diatomic Pairs Anchored on Hollow Carbonaceous Nanodisks for High-Performance Li-S Battery.
dual-metal single-atom catalysts
lithium-sulfur batteries
nonmetallic bonding interaction
separator modification
synergistic effects
Journal
Small (Weinheim an der Bergstrasse, Germany)
ISSN: 1613-6829
Titre abrégé: Small
Pays: Germany
ID NLM: 101235338
Informations de publication
Date de publication:
08 Sep 2023
08 Sep 2023
Historique:
medline:
9
9
2023
pubmed:
9
9
2023
entrez:
9
9
2023
Statut:
aheadofprint
Résumé
The issues of polysulfide shuttling and lethargic sulfur redox reaction (SROR) kinetics are the toughest obstacles of lithium-sulfur (Li-S) battery. Herein, integrating the merits of increased density of metal sites and synergistic catalytic effect, a unique single-atom catalyst (SAC) with nonmetallic-bonding Fe-Mn diatomic pairs anchored on hollow nitrogen-doped carbonaceous nanodisk (denoted as FeMnDA@NC) is successfully constructed and well characterized by aberration-corrected high-angle annular dark-field scanning transmission electron microscopy, X-ray absorption spectroscopy, etc. Density functional theory calculation indicates that the Fe-Mn diatomic pairs can effectively inhibit the shuttle effect by enhancing the adsorption ability retarding the polysulfide migration and accelerate the SROR kinetics. As a result, the Li-S battery assembled with FeMnDA@NC modified separator possesses an excellent electrochemical performance with ultrahigh specific capacities of 1419 mAh g
Identifiants
pubmed: 37688339
doi: 10.1002/smll.202306806
doi:
Types de publication
Journal Article
Langues
eng
Sous-ensembles de citation
IM
Pagination
e2306806Subventions
Organisme : Chinese National Science Foundation
ID : 22075008
Organisme : Chinese National Science Foundation
ID : 21571010
Organisme : Chinese National Science Foundation
ID : U0734002
Organisme : National Basic Research Programs of China
ID : 2014CB931800
Organisme : National Basic Research Programs of China
ID : 2011CB935700
Organisme : Chinese Aeronautic Project
ID : 2013ZF51069
Organisme : 111 Project
ID : B14009
Informations de copyright
© 2023 Wiley-VCH GmbH.
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