Toward Conductive Additive Free Organic Electrode for Lithium-Ion Battery Using Supramolecular Columnar Organization.
Li-ion batteries
columnar phase
conductive additive-free electrodes
organic batteries
perylene
Journal
Small (Weinheim an der Bergstrasse, Germany)
ISSN: 1613-6829
Titre abrégé: Small
Pays: Germany
ID NLM: 101235338
Informations de publication
Date de publication:
15 Sep 2023
15 Sep 2023
Historique:
medline:
15
9
2023
pubmed:
15
9
2023
entrez:
15
9
2023
Statut:
aheadofprint
Résumé
With the aim to meet the greatest challenge facing organic batteries, namely the low conductivity of the electrodes, the electrochemical properties of a series of substituted perylene diimides able to form semi-conductive columnar material are investigated. Depending on the substituent group, a strong influence of this group on the reversibility, redox potential but especially on the gravimetric capacity of the electrodes is observed. In the case of substitution by a simple propyl group, the corresponding diimide shows a complete electrochemical activity with only 10% by mass of conductive additive and even shows a half-capacity activity without any additive and without particular electrode engineering. Extensive research has highlighted the intrinsic reactivity of the columnar material but also its perpetual rearrangement during charge/discharge cycles. This study shows that the amount of conductive additive can be significantly reduced by adapting the design of the molecular material and favoring the assembly of redox units in the form of a conductive column.
Identifiants
pubmed: 37712120
doi: 10.1002/smll.202305701
doi:
Types de publication
Journal Article
Langues
eng
Sous-ensembles de citation
IM
Pagination
e2305701Informations de copyright
© 2023 Wiley-VCH GmbH.
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