Dynamic Local Structure in Caesium Lead Iodide: Spatial Correlation and Transient Domains.
CsPbI3
anharmonicity
dynamic structures
machine learning
metal halide perovskites
Journal
Small (Weinheim an der Bergstrasse, Germany)
ISSN: 1613-6829
Titre abrégé: Small
Pays: Germany
ID NLM: 101235338
Informations de publication
Date de publication:
21 Sep 2023
21 Sep 2023
Historique:
revised:
31
07
2023
received:
28
04
2023
medline:
22
9
2023
pubmed:
22
9
2023
entrez:
22
9
2023
Statut:
aheadofprint
Résumé
Metal halide perovskites are multifunctional semiconductors with tunable structures and properties. They are highly dynamic crystals with complex octahedral tilting patterns and strongly anharmonic atomic behavior. In the higher temperature, higher symmetry phases of these materials, several complex structural features are observed. The local structure can differ greatly from the average structure and there is evidence that dynamic 2D structures of correlated octahedral motion form. An understanding of the underlying complex atomistic dynamics is, however, still lacking. In this work, the local structure of the inorganic perovskite CsPbI
Identifiants
pubmed: 37736694
doi: 10.1002/smll.202303565
doi:
Types de publication
Journal Article
Langues
eng
Sous-ensembles de citation
IM
Pagination
e2303565Subventions
Organisme : Engineering and Physical Sciences Research Council
ID : EP/P022065/1
Organisme : Engineering and Physical Sciences Research Council
ID : EP/X035859/1
Organisme : Air Force Research Laboratory
ID : FA8655-21-1-7010
Organisme : Leverhulme Trust
ID : RPG-2021-191
Organisme : Vetenskapsrådet
ID : 2021-00486
Organisme : Consiglio Nazionale delle Ricerche
ID : ShortTermMobility2020prot.53767
Informations de copyright
© 2023 The Authors. Small published by Wiley-VCH GmbH.
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