Mesoporous Silica (MCM-41) Containing Dispersed Palladium Nanoparticles as Catalyst for Dehydrogenation, Methanolysis, and Reduction Reactions.

catalytic dehydrogenation heterogeneous catalysis mesoporous silica nitroarene reduction supported catalysts

Journal

ChemPlusChem
ISSN: 2192-6506
Titre abrégé: Chempluschem
Pays: Germany
ID NLM: 101580948

Informations de publication

Date de publication:
Oct 2023
Historique:
revised: 14 09 2023
received: 04 07 2023
medline: 22 9 2023
pubmed: 22 9 2023
entrez: 22 9 2023
Statut: ppublish

Résumé

Generating highly dispersed metal NPs of the desired size on surfaces such as porous silica is challenging due to wettability issues. Here, we report highly active and well-dispersed Pd incorporated mesoporous MCM-41 (Pd@MCM) using a facile impregnation via a molecular approach based on hydrogen bonding interaction of a palladium β-diketone complex with surface silanol groups of mesoporous silica. Controlled thermal treatment of so obtained materials in air, argon, and hydrogen provided the catalysts characterized by electron microscopy, nitrogen physisorption, X-ray diffraction and spectroscopy. Gratifyingly, our catalyst provided the lowest ever activation energy (14.3 kJ/mol) reported in literature for dehydrogenation of NaBH

Identifiants

pubmed: 37736704
doi: 10.1002/cplu.202300338
doi:

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Pagination

e202300338

Subventions

Organisme : Higher Education Commission (HEC) of Pakistan
ID : NRPU-5910

Informations de copyright

© 2023 Wiley-VCH GmbH.

Références

E. Roduner, Chem. Soc. Rev. 2014, 43 (24), 8226-8239.
J. Gong, R. Luque, Chem. Soc. Rev. 2014, 43 (22), 7466-7468.
J. Hagen, Industrial Catalysis: A Practical Approach, John Wiley & Sons: 2015.
G. J. Hutchings, J. Mater. Chem. 2009, 19 (9), 1222-1235.
R. Schlögl, Angew. Chem. Int. Ed. 2015, 54 (11), 3465-3520.
C. M. Friend, B. Xu, Acc. Chem. Res. 2017, 50 (3), 517-521.
I. Fechete, Y. Wang, J. C. Védrine, Catal. Today 2012, 189 (1), 2-27.
A. V. Neimark, L. I. Kheifets, V. B. Fenelonov, Ind. Eng. Chem. Prod. Res. Dev. 1981, 20 (3), 439-450.
P. Munnik, P. E. De Jongh, K. P. De Jong, Chem. Rev. 2015, 115 (14), 6687-6718.
C. Kresge, M. Leonowicz, W. J. Roth, J. Vartuli, J. Beck, Nature 1992, 359 (6397), 710.
R. Ller, R. Aler, The Chemistry of Silica: Solubility, Polymerization, Colloid and Surface Properties and Biochemistry of Silic,John Willey and Sons 1979, 326..
R. J. White, R. Luque, V. L. Budarin, J. H. Clark, D. J. Macquarrie, Chem. Soc. Rev. 2009, 38 (2), 481-494.
P. J. Harlick, A. Sayari, Ind. Eng. Chem. Res. 2007, 46 (2), 446-458.
B. Karimi, D. Zareyee, Org. Lett. 2008, 10 (18), 3989-3992.
X. J. Lin, A. Z. Zhong, Y. B. Sun, X. Zhang, W. G. Song, R. W. Lu, A. M. Cao, L. J. Wan, Chem. Commun. 2015, 51 (35), 7482-7485.
S. Soled, Science 2015, 350 (6265), 1171.
B. A. T. Mehrabadi, S. Eskandari, U. Khan, R. D. White, J. R. Regalbuto, Adv. Catal. 2017, 61, 1-35.
L. Jiao, J. R. Regalbuto, J. Catal. 2008, 260 (2), 329-341.
L. Jiao, J. Regalbuto, J. Catal. 2008, 260 (2), 342-350.
P. Van Der Voort, M. G. White, E. F. Vansant, Langmuir 1998, 14 (1), 106-112.
M. Baltes, O. Collart, P. Van Der Voort, E. Vansant, Langmuir 1999, 15 (18), 5841-5845.
J. C. Kenvin, M. G. White, M. B. Mitchell, Langmuir 1991, 7 (6), 1198-1205.
M. K. Samantaray, V. D'Elia, E. Pump, L. Falivene, M. Harb, S. Ould Chikh, L. Cavallo, J. M. Basset, Chem. Rev. 2020, 120 (2), 734-813.
S. Zhang, Y. Qian, W. S. Ahn, Chin. J. Catal. 2019, 40 (11), 1704-1712.
Z. Guan, S. Lu, C. Li, J. Catal. 2014, 311, 1-5.
C. Liu, J. Wang, L. Meng, Y. Deng, Y. Li, A. Lei, Angew. Chem. Int. Ed. 2011, 123 (22), 5250-5254.
Y. Wan, H. Wang, Q. Zhao, M. Klingstedt, O. Terasaki, D. Zhao, J. Am. Chem. Soc. 2009, 131 (12), 4541-4550.
B. Yuan, Y. Pan, Y. Li, B. Yin, H. Jiang, Angew. Chem. Int. Ed. 2010, 49 (24), 4054-4058.
A. Wang, J. Li, T. Zhang, Nat. Rev. chem 2018, 2 (6), 65-81.
L. Liu, A. Corma, Chem. Rev. 2018, 118 (10), 4981-5079.
L. Gibson, Chem. Soc. Rev. 2014, 43 (15), 5163-5172.
A. M, Hanu, S. Liu, V. Meynen, P. Cool, E. Popovici, E. F. Vansant, Microporous Mesoporous Mater. 2006, 95 (1-3), 31-38.
R. Holm, M. O'connor, Prog. Inorg. Chem. 1971, 14, 241-401.
P. Van Der Voort, M. Mathieu, E. Vansant, S. Rao, M. G. White, J. Porous Mater. 1998, 5 (3), 305-316.
O. Collart, P. Van Der Voort, E. Vansant, E. Gustin, A. Bouwen, D. Schoemaker, R. R. Rao, B. Weckhuysen, R. Schoonheydt, Phys. Chem. Chem. Phys. 1999, 1 (17), 4099-4104.
J.-P. Gallas, J.-M. Goupil, A. Vimont, J.-C. Lavalley, B. Gil, J.-P. Gilson, O. Miserque, Langmuir 2009, 25 (10), 5825-5834.
P. Van Der Voort, R. Ramachandra Rao, B. M. Weckhuysen, Phys. Chem. Chem. Phys. 1999, 1 (17), 4099-4104.
P. Van Der Voort, M. Morey, G. Stucky, M. Mathieu, E. Vansant, J. Phys. Chem. 1998, 102 (3), 585-590.
M. G. White, Catal. Today 1993, 18 (1), 73-109.
J. Van Ommen, H. Bosch, P. Gellings, J. Ross, Stud. Surf. Sci. Chem. 1987, 151-164.
H. Wang, T. Lu, Y. Li, B. Wu, J. Xue, F. Li, Z. Lv, J. Chem. 2016, 2016.
R. K. Biswas, P. Khan, S. Mukherjee, A. K. Mukhopadhyay, J. Ghosh, K. Muraleedharan, J. Non-Cryst. Solids 2018, 488, 1-9.
M.-Y. Kim, E. A. Kyriakidou, J.-S. Choi, T. J. Toops, A. J. Binder, C. Thomas, J. E. Parks II, V. Schwartz, J. Chen, D. K. Hensley, Appl. Catal. B 2016, 187, 181-194.
J. Mondal, R. Gomes, A. Modak, A. Bhaumik, Recycl. Catal. 2013, 1, 10-33.
R. Long, Z. Rao, K. Mao, Y. Li, C. Zhang, Q. Liu, C. Wang, Z. Y. Li, X. Wu, Y. Xiong, Angew. Chem. Int. Ed. 2015, 54 (8), 2425-2430.
R. Sharma, S. Sharma, Dalton Trans. 2014, 43 (3), 1292-1304.
X. Zhou, T. Shi, Appl. Surf. Sci. 2012, 259, 566-573.
N. S. Date, S. E. Kondawar, R. C. Chikate, C. V. Rode, ACS Omega 2018, 3 (8), 9860-9871.
M. Peuckert, J. Phys. Chem. 1985, 89 (12), 2481-2486.
T. Aditya, A. Pal, T. Pal, Chem. Commun. 2015, 51 (46), 9410-9431.
M. Irum, M. Zaheer, M. Friedrich, R. Kempe, RSC Adv. 2016, 6 (13), 10438-10441.
Y. Kojima, Y. Kawai, H. Nakanishi, S. Matsumoto, J. Power Sources 2004, 135 (1-2), 36-41.
A. Boran, S. Erkan, S. Ozkar, I. Eroglu, Int. J. Energy Res. 2013, 37 (5), 443-448.
R. Lin, M.-F. Luo, Q. Xin, G.-Q. Sun, Catal. Lett. 2004, 93, 139-144.
L. Meng, A. P. Jia, J. Q. Lu, L. F. Luo, W. X. Huang, M. F. Luo, J. Phys. Chem. C 2011, 115 (40), 19789-19796.
A. Hadi, I. I. Yaacob, Catal. Today 2004, 96 (3), 165-170.
X. Liu, J. Liu, F. Geng, Z. Li, P. Li, W. Gong, Front. Chem. Sci. Eng. 2012, 6, 34-37.
C. Huff, J. M. Long, A. Heyman, T. M. Abdel-Fattah, ACS Appl. Energ. Mater. 2018, 1 (9), 4635-4640.
H. Erdoğan, O. Metin, S. Özkar, Phys. Chem. Chem. Phys. 2009, 11 (44), 10519-10525.
J. Liu, G. Qin, P. Raveendran, Y. Ikushima, Chem. Eur. J. 2006, 12 (8), 2131-2138.
B. Baruah, G. J. Gabriel, M. J. Akbashev, M. E. Booher, Langmuir 2013, 29 (13), 4225-4234.
F. Hoffmann, M. Cornelius, J. Morell, M. Fröba, Angew. Chem. Int. Ed. 2006, 45 (20), 3216-3251.
S. Ek, A. Root, M. Peussa, L. Niinistö, Thermochim. Acta 2001, 379 (1-2), 201-212.
L. Zhuravlev, Colloids Surf. A 2000, 173 (1-3), 1-38.
S. Ek, A. Root, M. Peussa, L. Niinistö, Thermochim. Acta 2001, 379 (1-2), 201-212.
J. M. Kim, S. M. Chang, S. M. Kong, K. S. Kim, J. Kim, W. S. Kim, Ceram. Int. 2009, 35 (3), 1015-1019.
L. Zhuravlev, Langmuir 1987, 3 (3), 316-318.

Auteurs

Noor Ul Huda (N)

Department of chemistry and Chemical Engineering, Syed Babar Ali School of Science and Engineering, Lahore University of Management Sciences (LUMS), Sector U, DHA, Lahore, 54792, Pakistan.

Anwar Ul-Hamid (A)

Core Research Facilities, King Fahd University of Petroleum and Mineral, Dhahran, 31261, Saudi Arabia.

Muhammad Abdullah Khan (MA)

Renewable Energy Advancement Laboratory, Department of Environmental Sciences, Quaid-i-Azam University, Islamabad, Pakistan.

Shabnam Shahida (S)

Department of Chemistry, University of Poonch Rawalakot Azad Jammu and Kashmir, Rawalakot, Pakistan.

Muhammad Zaheer (M)

Department of chemistry and Chemical Engineering, Syed Babar Ali School of Science and Engineering, Lahore University of Management Sciences (LUMS), Sector U, DHA, Lahore, 54792, Pakistan.

Classifications MeSH