Elucidating the Mechanism of Large Phosphate Molecule Intercalation Through Graphene-Substrate Heterointerfaces.

defects graphene heterointerface intercalation reactions

Journal

ACS applied materials & interfaces
ISSN: 1944-8252
Titre abrégé: ACS Appl Mater Interfaces
Pays: United States
ID NLM: 101504991

Informations de publication

Date de publication:
11 Oct 2023
Historique:
medline: 2 10 2023
pubmed: 2 10 2023
entrez: 2 10 2023
Statut: ppublish

Résumé

Intercalation is the process of inserting chemical species into the heterointerfaces of two-dimensional (2D) layered materials. While much research has focused on the intercalation of metals and small gas molecules into graphene, the intercalation of larger molecules through the basal plane of graphene remains challenging. In this work, we present a new mechanism for intercalating large molecules through monolayer graphene to form confined oxide materials at the graphene-substrate heterointerface. We investigate the intercalation of phosphorus pentoxide (P

Identifiants

pubmed: 37782678
doi: 10.1021/acsami.3c07763
pmc: PMC10571006
doi:

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Pagination

47649-47660

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Auteurs

Jiayun Liang (J)

Department of Materials Science and Engineering, University of California, Berkeley, Berkeley, California 94720, United States.

Ke Ma (K)

Department of Materials Science and Engineering, University of California, Berkeley, Berkeley, California 94720, United States.

Xiao Zhao (X)

Department of Materials Science and Engineering, University of California, Berkeley, Berkeley, California 94720, United States.
Materials Sciences Division, Lawrence Berkeley National Laboratory, Berkeley, California 94720, United States.

Guanyu Lu (G)

Department of Mechanical Engineering, Vanderbilt University, Nashville, Tennessee 37235, United States.

Jake Riffle (J)

Department of Physics and Astronomy, University of New Hampshire, Durham, New Hampshire 03824, United States.

Carmen M Andrei (CM)

Canadian Centre for Electron Microscopy, McMaster University, Hamilton ,ON L8S 4L8, Canada.

Chengye Dong (C)

2D Crystal Consortium, The Pennsylvania State University, University Park, Pennsylvania 16802, United States.

Turker Furkan (T)

Department of Materials Science and Engineering, The Pennsylvania State University, University Park, Pennsylvania 16802, United States.

Siavash Rajabpour (S)

Department of Materials Science and Engineering, The Pennsylvania State University, University Park, Pennsylvania 16802, United States.

Rajiv Ramanujam Prabhakar (RR)

Chemical Sciences Division, Lawrence Berkeley National Laboratory, Berkeley, California 94720, United States.

Joshua A Robinson (JA)

2D Crystal Consortium, The Pennsylvania State University, University Park, Pennsylvania 16802, United States.
Department of Materials Science and Engineering, The Pennsylvania State University, University Park, Pennsylvania 16802, United States.

Vasquez Magdaleno (V)

Department of Mining, Metallurgy, and Materials Engineering, University of the Philippines, Diliman, Quezon City 1101, Philippines.

Quang Thang Trinh (QT)

Queensland Micro- and Nanotechnology Centre, Griffith University, Brisbane, 4111 Australia.

Joel W Ager (JW)

Department of Materials Science and Engineering, University of California, Berkeley, Berkeley, California 94720, United States.
Materials Sciences Division, Lawrence Berkeley National Laboratory, Berkeley, California 94720, United States.

Miquel Salmeron (M)

Department of Materials Science and Engineering, University of California, Berkeley, Berkeley, California 94720, United States.
Materials Sciences Division, Lawrence Berkeley National Laboratory, Berkeley, California 94720, United States.

Shaul Aloni (S)

The Molecular Foundry, Lawrence Berkeley National Laboratory, Berkeley, California 94720, United States.

Joshua D Caldwell (JD)

Department of Mechanical Engineering, Vanderbilt University, Nashville, Tennessee 37235, United States.

Shawna Hollen (S)

Department of Physics and Astronomy, University of New Hampshire, Durham, New Hampshire 03824, United States.

Hans A Bechtel (HA)

Advanced Light Source, Lawrence Berkeley National Laboratory, Berkeley, California 94720, United States.

Nabil D Bassim (ND)

Canadian Centre for Electron Microscopy, McMaster University, Hamilton ,ON L8S 4L8, Canada.
Department of Materials Science and Engineering, McMaster University, Hamilton ,ON L8S 4L8, Canada.

Matthew P Sherburne (MP)

Department of Materials Science and Engineering, University of California, Berkeley, Berkeley, California 94720, United States.

Zakaria Y Al Balushi (ZY)

Department of Materials Science and Engineering, University of California, Berkeley, Berkeley, California 94720, United States.
Materials Sciences Division, Lawrence Berkeley National Laboratory, Berkeley, California 94720, United States.

Classifications MeSH