New Protocol for the Synthesis of S-Thioesters from Benzylic, Allylic and Tertiary Alcohols with Thioacetic Acid.

alcohol kinetics mechanism thioesterification thiol

Journal

Chemistry (Weinheim an der Bergstrasse, Germany)
ISSN: 1521-3765
Titre abrégé: Chemistry
Pays: Germany
ID NLM: 9513783

Informations de publication

Date de publication:
12 Oct 2023
Historique:
received: 05 08 2023
pubmed: 12 10 2023
medline: 12 10 2023
entrez: 12 10 2023
Statut: aheadofprint

Résumé

A new one-pot solvent-less reaction to convert benzylic, allylic, ferrocenyl or tertiary alcohols into S-thioesters, bench-stable and less odorous precursors of the corresponding thiols, which is based on reactions in neat thioacetic acid in the presence of tetrafluoroboric acid, is presented. Reaction monitoring by NMR and GC of the benzyl alcohol conversion indicated the intermediate formation of benzyl acetate and benzyl thionoacetate (PhCH

Identifiants

pubmed: 37823749
doi: 10.1002/chem.202302551
doi:

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Pagination

e202302551

Informations de copyright

© 2023 Wiley-VCH GmbH.

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Auteurs

Abdelhak Lachguar (A)

LCC-CNRS, Université de Toulouse, UPS, INPT, 205 Route de Narbonne, 31077, Toulouse, Cedex 4, France.
IUT A Paul Sabatier, Dpt. De Chimie, Ave. G. Pompidou, 81104, Castres Cedex, France.

Uchchhal Bandyopadhyay (U)

LCC-CNRS, Université de Toulouse, UPS, INPT, 205 Route de Narbonne, 31077, Toulouse, Cedex 4, France.

Mehdi Ech-Chariy (M)

LCC-CNRS, Université de Toulouse, UPS, INPT, 205 Route de Narbonne, 31077, Toulouse, Cedex 4, France.
IUT A Paul Sabatier, Dpt. De Chimie, Ave. G. Pompidou, 81104, Castres Cedex, France.

Sandrine Vincendeau (S)

LCC-CNRS, Université de Toulouse, UPS, INPT, 205 Route de Narbonne, 31077, Toulouse, Cedex 4, France.

Catherine Audin (C)

LCC-CNRS, Université de Toulouse, UPS, INPT, 205 Route de Narbonne, 31077, Toulouse, Cedex 4, France.
IUT A Paul Sabatier, Dpt. De Chimie, Ave. G. Pompidou, 81104, Castres Cedex, France.

Jean-Claude Daran (JC)

LCC-CNRS, Université de Toulouse, UPS, INPT, 205 Route de Narbonne, 31077, Toulouse, Cedex 4, France.

Eric Manoury (E)

LCC-CNRS, Université de Toulouse, UPS, INPT, 205 Route de Narbonne, 31077, Toulouse, Cedex 4, France.

Rinaldo Poli (R)

LCC-CNRS, Université de Toulouse, UPS, INPT, 205 Route de Narbonne, 31077, Toulouse, Cedex 4, France.
Institut Universitaire de France, 1, rue Descartes, 75231, Paris, France.

Eric Deydier (E)

LCC-CNRS, Université de Toulouse, UPS, INPT, 205 Route de Narbonne, 31077, Toulouse, Cedex 4, France.
IUT A Paul Sabatier, Dpt. De Chimie, Ave. G. Pompidou, 81104, Castres Cedex, France.

Classifications MeSH