Design of Electrostatic Aberration Correctors for Scanning Transmission Electron Microscopy.

4D-STEM aberration correction phase plate scanning transmission electron microscopy simulation

Journal

Microscopy and microanalysis : the official journal of Microscopy Society of America, Microbeam Analysis Society, Microscopical Society of Canada
ISSN: 1435-8115
Titre abrégé: Microsc Microanal
Pays: England
ID NLM: 9712707

Informations de publication

Date de publication:
18 Oct 2023
Historique:
received: 16 03 2023
revised: 29 08 2023
accepted: 24 09 2023
medline: 18 10 2023
pubmed: 18 10 2023
entrez: 18 10 2023
Statut: aheadofprint

Résumé

In a scanning transmission electron microscope (STEM), producing a high-resolution image generally requires an electron beam focused to the smallest point possible. However, the magnetic lenses used to focus the beam are unavoidably imperfect, introducing aberrations that limit resolution. Modern STEMs overcome this by using hardware aberration correctors comprised of many multipole elements, but these devices are complex, expensive, and can be difficult to tune. We demonstrate a design for an electrostatic phase plate that can act as an aberration corrector. The corrector is comprised of annular segments, each of which is an independent two-terminal device that can apply a constant or ramped phase shift to a portion of the electron beam. We show the improvement in image resolution using an electrostatic corrector. Engineering criteria impose that much of the beam within the probe-forming aperture be blocked by support bars, leading to large probe tails for the corrected probe that sample the specimen beyond the central lobe. We also show how this device can be used to create other STEM beam profiles such as vortex beams and probes with a high degree of phase diversity, which improve information transfer in ptychographic reconstructions.

Identifiants

pubmed: 37851063
pii: 7321168
doi: 10.1093/micmic/ozad111
pii:
doi:

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Subventions

Organisme : U.S. Department of Energy
Organisme : Office of Science
Organisme : Workforce Development for Teachers and Scientists
Organisme : Office of Science Graduate Student Research (SCGSR) program
Organisme : Oak Ridge Institute for Science and Education
Organisme : National Science Foundation
ID : Grant No. DMR-1548924
Organisme : US Department of Energy Early Career Research Program
Organisme : SHyNE Resource
ID : NSF ECCS-2025633
Organisme : International Institute of Nanotechnology (IIN)
Organisme : Northwestern's MRSEC program
ID : NSF DMR-1720139
Organisme : Basic Energy Sciences

Informations de copyright

© The Author(s) 2023. Published by Oxford University Press on behalf of the Microscopy Society of America.

Auteurs

Stephanie M Ribet (SM)

Department of Materials Science and Engineering, Northwestern University, Evanston, IL 60208, USA.
International Institute of Nanotechnology, Northwestern University, Evanston, IL 60208, USA.
National Center for Electron Microscopy, Molecular Foundry, Lawrence Berkeley National Laboratory, Berkeley, CA 94720, USA.

Steven E Zeltmann (SE)

Platform for the Accelerated Realization, Analysis, and Discovery of Interface Materials (PARADIM), Cornell University, Ithaca, NY 14853, USA.
Department of Materials Science and Engineering, University of California, Berkeley, Berkeley, CA 94720, USA.

Karen C Bustillo (KC)

National Center for Electron Microscopy, Molecular Foundry, Lawrence Berkeley National Laboratory, Berkeley, CA 94720, USA.

Rohan Dhall (R)

National Center for Electron Microscopy, Molecular Foundry, Lawrence Berkeley National Laboratory, Berkeley, CA 94720, USA.

Peter Denes (P)

Molecular Foundry, Lawrence Berkeley National Laboratory, Berkeley, CA 94720, USA.

Andrew M Minor (AM)

National Center for Electron Microscopy, Molecular Foundry, Lawrence Berkeley National Laboratory, Berkeley, CA 94720, USA.
Department of Materials Science and Engineering, University of California, Berkeley, Berkeley, CA 94720, USA.

Roberto Dos Reis (R)

Department of Materials Science and Engineering, Northwestern University, Evanston, IL 60208, USA.
International Institute of Nanotechnology, Northwestern University, Evanston, IL 60208, USA.
The NUANCE Center, Northwestern University, Evanston, IL 60208, USA.

Vinayak P Dravid (VP)

Department of Materials Science and Engineering, Northwestern University, Evanston, IL 60208, USA.
International Institute of Nanotechnology, Northwestern University, Evanston, IL 60208, USA.
The NUANCE Center, Northwestern University, Evanston, IL 60208, USA.

Colin Ophus (C)

National Center for Electron Microscopy, Molecular Foundry, Lawrence Berkeley National Laboratory, Berkeley, CA 94720, USA.

Classifications MeSH