Design, synthesis and biological evaluation of novel DCLK1 inhibitor containing purine skeleton for the treatment of pancreatic cancer.


Journal

European journal of medicinal chemistry
ISSN: 1768-3254
Titre abrégé: Eur J Med Chem
Pays: France
ID NLM: 0420510

Informations de publication

Date de publication:
05 Dec 2023
Historique:
received: 02 08 2023
revised: 27 09 2023
accepted: 28 09 2023
medline: 3 11 2023
pubmed: 21 10 2023
entrez: 20 10 2023
Statut: ppublish

Résumé

Pancreatic cancer is a highly lethal form of malignancy that continues to pose a significant and unresolved health challenge. Doublecortin-like kinase 1 (DCLK1), a serine/threonine kinase, is found to be overexpressed in pancreatic cancer and holds promise as a potential therapeutic target for this disease. However, few potent inhibitors have been reported currently. Herein, a series of novel purine, pyrrolo [2,3-d]pyrimidine, and pyrazolo [3,4-d] pyrimidine derivatives were designed, synthesized, and evaluated their biological activities in vitro. Among them, compound I-5 stood out as the most potent compound with strong inhibitory activity against DCLK1 (IC

Identifiants

pubmed: 37862816
pii: S0223-5234(23)00813-9
doi: 10.1016/j.ejmech.2023.115846
pii:
doi:

Substances chimiques

Doublecortin-Like Kinases EC 2.7.1.11
Intracellular Signaling Peptides and Proteins 0
Protein Serine-Threonine Kinases EC 2.7.11.1
Pyrimidines 0
Purines 0
DCLK1 protein, human EC 2.7.1.11

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Pagination

115846

Informations de copyright

Copyright © 2023 Elsevier Masson SAS. All rights reserved.

Déclaration de conflit d'intérêts

Declaration of competing interest The authors declare that they have no known competing financial interests or personal relationships that could have appeared to influence the work reported in this paper.

Auteurs

Yuepeng Chen (Y)

Jiangsu Key Laboratory of Drug Design and Optimization, Department of Medicinal Chemistry, China Pharmaceutical University, Nanjing 211198, China.

Liuqiong Meng (L)

Jiangsu Key Laboratory of Drug Design and Optimization, Department of Medicinal Chemistry, China Pharmaceutical University, Nanjing 211198, China.

Wenze Wang (W)

Department of Pharmacology, China Pharmaceutical University, Nanjing 211198, China.

Liu Ye (L)

Department of Pharmacology, China Pharmaceutical University, Nanjing 211198, China.

Lei Huang (L)

Department of Pharmacology, China Pharmaceutical University, Nanjing 211198, China.

Chenghao Wang (C)

Department of Pharmacology, China Pharmaceutical University, Nanjing 211198, China.

Shuping Wang (S)

Jiangsu Key Laboratory of Drug Design and Optimization, Department of Medicinal Chemistry, China Pharmaceutical University, Nanjing 211198, China; Department of Pharmacology, China Pharmaceutical University, Nanjing 211198, China.

Mengyao Li (M)

Department of Pharmacology, China Pharmaceutical University, Nanjing 211198, China.

Yingxin Pei (Y)

Department of Pharmacology, China Pharmaceutical University, Nanjing 211198, China.

Shijie Zhang (S)

Department of Pharmacology, China Pharmaceutical University, Nanjing 211198, China.

Yi Zou (Y)

Jiangsu Key Laboratory of Drug Design and Optimization, Department of Medicinal Chemistry, China Pharmaceutical University, Nanjing 211198, China; Department of Pharmacology, China Pharmaceutical University, Nanjing 211198, China. Electronic address: zouyi@cpu.edu.cn.

Yungen Xu (Y)

Jiangsu Key Laboratory of Drug Design and Optimization, Department of Medicinal Chemistry, China Pharmaceutical University, Nanjing 211198, China; Department of Pharmacology, China Pharmaceutical University, Nanjing 211198, China. Electronic address: xyg@cpu.edu.cn.

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Classifications MeSH