Impact of Surface Ligand on the Biocompatibility of InP/ZnS Quantum Dots with Platelets.

InP/ZnS quantum dots (QDs) fluorescence fluorescence lifetime imaging microscopy (FLIM) hot-injections platelet imaging platelets biocompatibility

Journal

Small (Weinheim an der Bergstrasse, Germany)
ISSN: 1613-6829
Titre abrégé: Small
Pays: Germany
ID NLM: 101235338

Informations de publication

Date de publication:
09 Nov 2023
Historique:
revised: 24 10 2023
received: 09 06 2023
medline: 10 11 2023
pubmed: 10 11 2023
entrez: 10 11 2023
Statut: aheadofprint

Résumé

InP/ZnS quantum dots (QDs) have received a large focus in recent years as a safer alternative to heavy metal-based QDs. Given their intrinsic fluorescent imaging capabilities, these QDs can be potentially relevant for in vivo platelet imaging. The InP/ZnS QDs are synthesized and their biocompatibility investigated through the use of different phase transfer agents. Analysis of platelet function indicates that platelet-QD interaction can occur at all concentrations and for all QD permutations tested. However, as the QD concentration increases, platelet aggregation is induced by QDs alone independent of natural platelet agonists. This study helps to define a range of concentrations and coatings (thioglycolic acid and penicillamine) that are biocompatible with platelet function. With this information, the platelet-QD interaction can be identified using multiple methods. Fluorescent lifetime imaging microscopy (FLIM) and confocal studies have shown QDs localize on the surface of the platelet toward the center while showing evidence of energy transfer within the QD population. It is believed that these findings are an important stepping point for the development of fluorescent probes for platelet imaging.

Identifiants

pubmed: 37946631
doi: 10.1002/smll.202304881
doi:

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Pagination

e2304881

Subventions

Organisme : Medical Research Council
ID : MR/T002573/1
Pays : United Kingdom
Organisme : British Heart Foundation
ID : FS/16/62/32220
Pays : United Kingdom

Informations de copyright

© 2023 The Authors. Small published by Wiley-VCH GmbH.

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Auteurs

Hélio M Gil (HM)

Department of Imaging Chemistry and Biology, School of Biomedical Engineering and Imaging Sciences, King's College London, London, SE1 7EH, UK.
Centre for Biomedicine, Hull York Medical School, University of Hull, Hull, HU6 7RX, UK.

Zoe Booth (Z)

Centre for Biomedicine, Hull York Medical School, University of Hull, Hull, HU6 7RX, UK.

Thomas W Price (TW)

Department of Imaging Chemistry and Biology, School of Biomedical Engineering and Imaging Sciences, King's College London, London, SE1 7EH, UK.

Jessica Lee (J)

Centre for Biomedicine, University of Hull, Hull , HU6 7RX, UK.

Leigh Naylor-Adamson (L)

Centre for Biomedicine, Hull York Medical School, University of Hull, Hull, HU6 7RX, UK.

Michelle Avery (M)

Centre for Biomedicine, University of Hull, Hull , HU6 7RX, UK.

Alina Muravitskaya (A)

Department of Physics and Mathematics, University of Hull, Hull , HU6 7RX, UK.

Nicole Hondow (N)

School of Chemical and Process Engineering, University of Leeds, Leeds, LS2 9JT, UK.

David Allsup (D)

Centre for Biomedicine, Hull York Medical School, University of Hull, Hull, HU6 7RX, UK.

Jürgen E Schneider (JE)

School of Medicine, University of Leeds, Leeds, LS2 9JT, UK.

Khalid Naseem (K)

Leeds Institute of Cardiovascular and Metabolic Medicine, University of Leeds, Leeds, LS2 9JT, UK.

Ali M Adawi (AM)

Department of Physics and Mathematics, University of Hull, Hull , HU6 7RX, UK.

Jean-Sebastien G Bouillard (JG)

Department of Physics and Mathematics, University of Hull, Hull , HU6 7RX, UK.

Thomas W Chamberlain (TW)

Institute of Process Research and Development School of Chemistry, University of Leeds, Leeds, LS2 9JT, UK.

Simon D J Calaminus (SDJ)

Centre for Biomedicine, Hull York Medical School, University of Hull, Hull, HU6 7RX, UK.

Graeme J Stasiuk (GJ)

Department of Imaging Chemistry and Biology, School of Biomedical Engineering and Imaging Sciences, King's College London, London, SE1 7EH, UK.

Classifications MeSH