Pathway selection in the self-assembly of Rh
Journal
Communications chemistry
ISSN: 2399-3669
Titre abrégé: Commun Chem
Pays: England
ID NLM: 101725670
Informations de publication
Date de publication:
15 Nov 2023
15 Nov 2023
Historique:
received:
07
06
2023
accepted:
06
11
2023
medline:
16
11
2023
pubmed:
16
11
2023
entrez:
15
11
2023
Statut:
epublish
Résumé
Pathway selection principles in reversible reaction networks such as molecular self-assembly have not been established yet, because achieving kinetic control in reversible reaction networks is more complicated than in irreversible ones. In this study, we discovered that coordination squares consisting of cis-protected dinuclear rhodium(II) corner complexes and linear ditopic ligands are assembled under kinetic control, perfectly preventing the corresponding triangles, by modulating their energy landscapes with a weak monotopic carboxylate ligand (2,6-dichlorobenzoate: dcb
Identifiants
pubmed: 37968322
doi: 10.1038/s42004-023-01053-7
pii: 10.1038/s42004-023-01053-7
pmc: PMC10651846
doi:
Types de publication
Journal Article
Langues
eng
Pagination
248Subventions
Organisme : MEXT | Japan Society for the Promotion of Science (JSPS)
ID : 19H02731
Organisme : MEXT | Japan Society for the Promotion of Science (JSPS)
ID : 23H01970
Organisme : MEXT | Japan Society for the Promotion of Science (JSPS)
ID : 19K22196
Organisme : MEXT | Japan Society for the Promotion of Science (JSPS)
ID : 21K18974
Organisme : MEXT | Japan Society for the Promotion of Science (JSPS)
ID : 23K04663
Organisme : MEXT | Japan Society for the Promotion of Science (JSPS)
ID : 20K05417
Organisme : Asahi Glass Foundation
ID : none
Informations de copyright
© 2023. The Author(s).
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