Jamming of Miscible Liquids via Electrostatic Repulsion Between Polystyrene-Modified Gold Nanorods and Toluene.
charge transfer
matter delivery
miscible fluids
nanoparticle self-assembly
structured liquids
Journal
Small (Weinheim an der Bergstrasse, Germany)
ISSN: 1613-6829
Titre abrégé: Small
Pays: Germany
ID NLM: 101235338
Informations de publication
Date de publication:
21 Nov 2023
21 Nov 2023
Historique:
revised:
27
10
2023
received:
08
08
2023
medline:
22
11
2023
pubmed:
22
11
2023
entrez:
22
11
2023
Statut:
aheadofprint
Résumé
Structured liquids in miscible fluids, due to ineffective resistance to withstand particle self-diffusion, differ from that in immiscible liquids because of interfacial interactions. Here, a kind of structured liquid, jammed by thiol-terminated polystyrene-modified gold nanorods (GNRs) within tetrahydrofuran and toluene (TOL), is developed by introducing electrostatic repulsion to counterbalance the self-diffusion of GNRs. First-principle calculations reveal charge transfer between the GNRs and TOL, resulting in the electrostatic repulsion. The structured liquids can be regarded as mimic "loading vehicles" to controllably carry and transport matter under electric or magnetic fields, where release rate can be adjusted by changing the concentration of the soluble matter for slow release and using the photothermal effect of the assembled GNRs for fast release. This work has developed a new assembly mechanism to form structured liquids, allowing the construction of a flexible and robust droplet platform with possible applications in microreactors, biomimetic permeable membranes, and functional liquid robots.
Identifiants
pubmed: 37990397
doi: 10.1002/smll.202306767
doi:
Types de publication
Journal Article
Langues
eng
Sous-ensembles de citation
IM
Pagination
e2306767Subventions
Organisme : National Science Fund for Distinguished Young Scholars
ID : 52225308
Organisme : Fundamental Research Funds for the Central Universities
Organisme : Natural Science Foundation of Beijing Municipality
ID : 2202026
Organisme : National Natural Science Foundation of China-China Academy of General Technology Joint Fund for Basic Research
ID : 12074024
Organisme : National Natural Science Foundation of China-China Academy of General Technology Joint Fund for Basic Research
ID : 11974037
Organisme : National Natural Science Foundation of China-China Academy of General Technology Joint Fund for Basic Research
ID : 11774018
Informations de copyright
© 2023 Wiley-VCH GmbH.
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