Dissolution Reaction and Surface Modification of UICC Amosite in Mimicked Gamble's Solution: A Step towards Filling the Gap between Asbestos Toxicity and Its Crystal Chemical Features.

Gamble’s solution UICC amosite asbestos fibre dissolution

Journal

Nanomaterials (Basel, Switzerland)
ISSN: 2079-4991
Titre abrégé: Nanomaterials (Basel)
Pays: Switzerland
ID NLM: 101610216

Informations de publication

Date de publication:
12 Nov 2023
Historique:
received: 04 10 2023
revised: 02 11 2023
accepted: 10 11 2023
medline: 24 11 2023
pubmed: 24 11 2023
entrez: 24 11 2023
Statut: epublish

Résumé

This study focuses on the dissolution process and surface characterization of amosite fibres following interaction with a mimicked Gamble's solution at a pH of 4.5 and T = 37 °C, up to 720 h. To achieve this, a multi-analytical approach was adopted, and the results were compared to those previously obtained on a sample of asbestos tremolite and UICC crocidolite, which were investigated under the same experimental conditions. Combining surface chemical data obtained by XPS with cation release quantified by ICP-OES, an incongruent behaviour of the fibre dissolution was highlighted for amosite fibres, similarly to asbestos tremolite and UICC crocidolite. In particular, a preferential release of Mg and Ca from the amphibole structure was observed, in agreement with their Madelung site energies. Notably, no Fe release from amosite fibres was detected in our experimental conditions (pH of 4.5 and atmospheric pO

Identifiants

pubmed: 37999287
pii: nano13222933
doi: 10.3390/nano13222933
pmc: PMC10674585
pii:
doi:

Types de publication

Journal Article

Langues

eng

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Auteurs

Alessandro Pacella (A)

Department of Earth Sciences, Sapienza University of Rome, Piazzale Aldo Moro 5, 00185 Rome, Italy.

Paolo Ballirano (P)

Department of Earth Sciences, Sapienza University of Rome, Piazzale Aldo Moro 5, 00185 Rome, Italy.
Rectoral Laboratory Fibres and Inorganic Particulate, Sapienza University of Rome, Piazzale Aldo Moro 5, 00185 Rome, Italy.

Maria Cristina Di Carlo (MC)

Department of Earth Sciences, Sapienza University of Rome, Piazzale Aldo Moro 5, 00185 Rome, Italy.

Marzia Fantauzzi (M)

INSTM Research Unit, Department of Chemical and Geological Sciences, University of Cagliari, 09042 Monserrato, Italy.

Antonella Rossi (A)

INSTM Research Unit, Department of Chemical and Geological Sciences, University of Cagliari, 09042 Monserrato, Italy.

Elisa Nardi (E)

Institute for Environmental Protection and Research, ISPRA, Via Vitaliano Brancati 48, 00144 Rome, Italy.

Cecilia Viti (C)

Department of Physical, Earth and Environmental Sciences, University of Siena, Via Laterina 8, 53100 Siena, Italy.

Lorenzo Arrizza (L)

Microscopy Center, University of L' Aquila, Via Vetoio, Locality Coppito, 67100 L'Aquila, Italy.

Antonella Campopiano (A)

Department of Medicine, Epidemiology, Occupational and Environmental Hygiene, National Institute for Insurance against Accidents at Work (INAIL), Via Fontana Candida 1, 00078 Rome, Italy.

Annapaola Cannizzaro (A)

Department of Medicine, Epidemiology, Occupational and Environmental Hygiene, National Institute for Insurance against Accidents at Work (INAIL), Via Fontana Candida 1, 00078 Rome, Italy.

Andrea Bloise (A)

Department of Biology, Ecology and Earth Sciences, University of Calabria, V. P. Bucci, 87036 Arcavacata di Rende, Italy.

Maria Rita Montereali (MR)

Italian National Agency for New Technologies, ENEA, Casaccia Research Centre, Via Anguillarese 301, 00123 Rome, Italy.

Classifications MeSH