Chiral Supramolecular Organogel Constructed Using Riboflavin and Melamine: Its Application in Photo-Catalyzed Colorimetric Chiral Sensing and Enantioselective Adsorption.

self-assembly * gels * chiral sensing * optical resolution * riboflavin

Journal

Chemistry (Weinheim an der Bergstrasse, Germany)
ISSN: 1521-3765
Titre abrégé: Chemistry
Pays: Germany
ID NLM: 9513783

Informations de publication

Date de publication:
27 Nov 2023
Historique:
revised: 24 11 2023
received: 13 10 2023
accepted: 27 11 2023
medline: 28 11 2023
pubmed: 28 11 2023
entrez: 28 11 2023
Statut: aheadofprint

Résumé

The synthesis of a chiral supramolecular organogel via the hierarchical helical self-assembly of optically active riboflavin and melamine derivatives is described herein. Owing to the photocatalysis of riboflavin and the supramolecular chirality induced in the helically stacked riboflavin/melamine complex, the gel is observed to act as a light-stimulated chiral sensor of optically active alcohols by detecting the change in color from yellow to green. The gel also served as an efficient chiral adsorbent, enabling optical resolution of a racemic compound with high chiral recognition ability.

Identifiants

pubmed: 38012829
doi: 10.1002/chem.202303353
doi:

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Pagination

e202303353

Informations de copyright

© 2023 Wiley-VCH GmbH.

Auteurs

Marina Oka (M)

Shimane University, Department of Chemistry, JAPAN.

Ryo Kozako (R)

Shimane University, Department of Chemistry, JAPAN.

Yuta Teranishi (Y)

Shimane University, Department of Chemistry, JAPAN.

Yuta Yamada (Y)

Shimane University, Department of Chemistry, JAPAN.

Kazuhiro Miyake (K)

Nara Institute of Science and Technology: Nara Sentan Kagaku Gijutsu Daigakuin Daigaku, Center for Material Research Platform, JAPAN.

Takuya Fujimura (T)

Shimane University, Department of Chemistry, JAPAN.

Ryo Sasai (R)

Shimane University, Department of Chemistry, JAPAN.

Takahisa Ikeue (T)

Shimane University, Department of Chemistry, JAPAN.

Hiroki Iida (H)

Shimane University, Department of Chemistry, Graduate School of Natural Science and Technology, 1060 Nishikawatsu, 690-8504, Matsue, JAPAN.

Classifications MeSH