Enhanced Dynamics and Charge Transport at the Eutectic Point: A New Paradigm for the Use of Deep Eutectic Solvent Systems.


Journal

JACS Au
ISSN: 2691-3704
Titre abrégé: JACS Au
Pays: United States
ID NLM: 101775714

Informations de publication

Date de publication:
27 Nov 2023
Historique:
received: 28 07 2023
revised: 18 10 2023
accepted: 20 10 2023
medline: 30 11 2023
pubmed: 30 11 2023
entrez: 30 11 2023
Statut: epublish

Résumé

Deep eutectic solvents (DESs) are a class of versatile solvents with promise for a wide range of applications, from separation processes to electrochemical energy storage technologies. A fundamental understanding of the correlation among the structure, thermodynamics, and dynamics of these materials necessary for targeted rational design for specific applications is still nascent. Here, we employ differential scanning calorimetry (DSC), broadband dielectric spectroscopy (BDS), and femtosecond transient absorption spectroscopy (fs-TAS) to investigate the correlation among thermodynamics, dynamics, and charge transport in mixtures comprising a wide range of compositions of choline chloride (ChCl) and ethylene glycol (EG). Detailed analyses reveal that (i) the eutectic composition of this prototypical DES occurs in the 15-20 mol % ChCl in the EG range rather than the previously assumed 33 mol %, and (ii) both rotational dynamics and charge transport at the eutectic composition are enhanced in this composition range. These findings highlight the fundamental interplay between thermodynamics and dynamics in determining the properties of DESs that are relevant to many applications.

Identifiants

pubmed: 38034979
doi: 10.1021/jacsau.3c00420
pmc: PMC10685424
doi:

Types de publication

Journal Article

Langues

eng

Pagination

3024-3030

Informations de copyright

© 2023 The Authors. Published by American Chemical Society.

Déclaration de conflit d'intérêts

The authors declare no competing financial interest.

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Auteurs

Stephanie Spittle (S)

Department of Chemical and Biomolecular Engineering, University of Tennessee, Knoxville, Tennessee 37996, United States.

Ibrahim Alfurayj (I)

Department of Chemistry, Case Western Reserve University, Cleveland, Ohio 44106, United States.

Benworth Bryce Hansen (BB)

William G. Lowrie Department of Chemical and Biomolecular Engineering, The Ohio State University, Columbus, Ohio 43210, United States.

Kaylie Glynn (K)

William G. Lowrie Department of Chemical and Biomolecular Engineering, The Ohio State University, Columbus, Ohio 43210, United States.

William Brackett (W)

Department of Chemical and Biomolecular Engineering, University of Tennessee, Knoxville, Tennessee 37996, United States.

Rathiesh Pandian (R)

Department of Chemistry, Case Western Reserve University, Cleveland, Ohio 44106, United States.

Clemens Burda (C)

Department of Chemistry, Case Western Reserve University, Cleveland, Ohio 44106, United States.

Joshua Sangoro (J)

Department of Chemical and Biomolecular Engineering, University of Tennessee, Knoxville, Tennessee 37996, United States.
William G. Lowrie Department of Chemical and Biomolecular Engineering, The Ohio State University, Columbus, Ohio 43210, United States.

Classifications MeSH