Real-Time Simulation of Open Quantum Spin Chains with the Inchworm Method.


Journal

Journal of chemical theory and computation
ISSN: 1549-9626
Titre abrégé: J Chem Theory Comput
Pays: United States
ID NLM: 101232704

Informations de publication

Date de publication:
12 Dec 2023
Historique:
medline: 1 12 2023
pubmed: 1 12 2023
entrez: 1 12 2023
Statut: ppublish

Résumé

We study the real-time simulation of open quantum systems, where the system is modeled by a spin chain with each spin associated with its own harmonic bath. Our method couples the inchworm method for the spin-boson model and the modular path integral methodology for spin systems. In particular, the introduction of the inchworm method can significantly suppress the numerical sign problem. Both methods are tweaked to make them work seamlessly with each other. We represent our approach in the language of diagrammatic methods and analyze the asymptotic behavior of the computational cost. Extensive numerical experiments are performed to validate our method.

Identifiants

pubmed: 38039552
doi: 10.1021/acs.jctc.3c00751
doi:

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Pagination

8523-8540

Auteurs

Geshuo Wang (G)

Department of Mathematics, National University of Singapore, Block S17, 10 Lower Kent Ridge Road, Singapore 119076, Singapore.

Zhenning Cai (Z)

Department of Mathematics, National University of Singapore, Block S17, 10 Lower Kent Ridge Road, Singapore 119076, Singapore.

Classifications MeSH