Alkali Metal Metal(ates) Containing Divalent Earth Abundant Transition Metals.

Alkali metals Amides Ate complexes Cooperative effects Transition metals

Journal

Chimia
ISSN: 0009-4293
Titre abrégé: Chimia (Aarau)
Pays: Switzerland
ID NLM: 0373152

Informations de publication

Date de publication:
27 Apr 2022
Historique:
received: 02 02 2022
accepted: 22 02 2022
medline: 27 4 2022
pubmed: 27 4 2022
entrez: 9 12 2023
Statut: epublish

Résumé

Recent advances in cooperative chemistry have shown the enormous potential of main group heterobimetallic complexes for the functionalisation of aromatic molecules. Going beyond main group metal chemistry, here we provide an overview on the synthesis, structure and reactivity of bimetallic complexes which combine an alkali-metal (AM= Li, Na) with a divalent earth-abundant transition metal (M= Mn, Fe, Co, Ni), containing the utility silyl amide HMDS (HMDS = N(SiMe3)2). Advancing the understanding on how cooperative effects operate in these bimetallic (ate) systems, selected examples of their applications in deprotonative metalation are also discussed with special emphasis on the constitution of the metalated intermediates.

Identifiants

pubmed: 38069775
doi: 10.2533/chimia.2022.336
doi:

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Pagination

336-340

Subventions

Organisme : Swiss National Science Foundation
ID : 188753
Pays : Switzerland

Informations de copyright

Copyright 2022 Alessandra Logallo, Eva Hevia. License: This work is licensed under a Creative Commons Attribution 4.0 International License.

Auteurs

Alessandra Logallo (A)

Departement für Chemie und Biochemie (DCBP), Universität Bern, Freiestrasse 3, CH-3012, Bern, Switzerland. alessandra.logallo@unibe.ch.

Eva Hevia (E)

Departement für Chemie und Biochemie (DCBP), Universität Bern, Freiestrasse 3, CH-3012, Bern, Switzerland. eva.hevia@dcb.unibe.ch.

Classifications MeSH