Secondary 3-Chloropiperidines: Powerful Alkylating Agents.

alkylation antitumor agents aziridine primary chloroamine secondary 3-chloropiperidine

Journal

ChemistryOpen
ISSN: 2191-1363
Titre abrégé: ChemistryOpen
Pays: Germany
ID NLM: 101594811

Informations de publication

Date de publication:
13 Dec 2023
Historique:
revised: 15 10 2023
received: 21 09 2023
medline: 13 12 2023
pubmed: 13 12 2023
entrez: 13 12 2023
Statut: aheadofprint

Résumé

In previous works, we demonstrated that tertiary 3-chloropiperidines are potent chemotherapeutics, alkylating the DNA through the formation of bicyclic aziridinium ions. Herein, we report the synthesis of novel secondary 3-chloropiperidine analogues. The synthesis incorporates a new procedure to monochlorinate unsaturated primary amines utilizing N-chlorosuccinimide, while carefully monitoring the temperature to prevent dichlorination. Furthermore, we successfully isolated highly strained bicyclic aziridines by treating the secondary 3-chloropiperidines with a sufficient amount of base. We conclude this work with a DNA cleavage assay as a proof of principle, comparing our previously known substrates to the novel compounds. In this, the secondary 3-chloropiperidine as well as the isolated bicyclic aziridine, proved to be more effective than their tertiary counterpart.

Identifiants

pubmed: 38088585
doi: 10.1002/open.202300181
doi:

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Pagination

e202300181

Informations de copyright

© 2023 The Authors. ChemistryOpen published by Wiley-VCH GmbH.

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Auteurs

Mats Georg (M)

Institute of Organic Chemistry, Justus Liebig University Giessen, Heinrich-Buff-Ring 17, 35392, Giessen, Germany.

Lina Alexandra Laping (LA)

Institute of Organic Chemistry, Justus Liebig University Giessen, Heinrich-Buff-Ring 17, 35392, Giessen, Germany.

Veronica Billo (V)

Institute of Organic Chemistry, Justus Liebig University Giessen, Heinrich-Buff-Ring 17, 35392, Giessen, Germany.
Department of Pharmaceutical and Pharmacological Sciences, University of Padova, Padova, Italy.

Barbara Gatto (B)

Department of Pharmaceutical and Pharmacological Sciences, University of Padova, Padova, Italy.

Peter Friedhoff (P)

Institute of Biochemistry, Justus Liebig University Giessen, Heinrich-Buff-Ring 17, 35392, Giessen, Germany.

Richard Göttlich (R)

Institute of Organic Chemistry, Justus Liebig University Giessen, Heinrich-Buff-Ring 17, 35392, Giessen, Germany.

Classifications MeSH