Sustainable Recovery of Platinum Group Metals from Spent Automotive Three-Way Catalysts through a Biogenic Thiosulfate-Copper-Ammonia System.

biogas desulfurization bioleaching gas-lift platinum group metals three-way catalysts

Journal

Molecules (Basel, Switzerland)
ISSN: 1420-3049
Titre abrégé: Molecules
Pays: Switzerland
ID NLM: 100964009

Informations de publication

Date de publication:
14 Dec 2023
Historique:
received: 31 10 2023
revised: 08 12 2023
accepted: 12 12 2023
medline: 23 12 2023
pubmed: 23 12 2023
entrez: 23 12 2023
Statut: epublish

Résumé

This study explores an eco-friendly method for recovering platinum group metals from a synthetic automotive three-way catalyst (TWC). Bioleaching of palladium (Pd) using the thiosulfate-copper-ammonia leaching processes, with biogenic thiosulfate sourced from a bioreactor used for biogas biodesulfurization, is proposed as a sustainable alternative to conventional methods. Biogenic thiosulfate production was optimized in a gas-lift bioreactor by studying the pH (8-10) and operation modes (batch and continuous) under anoxic and microaerobic conditions for 35 d. The maximum concentration of 4.9 g S

Identifiants

pubmed: 38138568
pii: molecules28248078
doi: 10.3390/molecules28248078
pii:
doi:

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Subventions

Organisme : Regional Government of Andalusia
ID : FEDER-UCA18-106138
Organisme : Ministry of Universities
ID : ref. 2021-067/PN/MS-RECUAL/CD

Auteurs

Mariacristina Compagnone (M)

Department of Chemical Engineering and Food Technologies, Wine and Agrifood Research Institute (IVAGRO), Faculty of Sciences, University of Cadiz, Puerto Real, 11510 Cadiz, Spain.

José Joaquín González-Cortés (JJ)

Department of Chemical Engineering and Food Technologies, Wine and Agrifood Research Institute (IVAGRO), Faculty of Sciences, University of Cadiz, Puerto Real, 11510 Cadiz, Spain.

María Pilar Yeste (M)

Department of Material Science, Metallurgical Engineering and Inorganic Chemistry, Institute of Research on Electron Microscopy and Materials (IMEYMAT), Faculty of Sciences, University of Cadiz, Puerto Real, 11510 Cadiz, Spain.

Domingo Cantero (D)

Department of Chemical Engineering and Food Technologies, Wine and Agrifood Research Institute (IVAGRO), Faculty of Sciences, University of Cadiz, Puerto Real, 11510 Cadiz, Spain.

Martín Ramírez (M)

Department of Chemical Engineering and Food Technologies, Wine and Agrifood Research Institute (IVAGRO), Faculty of Sciences, University of Cadiz, Puerto Real, 11510 Cadiz, Spain.

Classifications MeSH