Conversion of Photoluminescence Blinking Types in Single Colloidal Quantum Dots.
CdSe/ZnS quantum dots
blinking mechanisms
blinking type conversion
perovskite quantum dots
photoluminescence blinking
Journal
Small (Weinheim an der Bergstrasse, Germany)
ISSN: 1613-6829
Titre abrégé: Small
Pays: Germany
ID NLM: 101235338
Informations de publication
Date de publication:
27 Dec 2023
27 Dec 2023
Historique:
revised:
29
11
2023
received:
10
10
2023
medline:
27
12
2023
pubmed:
27
12
2023
entrez:
27
12
2023
Statut:
aheadofprint
Résumé
Almost all colloidal quantum dots (QDs) exhibit undesired photoluminescence (PL) blinking, which poses a significant obstacle to their use in numerous luminescence applications. An in-depth study of the blinking behavior, along with the associated mechanisms, can provide critical opportunities for fabricating high-quality QDs for diverse applications. Here the blinking of a large series of colloidal QDs is investigated with different surface ligands, particle sizes, shell thicknesses, and compositions. It is found that the blinking behavior of single alloyed CdSe/ZnS QDs with a shell thickness of up to 2 nm undergoes an irreversible conversion from Auger-blinking to band-edge carrier blinking (BC-blinking). Contrastingly, single perovskite QDs with particle sizes smaller than their Bohr diameters exhibit reversible conversion between BC-blinking and more pronounced Auger-blinking. Changes in the effective trapping sites under different excitation conditions are found to be responsible for the blinking type conversions. Additionally, changes in shell thickness and particle size of QDs have a significant effect on the blinking type conversions due to altered wavefunction overlap between excitons and effective trapping sites. This study elucidates the discrepancies in the blinking behavior of various QD samples observed in previous reports and provides deeper understanding of the mechanisms underlying diverse types of blinking.
Identifiants
pubmed: 38150666
doi: 10.1002/smll.202309134
doi:
Types de publication
Journal Article
Langues
eng
Sous-ensembles de citation
IM
Pagination
e2309134Subventions
Organisme : National Key Research and Development Program of China
ID : 2022YFA1404201
Organisme : National Natural Science Foundation of China
ID : 62127817
Organisme : National Natural Science Foundation of China
ID : U22A2091
Organisme : National Natural Science Foundation of China
ID : U23A20380
Organisme : National Natural Science Foundation of China
ID : 62075120
Organisme : National Natural Science Foundation of China
ID : 62222509
Organisme : National Natural Science Foundation of China
ID : 62075122
Organisme : National Natural Science Foundation of China
ID : 22105011
Organisme : National Natural Science Foundation of China
ID : 62205187
Organisme : National Natural Science Foundation of China
ID : 62105193
Organisme : National Natural Science Foundation of China
ID : 62305201
Organisme : NSFC-STINT
ID : 62011530133
Organisme : China Postdoctoral Science Foundation
ID : 2022M722006
Organisme : Shanxi Province Science and Technology Innovation Talent Team
ID : 202204051001014
Organisme : Science and Technology Cooperation Project of Shanxi Province
ID : 202104041101021
Organisme : Natural Science Foundation of Shanxi Province
ID : 202103021223254
Organisme : PTIT, Shanxi "1331 Project", and 111 project
ID : D18001
Organisme : Program for Changjiang Scholars and Innovative Research Team
ID : IRT_17R70
Organisme : Shanxi Province Science and Technology Major Special Project
ID : 202201010101005
Informations de copyright
© 2023 Wiley-VCH GmbH.
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