Tailoring High-Entropy Oxides as Emerging Radiative Materials for Daytime Passive Cooling.
Journal
Chemistry of materials : a publication of the American Chemical Society
ISSN: 0897-4756
Titre abrégé: Chem Mater
Pays: United States
ID NLM: 9884133
Informations de publication
Date de publication:
26 Dec 2023
26 Dec 2023
Historique:
received:
17
05
2023
revised:
03
10
2023
accepted:
03
10
2023
medline:
2
1
2024
pubmed:
2
1
2024
entrez:
1
1
2024
Statut:
epublish
Résumé
In the framework of intense research about high-entropy materials and their applications in energy-oriented technologies, in the present work, we discuss the potential applicability of selected oxides and of the alloys they form at different concentrations for daytime radiative cooling implementation. In particular, by combining density functional theory and the finite difference method, we provide an unbiased, scattering-free description of structural, electronic, and dynamic features of the best candidates, showing the required strong radiative properties for passive cooling while offering the benefits of affordability and compatibility with commercial coating fabrication processes.
Identifiants
pubmed: 38162045
doi: 10.1021/acs.chemmater.3c01205
pmc: PMC10753767
doi:
Types de publication
Journal Article
Langues
eng
Pagination
10384-10393Informations de copyright
© 2023 The Authors. Published by American Chemical Society.
Déclaration de conflit d'intérêts
The authors declare no competing financial interest.