Sensitive simultaneous measurements of oxygenation and extracellular pH by EPR using a stable monophosphonated trityl radical and lithium phthalocyanine.

EPR ESR Hypoxia In vivo Metabolism Mitochondria Oxygenation Tumor microenvironment pH

Journal

Free radical biology & medicine
ISSN: 1873-4596
Titre abrégé: Free Radic Biol Med
Pays: United States
ID NLM: 8709159

Informations de publication

Date de publication:
11 Jan 2024
Historique:
received: 20 11 2023
revised: 09 01 2024
accepted: 10 01 2024
medline: 14 1 2024
pubmed: 14 1 2024
entrez: 13 1 2024
Statut: aheadofprint

Résumé

The monitoring of acidosis and hypoxia is crucial because both factors promote cancer progression and impact the efficacy of anti-cancer treatments. A phosphonated tetrathiatriarylmethyl (pTAM) has been previously described to monitor both parameters simultaneously, but the sensitivity to tackle subtle changes in oxygenation was limited. Here, we describe an innovative approach combining the pTAM radical and lithium phthalocyanine (LiPc) crystals to provide sensitive simultaneous measurements of extracellular pH (pH

Identifiants

pubmed: 38218552
pii: S0891-5849(24)00012-1
doi: 10.1016/j.freeradbiomed.2024.01.012
pii:
doi:

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Informations de copyright

Copyright © 2024. Published by Elsevier Inc.

Déclaration de conflit d'intérêts

Declaration of competing interest The authors declare no conflict of interest.

Auteurs

Chloe Buyse (C)

Biomedical Magnetic Resonance Research Group (REMA), Louvain Drug Research Institute (LDRI), UCLouvain, Brussels, Belgium.

Lionel Mignion (L)

Nuclear and Electron Spin Technologies Platform (NEST), Louvain Drug Research Institute (LDRI), UCLouvain, Brussels, Belgium.

Nicolas Joudiou (N)

Nuclear and Electron Spin Technologies Platform (NEST), Louvain Drug Research Institute (LDRI), UCLouvain, Brussels, Belgium.

Samia Melloul (S)

Biomedical Magnetic Resonance Research Group (REMA), Louvain Drug Research Institute (LDRI), UCLouvain, Brussels, Belgium.

Benoit Driesschaert (B)

Department of Pharmaceutical Sciences, School of Pharmacy & In Vivo Multifunctional Magnetic Resonance Center, West Virginia University, Morgantown, WV, USA.

Bernard Gallez (B)

Biomedical Magnetic Resonance Research Group (REMA), Louvain Drug Research Institute (LDRI), UCLouvain, Brussels, Belgium. Electronic address: bernard.gallez@uclouvain.be.

Classifications MeSH