Legacy Mercury Re-emission and Subsurface Migration at Contaminated Sites Constrained by Hg Isotopes and Chemical Speciation.

Hg contaminated sites Hg isotope fractionation Hg speciation MIE NVE re-emission subsurface migration

Journal

Environmental science & technology
ISSN: 1520-5851
Titre abrégé: Environ Sci Technol
Pays: United States
ID NLM: 0213155

Informations de publication

Date de publication:
12 Mar 2024
Historique:
medline: 13 3 2024
pubmed: 13 3 2024
entrez: 12 3 2024
Statut: aheadofprint

Résumé

The re-emission and subsurface migration of legacy mercury (Hg) are not well understood due to limited knowledge of the driving processes. To investigate these processes at a decommissioned chlor-alkali plant, we used mercury stable isotopes and chemical speciation analysis. The isotopic composition of volatilized Hg(0) was lighter compared to the bulk total Hg (THg) pool in salt-sludge and adjacent surface soil with mean ε

Identifiants

pubmed: 38472090
doi: 10.1021/acs.est.3c07276
doi:

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Auteurs

Wei Zhu (W)

State Key Laboratory of Environmental Geochemistry, Institute of Geochemistry, Chinese Academy of Sciences, Guiyang 550081, China.
Department of Forest Ecology and Management, Swedish University of Agricultural Sciences, Umeå SE-90183, Sweden.

Zhonggen Li (Z)

State Key Laboratory of Environmental Geochemistry, Institute of Geochemistry, Chinese Academy of Sciences, Guiyang 550081, China.
School of Resources and Environment, Zunyi Normal College, Zunyi 563006, China.

Ping Li (P)

State Key Laboratory of Environmental Geochemistry, Institute of Geochemistry, Chinese Academy of Sciences, Guiyang 550081, China.
University of Chinese Academy of Sciences, Beijing 100049, China.

Jonas Sommar (J)

State Key Laboratory of Environmental Geochemistry, Institute of Geochemistry, Chinese Academy of Sciences, Guiyang 550081, China.

Xuewu Fu (X)

State Key Laboratory of Environmental Geochemistry, Institute of Geochemistry, Chinese Academy of Sciences, Guiyang 550081, China.
University of Chinese Academy of Sciences, Beijing 100049, China.

Xinbin Feng (X)

State Key Laboratory of Environmental Geochemistry, Institute of Geochemistry, Chinese Academy of Sciences, Guiyang 550081, China.
University of Chinese Academy of Sciences, Beijing 100049, China.

Ben Yu (B)

State Key Laboratory of Environmental Geochemistry, Institute of Geochemistry, Chinese Academy of Sciences, Guiyang 550081, China.

Wei Zhang (W)

State Key Laboratory of Environmental Geochemistry, Institute of Geochemistry, Chinese Academy of Sciences, Guiyang 550081, China.

Ana T Reis (AT)

EPIUnit─Instituto de Saúde Pública, Universidade do Porto, Porto 4050-600, Portugal.
Laboratório para a Investigação Integrativa e Translacional em Saúde Populacional (ITR), Porto 4050-600, Portugal.

Eduarda Pereira (E)

LAQV-REQUIMTE─Associated Laboratory for Green Chemistry, University of Aveiro, Aveiro 3810-193, Portugal.

Classifications MeSH