Direct Synthesis of CuPd Icosahedra Supercrystals Studied by In Situ X-Ray Scattering.
PDF
SAXS
alloyed nanocrystals
oleic acid
oleylamine
segregation
self-assembly
Journal
Small (Weinheim an der Bergstrasse, Germany)
ISSN: 1613-6829
Titre abrégé: Small
Pays: Germany
ID NLM: 101235338
Informations de publication
Date de publication:
19 Mar 2024
19 Mar 2024
Historique:
revised:
20
02
2024
received:
15
12
2023
medline:
19
3
2024
pubmed:
19
3
2024
entrez:
19
3
2024
Statut:
aheadofprint
Résumé
Nanocrystal self-assembly into supercrystals provides a versatile platform for creating novel materials and devices with tailored properties. While common self-assembly strategies imply the use of purified nanoparticles after synthesis, conversion of chemical precursors directly into nanocrystals and then supercrystals in simple procedures has been rarely reported. Here, the nucleation and growth of CuPd icosahedra and their consecutive assembly into large closed-packed face-centered cubic (fcc) supercrystals are studied. To this end, the study simultaneously and in situ measures X-ray total scattering with pair distribution function analysis (TS-PDF) and small-angle X-ray scattering (SAXS). It is found that the supercrystals' formation is preceded by an intermediate dense phase of nanocrystals displaying short-range order (SRO). It is further shown that the organization of oleic acid/oleylamine surfactants into lamellar structures likely drives the emergence of the SRO phase and later of the supercrystals by reducing the volume accessible to particle diffusion. The supercrystals' formation as well as their disassembly are triggered by temperature. The study demonstrates that ordering of solvent molecules can be crucial in the direct synthesis of supercrystals. The study also provides a general approach to investigate novel preparation routes of supercrystals in situ and across several length scales via X-ray scattering.
Identifiants
pubmed: 38501853
doi: 10.1002/smll.202311714
doi:
Types de publication
Journal Article
Langues
eng
Sous-ensembles de citation
IM
Pagination
e2311714Subventions
Organisme : Bundesministerium für Bildung und Forschung
ID : 05K19GU7 / 05K19WMA
Organisme : Bundesministerium für Bildung und Forschung
ID : 05K22GU7
Organisme : Deutsche Forschungsgemeinschaft, Cluster of Excellence" CUI: AdvancedImagingofMatter"
ID : EXC2056-project-ID-390715994
Organisme : ERC Consolidator Grant LINCHPIN
ID : 818941
Informations de copyright
© 2024 The Authors. Small published by Wiley-VCH GmbH.
Références
a) S.-W. Hsu, A. L. Rodarte, M. Som, G. Arya, A. R. Tao, Chem. Rev. 2018, 118, 3100;
b) I. Cherniukh, G. Rainò, T. Stöferle, M. Burian, A. Travesset, D. Naumenko, H. Amenitsch, R. Erni, R. F. Mahrt, M. I. Bodnarchuk, M. V. Kovalenko, Nature. 2021, 593, 535.
a) C. R. Kagan, E. Lifshitz, E. H. Sargent, D. V. Talapin, Science. 2016, 353, aac5523;
b) M. Hadjimichael, Y. Li, E. Zatterin, G. A. Chahine, M. Conroy, K. Moore, E. N. O. Connell, P. Ondrejkovic, P. Marton, J. Hlinka, U. Bangert, S. Leake, P. Zubko, Nat. Mater. 2021, 20, 495.
a) H. Zhao, S. Sen, T. Udayabhaskararao, M. Sawczyk, K. Kučanda, D. Manna, P. K. Kundu, J.-W. Lee, P. Král, R. Klajn, Nat. Nanotechnol. 2016, 11, 82;
b) W. Baek, M. S. Bootharaju, K. M. Walsh, S. Lee, D. R. Gamelin, T. Hyeon, Nat. Mater. 2021, 20, 650.
M. R. Begley, D. S. Gianola, T. R. Ray, Science. 2019, 364, eaav4299.
a) J. Shi, Z. Xiao, N. Kamaly, O. C. Farokhzad, Acc. Chem. Res. 2011, 44, 1123;
b) H. Zhou, M. Guo, J. Li, F. Qin, Y. Wang, T. Liu, J. Liu, Z. F. Sabet, Y. Wang, Y. Liu, J. Am. Chem. Soc. 2021, 143, 1846;
c) Y. Shamay, J. Shah, M. Işık, A. Mizrachi, J. Leibold, D. F. Tschaharganeh, D. Roxbury, J. Budhathoki-Uprety, K. Nawaly, J. L. Sugarman, Nat. Mater. 2018, 17, 361.
a) M. V. Kovalenko, L. Manna, A. Cabot, Z. Hens, D. V. Talapin, C. R. Kagan, V. I. Klimov, A. L. Rogach, P. Reiss, D. J. Milliron, ACS Nano. 2015, 9, 1012;
b) K. S. Sugi, A. Maier, M. Scheele, Chem. Commun. 2022, 58, 6998;
c) C. Jenewein, S. M. Schupp, B. Ni, L. Schmidt-Mende, H. Cölfen, Small Science. 2022, 2, 2200014;
d) I. Coropceanu, E. M. Janke, J. Portner, D. Haubold, T. D. Nguyen, A. Das, C. P. N. Tanner, J. K. Utterback, S. W. Teitelbaum, M. H. Hudson, N. A. Sarma, A. M. Hinkle, C. J. Tassone, A. Eychmüller, D. T. Limmer, M. Olvera de la Cruz, N. S. Ginsberg, D. V. Talapin, Science. 2022, 375, 1422;
e) M. A. Boles, M. Engel, D. V. Talapin, Chem. Rev. 2016, 116, 11220;
f) H. Han, S. Kallakuri, Y. Yao, C. B. Williamson, D. R. Nevers, B. H. Savitzky, R. S. Skye, M. Xu, O. Voznyy, J. Dshemuchadse, L. F. Kourkoutis, S. J. Weinstein, T. Hanrath, R. D. Robinson, Nat. Mater. 2022, 21, 518.
a) A. R. Tao, S. Habas, P. Yang, Small. 2008, 4, 310;
b) R. Jin, C. Zeng, M. Zhou, Y. Chen, Chem. Rev. 2016, 116, 10346;
c) Y. Xia, K. D. Gilroy, H. C. Peng, X. Xia, Angew. Chem., Int. Ed. 2017, 56, 60;
d) P.-C. Chen, M. Liu, J. S. Du, B. Meckes, S. Wang, H. Lin, V. P. Dravid, C. Wolverton, C. A. Mirkin, Science. 2019, 363, 959;
e) V. Mantella, L. Castilla-Amorós, R. Buonsanti, Chem. Sci. 2020, 11, 11394;
f) N. Kar, M. McCoy, J. Wolfe, S. L. A. Bueno, I. H. Shafei, S. E. Skrabalak, Nat. Synth. 2024, 175.
a) J. Schlotheuber né Brunner, B. Maier, S. L. J. Thomä, F. Kirner, I. A. Baburin, D. Lapkin, R. Rosenberg, S. Sturm, D. Assalauova, J. Carnis, Y. Y. Kim, Z. Ren, F. Westermeier, S. Theiss, H. Borrmann, S. Polarz, A. Eychmüller, A. Lubk, I. A. Vartanyants, E. V. Sturm, Chem. Mater. 2021, 33, 9119;
b) W. Han, Z. Lin, Angew. Chem., Int. Ed. 2012, 51, 1534;
c) N. Vogel, M. Retsch, C.-A. Fustin, A. Del Campo, U. Jonas, Chem. Rev. 2015, 115, 6265;
d) W. Wei, F. Bai, H. Fan, Angew. Chem., Int. Ed. 2019, 58, 11956.
a) B. Abécassis, F. Testard, O. Spalla, Phys. Rev. Lett. 2008, 100, 115504;
b) L. Wu, J. J. Willis, I. S. McKay, B. T. Diroll, J. Qin, M. Cargnello, C. J. Tassone, Nature. 2017, 548, 197;
c) D. R. Nevers, C. B. Williamson, B. H. Savitzky, I. Hadar, U. Banin, L. F. Kourkoutis, T. Hanrath, R. D. Robinson, J. Am. Chem. Soc. 2018, 140, 3652;
d) F. Nakagawa, M. Saruyama, R. Takahata, R. Sato, K. Matsumoto, T. Teranishi, J. Am. Chem. Soc. 2022, 144, 5871;
e) F. Montanarella, Q. A. Akkerman, D. Bonatz, M. M. van der Sluijs, J. C. van der Bok, P. T. Prins, M. Aebli, A. Mews, D. Vanmaekelbergh, M. V. Kovalenko, Nano Lett. 2023, 23, 667.
T. Kister, D. Monego, P. Mulvaney, A. Widmer-Cooper, T. Kraus, ACS Nano. 2018, 12, 5969.
J. J. Calvin, A. S. Brewer, A. P. Alivisatos, Nat. Synth. 2022, 1, 127.
a) S. Karthika, T. Radhakrishnan, P. Kalaichelvi, Cryst. Growth Des. 2016, 16, 6663;
b) P. G. Vekilov, Nanoscale. 2010, 2, 2346.
a) D. Pontoni, T. Narayanan, A. Rennie, Langmuir. 2002, 18, 56;
b) B. Abécassis, F. Testard, O. Spalla, P. Barboux, Nano Lett. 2007, 7, 1723;
c) J. Polte, R. Erler, A. F. Thunemann, S. Sokolov, T. T. Ahner, K. Rademann, F. Emmerling, R. Kraehnert, ACS Nano. 2010, 4, 1076;
d) K. M. Jensen, M. Christensen, P. Juhas, C. Tyrsted, E. D. Bøjesen, N. Lock, S. J. Billinge, B. B. Iversen, J. Am. Chem. Soc. 2012, 134, 6785;
e) L. Grote, C. A. Zito, K. Frank, A.-C. Dippel, P. Reisbeck, K. Pitala, K. O. Kvashnina, S. Bauters, B. Detlefs, O. Ivashko, Nat. Commun. 2021, 12, 4429;
f) J. K. Mathiesen, J. Quinson, A. Dworzak, T. Vosch, M. Juelsholt, E. T. Kjaer, J. Schröder, J. J. Kirkensgaard, M. Oezaslan, M. Arenz, J. Phys. Chem. Lett. 2021, 12, 3224;
g) J. Li, F. L. Deepak, Chem. Rev. 2022, 122, 16911.
a) T. Li, A. J. Senesi, B. Lee, Chem. Rev. 2016, 116, 11128;
b) F. Montanarella, J. J. Geuchies, T. Dasgupta, P. T. Prins, C. van Overbeek, R. Dattani, P. Baesjou, M. Dijkstra, A. V. Petukhov, A. van Blaaderen, D. Vanmaekelbergh, Nano Lett. 2018, 18, 3675;
c) I. Lokteva, M. Koof, M. Walther, G. Grubel, F. Lehmkuhler, Small. 2019, 15, 1900438;
d) E. Marino, D. J. Rosen, S. Yang, E. H. R. Tsai, C. B. Murray, Nano Lett. 2023, 23, 4250;
e) C. P. N. Tanner, J. K. Utterback, J. Portner, I. Coropceanu, A. Das, C. J. Tassone, S. W. Teitelbaum, D. T. Limmer, D. V. Talapin, N. S. Ginsberg, ACS Nano. 2024, 18, 5778.
D. Derelli, F. Caddeo, K. Frank, K. Krötzsch, P. Ewerhardt, M. Krger, S. Medicus, L. Klemeyer, M. Skiba, C. Ruhmlieb, O. Gutowski, A. C. Dippel, W. J. Parak, B. Nickel, D. Koziej, Angew. Chem., Int. Ed. 2023, 62, 202307948.
a) X. Yin, M. Shi, K. S. Kwok, H. Zhao, D. L. Gray, J. A. Bertke, H. Yang, Nano Res. 2018, 11, 3442;
b) J. K. Mathiesen, E. D. Bøjesen, J. K. Pedersen, E. T. Kjaer, M. Juelsholt, S. Cooper, J. Quinson, A. S. Anker, G. Cutts, D. S. Keeble, Small Methods. 2022, 6, 2200420.
S. Banerjee, C. H. Liu, K. M. O. Jensen, P. Juhas, J. D. Lee, M. Tofanelli, C. J. Ackerson, C. B. Murray, S. J. L. Billinge, Acta Crystallogr. A. 2020, 76, 24.
a) Q. Zhang, J. Xie, J. Yang, J. Y. Lee, ACS Nano. 2009, 3, 139;
b) J. Reyes-Gasga, S. Tehuacanero-Nuñez, J. Montejano-Carrizales, X. Gao, M. Jose-Yacaman, Top. Catal. 2007, 46, 23;
c) J. Reyes-Gasga, S. Tehuacanero-Nuñez, J. Montejano-Carrizales, Acta Microsc. 2009, 18, 304.
a) M. Klokkenburg, J. Hilhorst, B. Erné, Vib. Spectrosc. 2007, 43, 243;
b) N. Shukla, C. Liu, P. M. Jones, D. Weller, J. Magn. Magn. Mater. 2003, 266, 178.
a) S. Mourdikoudis, M. Menelaou, N. Fiuza-Maneiro, G. Zheng, S. Wei, J. Pérez-Juste, L. Polavarapu, Z. Sofer, Nanoscale Horiz. 2022, 7, 941;
b) M. C. Weidman, Q. Nguyen, D.-M. Smilgies, W. A. Tisdale, Chem. Mater. 2018, 30, 807;
c) J. Borges, J. A. Ribeiro, E. M. Pereira, C. A. Carreira, C. M. Pereira, F. Silva, J. Colloid Interface Sci. 2011, 358, 626.
a) M. C. Weidman, D.-M. Smilgies, W. A. Tisdale, Nat. Mater. 2016, 15, 775;
b) B. De Nijs, S. Dussi, F. Smallenburg, J. D. Meeldijk, D. J. Groenendijk, L. Filion, A. Imhof, A. Van Blaaderen, M. Dijkstra, Nat. Mater. 2015, 14, 56;
c) A. Lesaine, D. Bonamy, C. L. Rountree, G. Gauthier, M. Impéror-Clerc, V. Lazarus, Soft Matter. 2021, 17, 1589.
a) R. Mondal, G. Kumaraswamy, Mater. Adv. 2022, 3, 3041;
b) R. Rajamanickam, S. Kumari, D. Kumar, S. Ghosh, J. C. Kim, G. Tae, S. Sen Gupta, G. Kumaraswamy, Chem. Mater. 2014, 26, 5161.
a) B. J. Alder, T. E. Wainwright, J. Chem. Phys. 1957, 27, 1208;
b) P. N. Pusey, W. Van Megen, Nature. 1986, 320, 340.
G. Ashiotis, A. Deschildre, Z. Nawaz, J. P. Wright, D. Karkoulis, F. E. Picca, J. Kieffer, J. Appl. Crystallogr. 2015, 48, 510.
P. Juhás, T. Davis, C. L. Farrow, S. J. L. Billinge, J. Appl. Crystallogr. 2013, 46, 560.
P. Juhás, C. L. Farrow, X. Yang, K. R. Knox, S. J. L. Billinge, in Acta Crystallographica Section A: Foundations and Advances, 71, 2015, 562.
A. Hjorth Larsen, J. Jorgen Mortensen, J. Blomqvist, I. E. Castelli, R. Christensen, M. Dulak, J. Friis, M. N. Groves, B. Hammer, C. Hargus, E. D. Hermes, P. C. Jennings, P. Bjerre Jensen, J. Kermode, J. R. Kitchin, E. Leonhard Kolsbjerg, J. Kubal, K. Kaasbjerg, S. Lysgaard, J. Bergmann Maronsson, T. Maxson, T. Olsen, L. Pastewka, A. Peterson, C. Rostgaard, J. Schiotz, O. Schutt, M. Strange, K. S. Thygesen, T. Vegge, et al., J Phys Condens Matter. 2017, 29, 273002.
M. Doucet, J. H. Cho, G. Alina, Z. Attala, J. Bakker, W. Bouwman, R. Bourne, P. Butler, I. Cadwallader-Jones, K. Campbell, T. Cooper-Benun, C. Durniak, L. Forster, P. Gilbert, M. Gonzalez, R. Heenan, A. Jackson, S. King, P. Kienzle, J. Krzywon, B. Maranville, R. Murphy, T. Nielsen, L. O'Driscoll, W. Potrzebowski, S. Prescott, R. Ferraz Leal, P. Rozyczko, T. Snow, A. Washington, et al., SasView version 5.0.5. Zenodo.
R. O. Matt Newville, A. Nelson, T. Stensitzki, A. Ingargiola, D. Allan, A. Fox, F. Carter, R. O. Michał, D. Pustakhod, lneuhaus, S. Weigand, A. Aristov, C. D. Glenn, mgunyho, Mark, A. L. R. Hansen, G. Pasquevich, L. Foks, N. Zobrist, O. Frost, Stuermer, azelcer, A. Polloreno, A. Persaud, J. H. Nielsen, M. Pompili, P. Eendebak, 2023. Imfit/lmfit-py: 1.2.2. Zenodo.