Synthesis and Unique Behaviors of High-Purity HEA Nanoparticles Using Femtosecond Laser Ablation.

electrocatalysis femtosecond laser high-entropy alloy laser ablation nanoparticle synthesis oxygen reduction reaction scalable synthesis

Journal

Nanomaterials (Basel, Switzerland)
ISSN: 2079-4991
Titre abrégé: Nanomaterials (Basel)
Pays: Switzerland
ID NLM: 101610216

Informations de publication

Date de publication:
21 Mar 2024
Historique:
received: 02 02 2024
revised: 18 03 2024
accepted: 18 03 2024
medline: 27 3 2024
pubmed: 27 3 2024
entrez: 27 3 2024
Statut: epublish

Résumé

High-entropy alloys (HEAs) are a class of metal alloys consisting of four or more molar equal or near-equal elements. HEA nanomaterials have garnered significant interest due to their wide range of applications, such as electrocatalysis, welding, and brazing. Their unique multi-principle high-entropy effect allows for the tailoring of the alloy composition to facilitate specific electrochemical reactions. This study focuses on the synthesis of high-purity HEA nanoparticles using the method of femtosecond laser ablation synthesis in liquid. The use of ultrashort energy pulses in femtosecond lasers enables uniform ablation of materials at significantly lower power levels compared to longer pulse or continuous pulse lasers. We investigate how various femtosecond laser parameters affect the morphology, phase, and other characteristics of the synthesized nanoparticles. An innovative aspect of our solution is its ability to rapidly generate multi-component nanoparticles with a high fidelity as the input multi-component target material at a significant yielding rate. Our research thus focuses on a novel synthesis of high-entropy alloying CuCoMn

Identifiants

pubmed: 38535702
pii: nano14060554
doi: 10.3390/nano14060554
pii:
doi:

Types de publication

Journal Article

Langues

eng

Auteurs

David Fieser (D)

Department of Mechanical, Aerospace, Biomedical Engineering, The University of Tennessee, Knoxville, 1512 Middle Drive, Knoxville, TN 37996, USA.

Yucheng Lan (Y)

Department of Physics and Engineering, Morgan State University, 1700 East Cold Spring Lane, Baltimore, MD 21251, USA.

Antonino Gulino (A)

Chemistry Department, University of Catania, Viale A. Doria 6, 95125 Catania, Italy.

Giuseppe Compagnini (G)

Chemistry Department, University of Catania, Viale A. Doria 6, 95125 Catania, Italy.

Doug Aaron (D)

Department of Mechanical, Aerospace, Biomedical Engineering, The University of Tennessee, Knoxville, 1512 Middle Drive, Knoxville, TN 37996, USA.

Matthew Mench (M)

Department of Mechanical, Aerospace, Biomedical Engineering, The University of Tennessee, Knoxville, 1512 Middle Drive, Knoxville, TN 37996, USA.

Denzel Bridges (D)

Department of Mechanical, Aerospace, Biomedical Engineering, The University of Tennessee, Knoxville, 1512 Middle Drive, Knoxville, TN 37996, USA.

Hugh Shortt (H)

Department of Materials Science and Engineering, The University of Tennessee, Knoxville, 1512 Middle Drive, Knoxville, TN 37996, USA.

Peter Liaw (P)

Department of Materials Science and Engineering, The University of Tennessee, Knoxville, 1512 Middle Drive, Knoxville, TN 37996, USA.

Anming Hu (A)

Department of Mechanical, Aerospace, Biomedical Engineering, The University of Tennessee, Knoxville, 1512 Middle Drive, Knoxville, TN 37996, USA.

Classifications MeSH