Mechanism of autocatalytic activation during proteasome assembly.


Journal

Nature structural & molecular biology
ISSN: 1545-9985
Titre abrégé: Nat Struct Mol Biol
Pays: United States
ID NLM: 101186374

Informations de publication

Date de publication:
10 Apr 2024
Historique:
received: 14 11 2023
accepted: 04 03 2024
medline: 11 4 2024
pubmed: 11 4 2024
entrez: 10 4 2024
Statut: aheadofprint

Résumé

Many large molecular machines are too elaborate to assemble spontaneously and are built through ordered pathways orchestrated by dedicated chaperones. During assembly of the core particle (CP) of the proteasome, where protein degradation occurs, its six active sites are simultaneously activated via cleavage of N-terminal propeptides. Such activation is autocatalytic and coupled to fusion of two half-CP intermediates, which protects cells by preventing activation until enclosure of the active sites within the CP interior. Here we uncover key mechanistic aspects of autocatalytic activation, which proceeds through alignment of the β5 and β2 catalytic triad residues, respectively, with these triads being misaligned before fusion. This mechanism contrasts with most other zymogens, in which catalytic centers are preformed. Our data also clarify the mechanism by which individual subunits can be added in a precise, temporally ordered manner. This work informs two decades-old mysteries in the proteasome field, with broader implications for protease biology and multisubunit complex assembly.

Identifiants

pubmed: 38600323
doi: 10.1038/s41594-024-01262-1
pii: 10.1038/s41594-024-01262-1
doi:

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Informations de copyright

© 2024. The Author(s), under exclusive licence to Springer Nature America, Inc.

Références

Jäger, S., Groll, M., Huber, R., Wolf, D. H. & Heinemeyer, W. Proteasome beta-type subunits: unequal roles of propeptides in core particle maturation and a hierarchy of active site function. J. Mol. Biol. 291, 997–1013 (1999).
pubmed: 10452902 doi: 10.1006/jmbi.1999.2995
Schnell, H. M., Walsh, R. M., Rawson, S. & Hanna, J. Chaperone-mediated assembly of the proteasome core particle – recent developments and structural insights. J. Cell Sci. 135, jcs259622 (2022).
pubmed: 35451017 pmcid: 9080555 doi: 10.1242/jcs.259622
Watanabe, A., Yashiroda, H., Ishihara, S., Lo, M. & Murata, S. The molecular mechanisms governing the assembly of the immuno- and thymoproteasomes in the presence of constitutive proteasomes. Cells 11, 1580 (2022).
pubmed: 35563886 pmcid: 9105311 doi: 10.3390/cells11091580
Chen, P. & Hochstrasser, M. Autocatalytic subunit processing couples active site formation in the 20S proteasome to completion of assembly. Cell 86, 961–972 (1996).
pubmed: 8808631 doi: 10.1016/S0092-8674(00)80171-3
Hirano, Y. et al. Dissecting beta-ring assembly pathway of the mammalian 20S proteasome. EMBO J. 27, 2204–2213 (2008).
pubmed: 18650933 pmcid: 2519102 doi: 10.1038/emboj.2008.148
Schnell, H. M. et al. Structures of chaperone-associated assembly intermediates reveal coordinated mechanisms of proteasome biogenesis. Nat. Struct. Mol. Biol. 28, 418–425 (2021).
pubmed: 33846632 pmcid: 8160580 doi: 10.1038/s41594-021-00583-9
Seemüller, E., Lupas, A. & Baumeister, W. Autocatalytic processing of the 20S proteasome. Nature 382, 468–470 (1996).
pubmed: 8684489 doi: 10.1038/382468a0
Huber, E. M. et al. A unified mechanism for proteolysis and autocatalytic activation in the 20S proteasome. Nat. Commun. 7, 10900 (2016).
pubmed: 26964885 pmcid: 4792962 doi: 10.1038/ncomms10900
Groll, M. et al. Structure of 20S proteasome from yeast at 2.4 Å resolution. Nature 386, 463–471 (1997).
pubmed: 9087403 doi: 10.1038/386463a0
Ramos, P. C., Marques, A. J., London, M. K. & Dohmen, R. J. Role of C-terminal extensions of subunits beta2 and beta7 in assembly and activity of eukaryotic proteasomes. J. Biol. Chem. 279, 14323–14330 (2004).
pubmed: 14722099 doi: 10.1074/jbc.M308757200
Walsh, R. M. et al. Structure of the preholoproteasome reveals late steps in proteasome core particle biogenesis. Nat. Struct. Mol. Biol. 30, 1516–1524 (2023).
pubmed: 37653242 pmcid: 10879985 doi: 10.1038/s41594-023-01081-w
Gerlinger, U. M., Gückel, R., Hoffmann, M., Wolf, D. H. & Hilt, W. Yeast cycloheximide-resistant crl mutants are proteasome mutants defective in protein degradation. Mol. Biol. Cell 8, 2487–2499 (1997).
pubmed: 9398670 pmcid: 25722 doi: 10.1091/mbc.8.12.2487
Kock, M. et al. Proteasome assembly from 15S precursors involves major conformational changes and recycling of the Pba1–Pba2 chaperone. Nat. Commun. 6, 6123 (2015).
pubmed: 25609009 doi: 10.1038/ncomms7123
Li, X., Li, Y., Arendt, C. S. & Hochstrasser, M. Distinct elements in the proteasomal β5 subunit propeptide required for autocatalytic processing and proteasome assembly. J. Biol. Chem. 291, 1991–2003 (2016).
pubmed: 26627836 doi: 10.1074/jbc.M115.677047
Xie, Y. & Varshavsky, A. RPN4 is a ligand, substrate, and transcriptional regulator of the 26S proteasome: a negative feedback circuit. Proc. Natl Acad. Sci. USA 98, 3056–3061 (2001).
pubmed: 11248031 pmcid: 30606 doi: 10.1073/pnas.071022298
Guerra-Moreno, A. & Hanna, J. Induction of proteotoxic stress by the mycotoxin patulin. Toxicol. Lett. 276, 85–91 (2017).
pubmed: 28529145 pmcid: 5516271 doi: 10.1016/j.toxlet.2017.05.015
Ramos, P. C., Höckendorff, J., Johnson, E. S., Varshavsky, A. & Dohmen, R. J. Ump1p is required for proper maturation of the 20S proteasome and becomes its substrate upon completion of the assembly. Cell 92, 489–499 (1998).
pubmed: 9491890 doi: 10.1016/S0092-8674(00)80942-3
Marques, A. J., Glanemann, C., Ramos, P. C. & Dohmen, R. J. The C-terminal extension of the beta7 subunit and activator complexes stabilize nascent 20S proteasomes and promote their maturation. J. Biol. Chem. 282, 34869–34876 (2007).
pubmed: 17911101 doi: 10.1074/jbc.M705836200
Arendt, C. S. & Hochstrasser, M. Eukaryotic 20S proteasome catalytic subunit propeptides prevent active site inactivation by N-terminal acetylation and promote particle assembly. EMBO J. 18, 3575–3585 (1999).
pubmed: 10393174 pmcid: 1171436 doi: 10.1093/emboj/18.13.3575
Matias, A. C., Matos, J., Dohmen, R. J. & Ramos, P. C. Hsp70 and Hsp110 chaperones promote early steps of proteasome assembly. Biomolecules 13, 11 (2022).
pubmed: 36671396 pmcid: 9855889 doi: 10.3390/biom13010011
Khan, A. R. & James, M. N. Molecular mechanisms for the conversion of zymogens to active proteolytic enzymes. Protein Sci. 7, 815–836 (1998).
pubmed: 9568890 pmcid: 2143990 doi: 10.1002/pro.5560070401
Richter, C., Tanaka, T. & Yada, R. Y. Mechanism of activation of the gastric aspartic proteinases: pepsinogen, progastricsin and prochymosin. Biochem. J. 335, 481–490 (1998).
pubmed: 9794784 pmcid: 1219805 doi: 10.1042/bj3350481
Arolas, J. L., Goulas, T., Cuppari, A. & Gomis-Rüth, F. X. Multiple architectures and mechanisms of latency in metallopeptidase zymogens. Chem. Rev. 118, 5581–5597 (2018).
pubmed: 29775286 doi: 10.1021/acs.chemrev.8b00030
Poli, M. C. et al. Heterozygous truncating variants in POMP escape nonsense-mediated decay and cause a unique immune dysregulatory syndrome. Am. J. Hum. Genet. 102, 1126–1142 (2018).
pubmed: 29805043 pmcid: 5992134 doi: 10.1016/j.ajhg.2018.04.010
de Jesus, A. A. et al. Novel proteasome assembly chaperone mutations in PSMG2/PAC2 cause the autoinflammatory interferonopathy CANDLE/PRAAS4. J. Allergy Clin. Immunol. 143, 1939–1943.e8 (2019).
pubmed: 30664889 pmcid: 6565382 doi: 10.1016/j.jaci.2018.12.1012
Dahlqvist, J. et al. A single-nucleotide deletion in the POMP 5′ UTR causes a transcriptional switch and altered epidermal proteasome distribution in KLICK genodermatosis. Am. J. Hum. Genet. 86, 596–603 (2010).
pubmed: 20226437 pmcid: 2850438 doi: 10.1016/j.ajhg.2010.02.018
Ansar, M. et al. Biallelic variants in PSMB1 encoding the proteasome subunit β6 cause impairment of proteasome function, microcephaly, intellectual disability, developmental delay and short stature. Hum. Mol. Genet. 29, 1132–1143 (2020).
pubmed: 32129449 doi: 10.1093/hmg/ddaa032
Hwang, G.-W., Ishida, Y. & Naganuma, A. Identification of F-box proteins that are involved in resistance to methylmercury in Saccharomyces cerevisiae. FEBS Lett. 580, 6813–6818 (2006).
pubmed: 17141224 doi: 10.1016/j.febslet.2006.11.045
Wani, P. S., Rowland, M. A., Ondracek, A., Deeds, E. J. & Roelofs, J. Maturation of the proteasome core particle induces an affinity switch that controls regulatory particle association. Nat. Commun. 6, 6384 (2015).
pubmed: 25812915 doi: 10.1038/ncomms7384
Weisshaar, N., Welsch, H., Guerra-Moreno, A. & Hanna, J. Phospholipase Lpl1 links lipid droplet function with quality control protein degradation. Mol. Biol. Cell 28, 716–725 (2017).
pubmed: 28100635 pmcid: 5349779 doi: 10.1091/mbc.e16-10-0717
Mastronarde, D. N. Automated electron microscope tomography using robust prediction of specimen movements. J. Struct. Biol. 152, 36–51 (2005).
pubmed: 16182563 doi: 10.1016/j.jsb.2005.07.007
Zheng, S. Q. et al. MotionCor2: anisotropic correction of beam-induced motion for improved cryo-electron microscopy. Nat. Methods 14, 331–332 (2017).
pubmed: 28250466 pmcid: 5494038 doi: 10.1038/nmeth.4193
Rohou, A. & Grigorieff, N. CTFFIND4: fast and accurate defocus estimation from electron micrographs. J. Struct. Biol. 192, 216–221 (2015).
pubmed: 26278980 pmcid: 6760662 doi: 10.1016/j.jsb.2015.08.008
Wagner, T. et al. SPHIRE-crYOLO is a fast and accurate fully automated particle picker for cryo-EM. Commun. Biol. 2, 218 (2019).
pubmed: 31240256 pmcid: 6584505 doi: 10.1038/s42003-019-0437-z
Scheres, S. H. W. RELION: implementation of a Bayesian approach to cryo-EM structure determination. J. Struct. Biol. 180, 519–530 (2012).
pubmed: 23000701 pmcid: 3690530 doi: 10.1016/j.jsb.2012.09.006
Punjani, A., Rubinstein, J. L., Fleet, D. J. & Brubaker, M. A. CryoSPARC: algorithms for rapid unsupervised cryo-EM structure determination. Nat. Methods 14, 290–296 (2017).
pubmed: 28165473 doi: 10.1038/nmeth.4169
Zhong, E. D., Bepler, T., Berger, B. & Davis, J. H. CryoDRGN: reconstruction of heterogeneous cryo-EM structures using neural networks. Nat. Methods 18, 176–185 (2021).
pubmed: 33542510 pmcid: 8183613 doi: 10.1038/s41592-020-01049-4
Morin, A. et al. Collaboration gets the most out of software. eLife 2, e01456 (2013).
pubmed: 24040512 pmcid: 3771563 doi: 10.7554/eLife.01456
Jamali, K. et al. Automated model building and protein identification in cryo-EM maps. Nature https://doi.org/10.1038/s41586-024-07215-4 (2024).
Pettersen, E. F. et al. UCSF Chimera – a visualization system for exploratory research and analysis. J. Comput. Chem. 25, 1605–1612 (2004).
pubmed: 15264254 doi: 10.1002/jcc.20084
Emsley, P., Lohkamp, B., Scott, W. G. & Cowtan, K. Features and development of Coot. Acta Crystallogr. D Biol. Crystallogr. 66, 486–501 (2010).
pubmed: 20383002 pmcid: 2852313 doi: 10.1107/S0907444910007493
Croll, T. I. ISOLDE: a physically realistic environment for model building into low-resolution electron-density maps. Acta Crystallogr. D Struct. Biol. 74, 519–530 (2018).
pubmed: 29872003 pmcid: 6096486 doi: 10.1107/S2059798318002425
Liebschner, D. et al. Macromolecular structure determination using X-rays, neutrons and electrons: recent developments in Phenix. Acta Crystallogr. D Struct. Biol. 75, 861–877 (2019).
pubmed: 31588918 pmcid: 6778852 doi: 10.1107/S2059798319011471
Kao, A. et al. Development of a novel cross-linking strategy for fast and accurate identification of cross-linked peptides of protein complexes. Mol. Cell Proteomics 10, M110.002212 (2011).
pubmed: 20736410 doi: 10.1074/mcp.M110.002212
Gutierrez, C. B. et al. Developing an acidic residue reactive and sulfoxide-containing MS-cleavable homobifunctional cross-linker for probing protein–protein interactions. Anal. Chem. 88, 8315–8322 (2016).
pubmed: 27417384 pmcid: 4989248 doi: 10.1021/acs.analchem.6b02240
Wiśniewski, J. R., Zougman, A., Nagaraj, N. & Mann, M. Universal sample preparation method for proteome analysis. Nat. Methods 6, 359–362 (2009).
pubmed: 19377485 doi: 10.1038/nmeth.1322
Jiao, F. et al. Two-dimensional fractionation method for proteome-wide cross-linking mass spectrometry analysis. Anal. Chem. 94, 4236–4242 (2022).
pubmed: 35235311 pmcid: 9056026 doi: 10.1021/acs.analchem.1c04485
Jiao, F. et al. Exploring an alternative cysteine-reactive chemistry to enable proteome-wide PPI analysis by cross-linking mass spectrometry. Anal. Chem. 95, 2532–2539 (2023).
pubmed: 36652389 pmcid: 10284117 doi: 10.1021/acs.analchem.2c04986
Finley, D., Ozkaynak, E. & Varshavsky, A. The yeast polyubiquitin gene is essential for resistance to high temperatures, starvation, and other stresses. Cell 48, 1035–1046 (1987).
pubmed: 3030556 doi: 10.1016/0092-8674(87)90711-2
Gietz, R. D. & Sugino, A. New yeast–Escherichia coli shuttle vectors constructed with in vitro mutagenized yeast genes lacking six-base pair restriction sites. Gene 74, 527–534 (1988).
pubmed: 3073106 doi: 10.1016/0378-1119(88)90185-0

Auteurs

Benjamin Velez (B)

Department of Pathology, Harvard Medical School and Brigham and Women's Hospital, Boston, MA, USA.

Richard M Walsh (RM)

Harvard Cryo-Electron Microscopy Center for Structural Biology, Harvard Medical School, Boston, MA, USA.
Department of Biological Chemistry and Molecular Pharmacology, Blavatnik Institute, Harvard Medical School, Boston, MA, USA.

Shaun Rawson (S)

Harvard Cryo-Electron Microscopy Center for Structural Biology, Harvard Medical School, Boston, MA, USA.
Department of Biological Chemistry and Molecular Pharmacology, Blavatnik Institute, Harvard Medical School, Boston, MA, USA.

Aida Razi (A)

Department of Pathology, Harvard Medical School and Brigham and Women's Hospital, Boston, MA, USA.

Lea Adams (L)

Department of Pathology, Harvard Medical School and Brigham and Women's Hospital, Boston, MA, USA.

Erignacio Fermin Perez (EF)

Department of Pathology, Harvard Medical School and Brigham and Women's Hospital, Boston, MA, USA.

Fenglong Jiao (F)

Department of Physiology and Biophysics, University of California-Irvine, Irvine, CA, USA.

Marie Blickling (M)

Department of Pathology, Harvard Medical School and Brigham and Women's Hospital, Boston, MA, USA.

Tamayanthi Rajakumar (T)

Department of Pathology, Harvard Medical School and Brigham and Women's Hospital, Boston, MA, USA.

Darlene Fung (D)

Department of Pathology, Harvard Medical School and Brigham and Women's Hospital, Boston, MA, USA.

Lan Huang (L)

Department of Physiology and Biophysics, University of California-Irvine, Irvine, CA, USA.

John Hanna (J)

Department of Pathology, Harvard Medical School and Brigham and Women's Hospital, Boston, MA, USA. jwhanna@bwh.harvard.edu.

Classifications MeSH