Enhancing the Efficiency and Stability of Tin-Lead Perovskite Solar Cells via Sodium Hydroxide Dedoping of PEDOT:PSS.

charge carrier recombination doping narrow‐bandgap perovskite pedot:pss sn‐pb perovskite

Journal

Small methods
ISSN: 2366-9608
Titre abrégé: Small Methods
Pays: Germany
ID NLM: 101724536

Informations de publication

Date de publication:
18 Apr 2024
Historique:
revised: 09 04 2024
received: 01 04 2024
medline: 18 4 2024
pubmed: 18 4 2024
entrez: 18 4 2024
Statut: aheadofprint

Résumé

Tin-lead (Sn-Pb) perovskite solar cells (PSCs) have gained interest as candidates for the bottom cell of all-perovskite tandem solar cells due to their broad absorption of the solar spectrum. A notable challenge arises from the prevalent use of the hole transport layer, PEDOT:PSS, known for its inherently high doping level. This high doping level can lead to interfacial recombination, imposing a significant limitation on efficiency. Herein, NaOH is used to dedope PEDOT:PSS, with the aim of enhancing the efficiency of Sn-Pb PSCs. Secondary ion mass spectrometer profiles indicate that sodium ions diffuse into the perovskite layer, improving its crystallinity and enlarging its grains. Comprehensive evaluations, including photoluminescence and nanosecond transient absorption spectroscopy, confirm that dedoping significantly reduces interfacial recombination, resulting in an open-circuit voltage as high as 0.90 V. Additionally, dedoping PEDOT:PSS leads to increased shunt resistance and high fill factor up to 0.81. As a result of these improvements, the power conversion efficiency is enhanced from 19.7% to 22.6%. Utilizing NaOH to dedope PEDOT:PSS also transitions its nature from acidic to basic, enhancing stability and exhibiting less than a 7% power conversion efficiency loss after 1176 h of storage in N

Identifiants

pubmed: 38634222
doi: 10.1002/smtd.202400302
doi:

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Pagination

e2400302

Subventions

Organisme : National Science and Technology Council
ID : 110-2222-E-005-005 -MY3
Organisme : National Science and Technology Council
ID : 112-2628-E-005 -002
Organisme : National Science and Technology Council
ID : 112-2218-E-007-020-
Organisme : Royal Society University Research Fellowship
ID : URF/R1/221834
Organisme : National Research Foundation of Korea
Organisme : Engineering and Physical Sciences Research Council
ID : EP/S030727/1
Organisme : Royal Society
ID : RF/ERE/221066
Organisme : Royal Commission for the Exhibition of 1851
Organisme : Ministry of Education

Informations de copyright

© 2024 Wiley‐VCH GmbH.

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Auteurs

Dong-Tai Wu (DT)

Department of Chemical Engineering, National Chung Hsing University, 145 Xingda Road, Taichung, 402-27, Taiwan.

Wen-Xian Zhu (WX)

Department of Chemical Engineering, National Chung Hsing University, 145 Xingda Road, Taichung, 402-27, Taiwan.

Yueyao Dong (Y)

School of Engineering and Materials Science, Queen Mary University of London, London, E1 4NS, UK.

Matyas Daboczi (M)

Department of Chemical Engineering and Centre for Processable Electronics, Imperial College London, London, SW7 2AZ, UK.

Gayoung Ham (G)

Department of Energy Convergence and Climate Change, Kyungpook National University, Daegu, 41566, Republic of Korea.

Hsing-Jung Hsieh (HJ)

Department of Chemical Engineering, National Chung Hsing University, 145 Xingda Road, Taichung, 402-27, Taiwan.

Chi-Jing Huang (CJ)

Department of Chemical Engineering, National Chung Hsing University, 145 Xingda Road, Taichung, 402-27, Taiwan.

Weidong Xu (W)

Department of Chemical Engineering and Biotechnology, University of Cambridge, Philippa Fawcett Drive, Cambridge, CB3 0AS, UK.

Charlie Henderson (C)

Department of Physics and Centre for Processable Electronics, Imperial College London, London, SW7 2AZ, UK.

Ji-Seon Kim (JS)

Department of Physics and Centre for Processable Electronics, Imperial College London, London, SW7 2AZ, UK.

Salvador Eslava (S)

Department of Chemical Engineering and Centre for Processable Electronics, Imperial College London, London, SW7 2AZ, UK.

Hyojung Cha (H)

Department of Energy Convergence and Climate Change, Kyungpook National University, Daegu, 41566, Republic of Korea.
Department of Hydrogen and Renewable Energy, Kyungpook National University, Daegu, 41566, Republic of Korea.

Thomas J Macdonald (TJ)

School of Engineering and Materials Science, Queen Mary University of London, London, E1 4NS, UK.

Chieh-Ting Lin (CT)

Department of Chemical Engineering, National Chung Hsing University, 145 Xingda Road, Taichung, 402-27, Taiwan.
Innovation and Development Center of Sustainable Agriculture, National Chung Hsing University, Taichung City, 402, Taiwan.

Classifications MeSH