Testing functional anchor groups for the efficient immobilization of molecular catalysts on silver surfaces.
Journal
Communications chemistry
ISSN: 2399-3669
Titre abrégé: Commun Chem
Pays: England
ID NLM: 101725670
Informations de publication
Date de publication:
10 May 2024
10 May 2024
Historique:
received:
13
12
2022
accepted:
23
04
2024
medline:
10
5
2024
pubmed:
10
5
2024
entrez:
9
5
2024
Statut:
epublish
Résumé
Modifications of complexes by attachment of anchor groups are widely used to control molecule-surface interactions. This is of importance for the fabrication of (catalytically active) hybrid systems, viz. of surface immobilized molecular catalysts. In this study, the complex fac-Re(
Identifiants
pubmed: 38724592
doi: 10.1038/s42004-024-01186-3
pii: 10.1038/s42004-024-01186-3
doi:
Types de publication
Journal Article
Langues
eng
Pagination
107Subventions
Organisme : Deutsche Forschungsgemeinschaft (German Research Foundation)
ID : 217133147/SFB 1073
Organisme : Deutsche Forschungsgemeinschaft (German Research Foundation)
ID : 217133147/SFB 1073
Organisme : Deutsche Forschungsgemeinschaft (German Research Foundation)
ID : 217133147/SFB 1073
Organisme : Deutsche Forschungsgemeinschaft (German Research Foundation)
ID : 4391096 (Me1313/15-2).
Informations de copyright
© 2024. The Author(s).
Références
Ulrich, S. et al. Modifying the adsorption characteristic of inert silica films by inserting anchoring sites. Phys. Rev. Lett. 102, 016102 (2009).
pubmed: 19257215
doi: 10.1103/PhysRevLett.102.016102
Granja, A., Alonso, J. A., Cabria, I. & López, M. J. Competition between molecular and dissociative adsorption of hydrogen on palladium clusters deposited on defective graphene. RSC Adv. 5, 47945–47953 (2015).
doi: 10.1039/C5RA08091F
Zhang, J. et al. A promising anchor group for efficient organic dye sensitized solar cells with iodine-free redox shuttles: a theoretical evaluation. J. Mater. Chem. A 1, 14000–14007 (2013).
doi: 10.1039/c3ta12311a
Zhao, X. & Stadler, R. DFT-based study of electron transport through ferrocene compounds with different anchor groups in different adsorption configurations of an STM setup. Phys. Rev. B 99, 045431 (2019).
doi: 10.1103/PhysRevB.99.045431
Mayor, M. et al. Electric current through a molecular rod—relevance of the position of the anchor groups. Angew. Chem. Int. Ed. 42, 5834–5838 (2003).
doi: 10.1002/anie.200352179
Huang, M. et al. Developing longer-lived single molecule junctions with a functional flexible electrode. Small 17, 1–7 (2021).
doi: 10.1002/smll.202101911
Limburg, B. et al. Anchor groups for graphene-porphyrin single-molecule transistors. Adv. Funct. Mater. 28, 1803629 (2018).
doi: 10.1002/adfm.201803629
Koike, K. et al. Key process of the photocatalytic reduction of CO
Clark, M. L. et al. CO
pubmed: 30468391
doi: 10.1021/jacs.8b09852
Clark, M. L., Cheung, P. L., Lessio, M., Carter, E. A. & Kubiak, C. P. Kinetic and mechanistic effects of bipyridine (bpy) substituent, labile ligand, and brønsted acid on electrocatalytic CO
doi: 10.1021/acscatal.7b03971
Paul, L. A. et al. A dinuclear rhenium complex in the electrochemically driven homogeneous and heterogeneous H+/CO2-reduction. Dalt. Trans. 49, 8367–8374 (2020).
doi: 10.1039/D0DT00381F
Materna, K. L., Crabtree, R. H. & Brudvig, G. W. Anchoring groups for photocatalytic water oxidation on metal oxide surfaces. Chem. Soc. Rev. 46, 6099–6110 (2017).
pubmed: 28640299
doi: 10.1039/C7CS00314E
Lindner, M. et al. Importance of the anchor group position (para versus meta) in tetraphenylmethane tripods: synthesis and self-assembly features. Chem. A Eur. J. 22, 13218–13235 (2016).
doi: 10.1002/chem.201602019
Li, Z., Tang, J. & Zhong, Y. Multidentate anchors for surface functionalization. Chem. Asian J. 14, 3119–3126 (2019).
pubmed: 31389657
doi: 10.1002/asia.201900989
Rajabi, S. et al. Water oxidizing diruthenium electrocatalysts immobilized on carbon nanotubes: effects of the number and positioning of pyrene anchors. ACS Catal. 10, 10614–10626 (2020).
doi: 10.1021/acscatal.0c01577
Anfuso, C. L. et al. Orientation of a series of CO2 reduction catalysts on single crystal TiO2 probed by phase-sensitive vibrational sum frequency generation spectroscopy (PS-VSFG). J. Phys. Chem. C. 116, 24107–24114 (2012).
doi: 10.1021/jp307406j
Jones, A. O. F. et al. Thermal stability and molecular ordering of organic semiconductor monolayers: effect of an anchor group. ChemPhysChem 16, 1712–1718 (2015).
pubmed: 25827354
doi: 10.1002/cphc.201500098
Asbury, J. B., Hao, E., Wang, Y. & Lian, T. Bridge length-dependent ultrafast electron transfer from re polypyridyl complexes to nanocrystalline TiO2 thin films studied by femtosecond infrared spectroscopy. J. Phys. Chem. B 104, 11957–11964 (2000).
doi: 10.1021/jp002541g
Hawecker, J., Lehn, J. M. & Ziessel, R. Efficient photochemical reduction of CO2 to CO by visible light irradiation of systems containing Re(bipy)(CO)3X or Ru(bipy) 32+-Co2+ combinations as homogeneous catalysts. J. Chem. Soc. Chem. Commun. 536–538 (1983).
Cattaneo, M. et al. 2,2′-bipyridine equipped with a disulfide/dithiol switch for coupled two-electron and two-proton transfer. Chem. A Eur. J. 24, 4864–4870 (2018).
doi: 10.1002/chem.201705022
Hua, S.-A. et al. A bioinspired disulfide/dithiol redox switch in a rhenium complex as proton, H atom, and hydride transfer reagent. J. Am. Chem. Soc. 143, 6238–6247 (2021).
pubmed: 33861085
doi: 10.1021/jacs.1c01763
Cattaneo, M. et al. Robust binding of disulfide-substituted rhenium bipyridyl complexes for CO2 reduction on gold electrodes. Front. Chem. 8, 1–10 (2020).
doi: 10.3389/fchem.2020.00086
Bunjes, O. et al. Ordering a rhenium catalyst on Ag(001) through molecule-surface step interaction. Commun. Chem. 5, 3 (2022).
pubmed: 36697683
pmcid: 9814538
doi: 10.1038/s42004-021-00617-9
Bunjes, O. et al. Making and breaking of chemical bonds in single nanoconfined molecules. Sci. Adv. 8, eabq7776 (2022).
pubmed: 36083910
pmcid: 9462694
doi: 10.1126/sciadv.abq7776
Sone, K. & Fukuda, Y. Inorganic thermochromism. 10, (Springer Berlin Heidelberg, 1987).
Spurgeon, P. M. et al. Characteristics of sulfur atoms adsorbed on Ag(100), Ag(110), and Ag(111) as probed with scanning tunneling microscopy: experiment and theory. Phys. Chem. Chem. Phys. 21, 10540–10551 (2019).
pubmed: 31073566
doi: 10.1039/C9CP01626K
Chelvayohan, M. & Mee, C. H. B. Work function measurements on (110), (100) and (111) surfaces of silver. J. Phys. C. Solid State Phys. 15, 2305–2312 (1982).
doi: 10.1088/0022-3719/15/10/029
Sandroff, C. J. & Herschbach, D. R. Surface-enhanced Raman study of organic sulfides adsorbed on silver: facile cleavage of sulfur-sulfur and carbon-sulfur bonds. J. Phys. Chem. 86, 3277–3279 (1982).
doi: 10.1021/j100214a002
Kondoh, H., Tsukabayashi, H., Yokoyama, T. & Ohta, T. S K-edge X-ray absorption fine structure study of vacuum-deposited dihexyldisulfide on Ag(100). Surf. Sci. 489, 20–28 (2001).
doi: 10.1016/S0039-6028(01)01181-5
Tersoff, J. & Hamann, D. R. Theory of the scanning tunneling microscope. Phys. Rev. B 31, 805–813 (1985).
doi: 10.1103/PhysRevB.31.805
Shaporenko, A., Brunnbauer, M., Terfort, A., Grunze, M. & Zharnikov, M. Structural forces in self-assembled monolayers: terphenyl-substituted alkanethiols on noble metal substrates. J. Phys. Chem. B 108, 14462–14469 (2004).
doi: 10.1021/jp0400521
Yang, W. et al. Electrocatalytic CO
pubmed: 30040401
doi: 10.1021/acs.inorgchem.8b01775
Benson, E. E. & Kubiak, C. P. Structural investigations into the deactivation pathway of the CO
doi: 10.1039/c2cc32617e
Liang, W. et al. Site isolation leads to stable photocatalytic reduction of CO2 over a rhenium-based catalyst. Chem. A Eur. J. 21, 18576–18579 (2015).
doi: 10.1002/chem.201502796
Grice, K. A. & Kubiak, C. P. Recent studies of rhenium and manganese bipyridine carbonyl catalysts for the electrochemical reduction of CO
Neri, G., Donaldson, P. M. & Cowan, A. J. The role of electrode–catalyst interactions in enabling efficient CO
pubmed: 28895400
doi: 10.1021/jacs.7b06898
Kresse, G. & Hafner, J. Ab initio molecular dynamics for liquid metals. Phys. Rev. B 47, 558–561 (1993).
doi: 10.1103/PhysRevB.47.558
Kresse, G. & Furthmüller, J. Efficiency of ab-initio total energy calculations for metals and semiconductors using a plane-wave basis set. Comput. Mater. Sci. 6, 15–50 (1996).
doi: 10.1016/0927-0256(96)00008-0
Kresse, G. & Furthmüller, J. Efficient iterative schemes for ab initio total-energy calculations using a plane-wave basis set. Phys. Rev. B 54, 11169–11186 (1996).
doi: 10.1103/PhysRevB.54.11169
Blöchl, P. E. Projector augmented-wave method. Phys. Rev. B 50, 17953–17979 (1994).
doi: 10.1103/PhysRevB.50.17953
Kresse, G. & Joubert, D. From ultrasoft pseudopotentials to the projector augmented-wave method. Phys. Rev. B 59, 1758–1775 (1999).
doi: 10.1103/PhysRevB.59.1758
Klimeš, J., Bowler, D. R. & Michaelides, A. Van der Waals density functionals applied to solids. Phys. Rev. B 83, 195131 (2011).
doi: 10.1103/PhysRevB.83.195131
Malone, W., Yildirim, H., Matos, J. & Kara, A. A van der waals inclusive density functional theory study of the nature of bonding for thiophene adsorption on Ni(100) and Cu(100.) surfaces. J. Phys. Chem. C 121, 6090–6103 (2017).
Jarvis, S. P. et al. Physisorption controls the conformation and density of states of an adsorbed porphyrin. J. Phys. Chem. C. 119, 27982–27994 (2015).
doi: 10.1021/acs.jpcc.5b08350
Jarvis, S. P. et al. Measuring the mechanical properties of molecular conformers. Nat. Commun. 6, 8338 (2015).
pubmed: 26388232
doi: 10.1038/ncomms9338
Hofer, W. A., Foster, A. S. & Shluger, A. L. Theories of scanning probe microscopes at the atomic scale. Rev. Mod. Phys. 75, 1287–1331 (2003).
doi: 10.1103/RevModPhys.75.1287
Harikumar, K. R., McNab, I. R., Polanyi, J. C., Zabet-Khosousi, A. & Hofer, W. A. Imprinting self-assembled patterns of lines at a semiconductor surface, using heat, light, or electrons. Proc. Natl Acad. Sci. USA 108, 950–955 (2011).
pubmed: 20798058
doi: 10.1073/pnas.1006657107
Stukowski, A. Visualization and analysis of atomistic simulation data with OVITO–the open visualization tool. Model. Simul. Mater. Sci. Eng. 18, 015012 (2010).
doi: 10.1088/0965-0393/18/1/015012