ACKR3 Antagonism Enhances the Repair of Demyelinated Lesions Through Both Immunomodulatory and Remyelinating Effects.

ACKR3/CXCR7 CXCL11 CXCL12 Immunomodulation Multiple sclerosis Remyelination

Journal

Neurochemical research
ISSN: 1573-6903
Titre abrégé: Neurochem Res
Pays: United States
ID NLM: 7613461

Informations de publication

Date de publication:
31 May 2024
Historique:
received: 27 01 2024
accepted: 22 05 2024
revised: 16 04 2024
medline: 31 5 2024
pubmed: 31 5 2024
entrez: 31 5 2024
Statut: aheadofprint

Résumé

Addressing inflammation, demyelination, and associated neurodegeneration in inflammatory demyelinating diseases like multiple sclerosis (MS) remains challenging. ACT-1004-1239, a first-in-class and potent ACKR3 antagonist, currently undergoing clinical development, showed promise in preclinical MS models, reducing neuroinflammation and demyelination. However, its effectiveness in treating established disease and impact on remyelination after the occurrence of demyelinated lesions remain unexplored. This study assessed the therapeutic effect of ACT-1004-1239 in two demyelinating disease models. In the proteolipid protein (PLP)-induced experimental autoimmune encephalomyelitis (EAE) model, ACT-1004-1239 administered upon the detection of the first signs of paralysis, resulted in a dose-dependent reduction in EAE disease severity, concomitant with diminished immune cell infiltrates in the CNS and reduced demyelination. Notably, efficacy correlated with elevated plasma concentrations of CXCL11 and CXCL12, two pharmacodynamic biomarkers of ACKR3 antagonism. Combining ACT-1004-1239 with siponimod, an approved immunomodulatory treatment for MS, synergistically reduced EAE severity. In the cuprizone-induced demyelination model, ACT-1004-1239 administered after 5 weeks of cuprizone exposure, significantly accelerated remyelination, already quantifiable one week after cuprizone withdrawal. Additionally, ACT-1004-1239 penetrated the CNS, elevating brain CXCL12 concentrations. These results demonstrate that ACKR3 antagonism significantly reduces the severity of experimental demyelinating diseases, even when treatment is initiated therapeutically, after the occurrence of lesions. It confirms the dual mode of action of ACT-1004-1239, exhibiting both immunomodulatory effects by reducing neuroinflammation and promyelinating effects by accelerating myelin repair. The results further strengthen the rationale for evaluating ACT-1004-1239 in clinical trials for patients with demyelinating diseases.

Identifiants

pubmed: 38819698
doi: 10.1007/s11064-024-04173-1
pii: 10.1007/s11064-024-04173-1
doi:

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Informations de copyright

© 2024. The Author(s).

Références

Plemel JR, Liu W-Q, Yong VW (2017) Remyelination therapies: a new direction and challenge in multiple sclerosis. Nat Rev Drug Discovery 16(9):617–634
pubmed: 28685761 doi: 10.1038/nrd.2017.115
Cunniffe N, Coles A (2021) Promoting remyelination in multiple sclerosis. J Neurol 268(1):30–44
pubmed: 31190170 doi: 10.1007/s00415-019-09421-x
Melchor GS, Khan T, Reger JF, Huang JK (2019) Remyelination Pharmacotherapy investigations Highlight Diverse mechanisms underlying multiple sclerosis progression. ACS Pharmacol Translational Sci 2(6):372–386
doi: 10.1021/acsptsci.9b00068
Cruz-Orengo L, Holman DW, Dorsey D, Zhou L, Zhang P, Wright M et al (2011) CXCR7 influences leukocyte entry into the CNS parenchyma by controlling abluminal CXCL12 abundance during autoimmunity. J Exp Med 208(2):327–339
pubmed: 21300915 pmcid: 3039853 doi: 10.1084/jem.20102010
Chu T, Shields LBE, Zhang YP, Feng SQ, Shields CB, Cai J (2017) CXCL12/CXCR4/CXCR7 Chemokine Axis in the Central Nervous System: therapeutic targets for Remyelination in Demyelinating diseases. Neuroscientist 23(6):627–648
pubmed: 29283028 doi: 10.1177/1073858416685690
Pouzol L, Baumlin N, Sassi A, Tunis M, Marrie J, Vezzali E et al (2021) ACT-1004-1239, a first-in-class CXCR7 antagonist with both immunomodulatory and promyelinating effects for the treatment of inflammatory demyelinating diseases. FASEB J 35(3):e21431
pubmed: 33595155 doi: 10.1096/fj.202002465R
Banisadr G, Podojil JR, Miller SD, Miller RJ (2016) Pattern of CXCR7 gene expression in mouse brain under normal and inflammatory conditions. J Neuroimmune Pharmacol 11(1):26–35
pubmed: 25997895 doi: 10.1007/s11481-015-9616-y
Williams JL, Patel JR, Daniels BP, Klein RS (2014) Targeting CXCR7/ACKR3 as a therapeutic strategy to promote remyelination in the adult central nervous system. J Exp Med 211(5):791–799
pubmed: 24733828 pmcid: 4010893 doi: 10.1084/jem.20131224
Puchert M, Pelkner F, Stein G, Angelov DN, Boltze J, Wagner DC et al (2017) Astrocytic expression of the CXCL12 receptor, CXCR7/ACKR3 is a hallmark of the diseased, but not developing CNS. Mol Cell Neurosci 85:105–118
pubmed: 28889992 doi: 10.1016/j.mcn.2017.09.001
Ma W, Liu Y, Ellison N, Shen J (2013) Induction of C-X-C chemokine receptor type 7 (CXCR7) switches stromal cell-derived factor-1 (SDF-1) signaling and phagocytic activity in macrophages linked to atherosclerosis. J Biol Chem 288(22):15481–15494
pubmed: 23599431 pmcid: 3668710 doi: 10.1074/jbc.M112.445510
Bao J, Zhu J, Luo S, Cheng Y, Zhou S (2016) CXCR7 suppression modulates microglial chemotaxis to ameliorate experimentally-induced autoimmune encephalomyelitis. Biochem Biophys Res Commun 469(1):1–7
pubmed: 26607112 doi: 10.1016/j.bbrc.2015.11.059
Veenstra M, Williams DW, Calderon TM, Anastos K, Morgello S, Berman JW, Frontline Science (2017) CXCR7 mediates CD14(+)CD16(+) monocyte transmigration across the blood brain barrier: a potential therapeutic target for NeuroAIDS. J Leukoc Biol 102(5):1173–1185
pubmed: 28754798 pmcid: 5636044 doi: 10.1189/jlb.3HI0517-167R
Williams JL, Manivasagam S, Smith BC, Sim J, Vollmer LL, Daniels BP et al (2020) Astrocyte-T cell crosstalk regulates region-specific neuroinflammation. Glia 68(7):1361–1374
pubmed: 31961459 pmcid: 7317491 doi: 10.1002/glia.23783
Fumagalli A, Heuninck J, Pizzoccaro A, Moutin E, Koenen J, Séveno M et al (2020) The atypical chemokine receptor 3 interacts with Connexin 43 inhibiting astrocytic gap junctional intercellular communication. Nat Commun 11(1):4855
pubmed: 32978390 pmcid: 7519114 doi: 10.1038/s41467-020-18634-y
Huynh C, Brussee JM, Pouzol L, Fonseca M, Meyer Zu Schwabedissen HE, Dingemanse J, Sidharta PN (2021) Target engagement of the first-in-class CXCR7 antagonist ACT-1004-1239 following multiple-dose administration in mice and humans. Biomed Pharmacother 144:112363
pubmed: 34794236 doi: 10.1016/j.biopha.2021.112363
Sierro F, Biben C, Martinez-Munoz L, Mellado M, Ransohoff RM, Li M et al (2007) Disrupted cardiac development but normal hematopoiesis in mice deficient in the second CXCL12/SDF-1 receptor, CXCR7. Proc Natl Acad Sci U S A 104(37):14759–14764
pubmed: 17804806 pmcid: 1976222 doi: 10.1073/pnas.0702229104
Richard-Bildstein S, Aissaoui H, Pothier J, Schafer G, Gnerre C, Lindenberg E et al (2020) Discovery of the potent, selective, orally available CXCR7 antagonist ACT-1004-1239. J Med Chem 63(24):15864–15882
pubmed: 33314938 doi: 10.1021/acs.jmedchem.0c01588
Pouzol L, Sassi A, Baumlin N, Tunis M, Strasser DS, Lehembre F, Martinic MM (2021) CXCR7 antagonism reduces Acute Lung Injury Pathogenesis. Front Pharmacol 12:748740
pubmed: 34803691 pmcid: 8602191 doi: 10.3389/fphar.2021.748740
Andrews SP, Cox RJ (2016) Small molecule CXCR3 antagonists. J Med Chem 59(7):2894–2917
pubmed: 26535614 doi: 10.1021/acs.jmedchem.5b01337
Green AJ, Gelfand JM, Cree BA, Bevan C, Boscardin WJ, Mei F et al (2017) Clemastine fumarate as a remyelinating therapy for multiple sclerosis (ReBUILD): a randomised, controlled, double-blind, crossover trial. Lancet 390(10111):2481–2489
pubmed: 29029896 doi: 10.1016/S0140-6736(17)32346-2
Deshmukh VA, Tardif V, Lyssiotis CA, Green CC, Kerman B, Kim HJ et al (2013) A regenerative approach to the treatment of multiple sclerosis. Nature 502(7471):327–332
pubmed: 24107995 pmcid: 4431622 doi: 10.1038/nature12647
Liu L, Darnall L, Hu T, Choi K, Lane TE, Ransohoff RM (2010) Myelin repair is accelerated by inactivating CXCR2 on nonhematopoietic cells. J Neurosci 30(27):9074–9083
pubmed: 20610741 pmcid: 2917803 doi: 10.1523/JNEUROSCI.1238-10.2010
Kataoka H, Sugahara K, Shimano K, Teshima K, Koyama M, Fukunari A, Chiba K (2005) FTY720, sphingosine 1-phosphate receptor modulator, ameliorates experimental autoimmune encephalomyelitis by inhibition of T cell infiltration. Cell Mol Immunol 2(6):439–448
pubmed: 16426494
Fischer S, Proschmann U, Akgün K, Ziemssen T (2021) Lymphocyte counts and multiple sclerosis therapeutics: between mechanisms of action and treatment-limiting Side effects. Cells. ;10(11)
Sanchez-Alcaniz JA, Haege S, Mueller W, Pla R, Mackay F, Schulz S et al (2011) Cxcr7 controls neuronal migration by regulating chemokine responsiveness. Neuron 69(1):77–90
pubmed: 21220100 doi: 10.1016/j.neuron.2010.12.006
Bigaud M, Rudolph B, Briard E, Beerli C, Hofmann A, Hermes E et al (2021) Siponimod (BAF312) penetrates, distributes, and acts in the central nervous system: preclinical insights. Multiple Scler J - Experimental Translational Clin 7(4):20552173211049168
Gentile A, Musella A, Bullitta S, Fresegna D, De Vito F, Fantozzi R et al (2016) Siponimod (BAF312) prevents synaptic neurodegeneration in experimental multiple sclerosis. J Neuroinflammation 13(1):207
pubmed: 27566665 pmcid: 5002118 doi: 10.1186/s12974-016-0686-4
Li Z, He Y, Fan S, Sun B (2015) Clemastine rescues behavioral changes and enhances remyelination in the cuprizone mouse model of demyelination. Neurosci Bull 31(5):617–625
pubmed: 26253956 pmcid: 5563681 doi: 10.1007/s12264-015-1555-3
Vega-Riquer JM, Mendez-Victoriano G, Morales-Luckie RA, Gonzalez-Perez O (2019) Five decades of Cuprizone, an updated model to replicate demyelinating diseases. Curr Neuropharmacol 17(2):129–141
pubmed: 28714395 pmcid: 6343207 doi: 10.2174/1570159X15666170717120343
Lubetzki C, Zalc B, Williams A, Stadelmann C, Stankoff B (2020) Remyelination in multiple sclerosis: from basic science to clinical translation. Lancet Neurol 19(8):678–688
pubmed: 32702337 doi: 10.1016/S1474-4422(20)30140-X
Carrithers MD (2014) Update on Disease-modifying treatments for multiple sclerosis. Clin Ther 36(12):1938–1945
pubmed: 25218310 doi: 10.1016/j.clinthera.2014.08.006
Robertson D, Moreo N (2016) Disease-Modifying therapies in multiple sclerosis: overview and treatment considerations. Fed Pract 33(6):28–34
pubmed: 30766181 pmcid: 6366576
Mezydlo A, Treiber N, Ullrich Gavilanes EM, Eichenseer K, Ancău M, Wens A et al (2023) Remyelination by surviving oligodendrocytes is inefficient in the inflamed mammalian cortex. Neuron 111(11):1748–59e8
pubmed: 37071991 doi: 10.1016/j.neuron.2023.03.031
Miller SD, Karpus WJ Experimental autoimmune encephalomyelitis in the mouse. Curr Protoc Immunol 2007;Chap 15:Unit 15 1.
Berahovich RD, Zabel BA, Lewen S, Walters MJ, Ebsworth K, Wang Y et al (2014) Endothelial expression of CXCR7 and the regulation of systemic CXCL12 levels. Immunology 141(1):111–122
pubmed: 24116850 doi: 10.1111/imm.12176
Zohar Y, Wildbaum G, Novak R, Salzman AL, Thelen M, Alon R et al (2014) CXCL11-dependent induction of FOXP3-negative regulatory T cells suppresses autoimmune encephalomyelitis. J Clin Invest 124(5):2009–2022
pubmed: 24713654 pmcid: 4001543 doi: 10.1172/JCI71951
Meiron M, Zohar Y, Anunu R, Wildbaum G, Karin N (2008) CXCL12 (SDF-1alpha) suppresses ongoing experimental autoimmune encephalomyelitis by selecting antigen-specific regulatory T cells. J Exp Med 205(11):2643–2655
pubmed: 18852294 pmcid: 2571938 doi: 10.1084/jem.20080730
Brinkmann V, Davis MD, Heise CE, Albert R, Cottens S, Hof R et al (2002) The immune modulator FTY720 targets sphingosine 1-phosphate receptors. J Biol Chem 277(24):21453–21457
pubmed: 11967257 doi: 10.1074/jbc.C200176200
Pouzol L, Piali L, Bernard CC, Martinic MM, Steiner B, Clozel M (2019) Therapeutic potential of Ponesimod Alone and in combination with Dimethyl Fumarate in Experimental models of multiple sclerosis. Innov Clin Neurosci 16(3–4):22–30
pubmed: 31214480 pmcid: 6538399
Chun J, Giovannoni G, Hunter SF (2021) Sphingosine 1-phosphate receptor modulator therapy for multiple sclerosis: Differential downstream receptor signalling and clinical Profile effects. Drugs 81(2):207–231
pubmed: 33289881 doi: 10.1007/s40265-020-01431-8
Kappos L, Bar-Or A, Cree BAC, Fox RJ, Giovannoni G, Gold R et al (2018) Siponimod versus placebo in secondary progressive multiple sclerosis (EXPAND): a double-blind, randomised, phase 3 study. Lancet 391(10127):1263–1273
pubmed: 29576505 doi: 10.1016/S0140-6736(18)30475-6
Zirngibl M, Assinck P, Sizov A, Caprariello AV, Plemel JR (2022) Oligodendrocyte death and myelin loss in the cuprizone model: an updated overview of the intrinsic and extrinsic causes of cuprizone demyelination. Mol Neurodegener 17(1):34
pubmed: 35526004 pmcid: 9077942 doi: 10.1186/s13024-022-00538-8
Franklin RJM, Frisen J, Lyons DA (2021) Revisiting remyelination: towards a consensus on the regeneration of CNS myelin. Semin Cell Dev Biol 116:3–9
pubmed: 33082115 doi: 10.1016/j.semcdb.2020.09.009

Auteurs

Laetitia Pouzol (L)

Idorsia Pharmaceuticals Ltd, Hegenheimermattweg 91, Allschwil 4123, Basel-Landschaft, Switzerland. laetitia.pouzol@gmail.com.

Anna Sassi (A)

Idorsia Pharmaceuticals Ltd, Hegenheimermattweg 91, Allschwil 4123, Basel-Landschaft, Switzerland.

Mélanie Tunis (M)

Idorsia Pharmaceuticals Ltd, Hegenheimermattweg 91, Allschwil 4123, Basel-Landschaft, Switzerland.

Anaïs Zurbach (A)

Idorsia Pharmaceuticals Ltd, Hegenheimermattweg 91, Allschwil 4123, Basel-Landschaft, Switzerland.

Nadège Baumlin (N)

Idorsia Pharmaceuticals Ltd, Hegenheimermattweg 91, Allschwil 4123, Basel-Landschaft, Switzerland.

Carmela Gnerre (C)

Idorsia Pharmaceuticals Ltd, Hegenheimermattweg 91, Allschwil 4123, Basel-Landschaft, Switzerland.

Daniel S Strasser (DS)

Idorsia Pharmaceuticals Ltd, Hegenheimermattweg 91, Allschwil 4123, Basel-Landschaft, Switzerland.

Julia Marrie (J)

Idorsia Pharmaceuticals Ltd, Hegenheimermattweg 91, Allschwil 4123, Basel-Landschaft, Switzerland.

Enrico Vezzali (E)

Idorsia Pharmaceuticals Ltd, Hegenheimermattweg 91, Allschwil 4123, Basel-Landschaft, Switzerland.

Marianne M Martinic (MM)

Idorsia Pharmaceuticals Ltd, Hegenheimermattweg 91, Allschwil 4123, Basel-Landschaft, Switzerland.

Classifications MeSH