Multi-objective Bayesian active learning for MeV-ultrafast electron diffraction.


Journal

Nature communications
ISSN: 2041-1723
Titre abrégé: Nat Commun
Pays: England
ID NLM: 101528555

Informations de publication

Date de publication:
03 Jun 2024
Historique:
received: 06 09 2023
accepted: 16 05 2024
medline: 4 6 2024
pubmed: 4 6 2024
entrez: 3 6 2024
Statut: epublish

Résumé

Ultrafast electron diffraction using MeV energy beams(MeV-UED) has enabled unprecedented scientific opportunities in the study of ultrafast structural dynamics in a variety of gas, liquid and solid state systems. Broad scientific applications usually pose different requirements for electron probe properties. Due to the complex, nonlinear and correlated nature of accelerator systems, electron beam property optimization is a time-taking process and often relies on extensive hand-tuning by experienced human operators. Algorithm based efficient online tuning strategies are highly desired. Here, we demonstrate multi-objective Bayesian active learning for speeding up online beam tuning at the SLAC MeV-UED facility. The multi-objective Bayesian optimization algorithm was used for efficiently searching the parameter space and mapping out the Pareto Fronts which give the trade-offs between key beam properties. Such scheme enables an unprecedented overview of the global behavior of the experimental system and takes a significantly smaller number of measurements compared with traditional methods such as a grid scan. This methodology can be applied in other experimental scenarios that require simultaneously optimizing multiple objectives by explorations in high dimensional, nonlinear and correlated systems.

Identifiants

pubmed: 38830874
doi: 10.1038/s41467-024-48923-9
pii: 10.1038/s41467-024-48923-9
doi:

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Pagination

4726

Informations de copyright

© 2024. This is a U.S. Government work and not under copyright protection in the US; foreign copyright protection may apply.

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Auteurs

Fuhao Ji (F)

SLAC National Accelerator Laboratory, Menlo Park, 94025, California, USA. fuhaoji@slac.stanford.edu.

Auralee Edelen (A)

SLAC National Accelerator Laboratory, Menlo Park, 94025, California, USA.

Ryan Roussel (R)

SLAC National Accelerator Laboratory, Menlo Park, 94025, California, USA.

Xiaozhe Shen (X)

SLAC National Accelerator Laboratory, Menlo Park, 94025, California, USA.

Sara Miskovich (S)

SLAC National Accelerator Laboratory, Menlo Park, 94025, California, USA.

Stephen Weathersby (S)

SLAC National Accelerator Laboratory, Menlo Park, 94025, California, USA.

Duan Luo (D)

SLAC National Accelerator Laboratory, Menlo Park, 94025, California, USA.

Mianzhen Mo (M)

SLAC National Accelerator Laboratory, Menlo Park, 94025, California, USA.

Patrick Kramer (P)

SLAC National Accelerator Laboratory, Menlo Park, 94025, California, USA.

Christopher Mayes (C)

SLAC National Accelerator Laboratory, Menlo Park, 94025, California, USA.

Mohamed A K Othman (MAK)

SLAC National Accelerator Laboratory, Menlo Park, 94025, California, USA.

Emilio Nanni (E)

SLAC National Accelerator Laboratory, Menlo Park, 94025, California, USA.

Xijie Wang (X)

SLAC National Accelerator Laboratory, Menlo Park, 94025, California, USA.

Alexander Reid (A)

SLAC National Accelerator Laboratory, Menlo Park, 94025, California, USA.

Michael Minitti (M)

SLAC National Accelerator Laboratory, Menlo Park, 94025, California, USA.

Robert Joel England (RJ)

SLAC National Accelerator Laboratory, Menlo Park, 94025, California, USA. england@slac.stanford.edu.

Classifications MeSH