Enhancing P2/O3 Biphasic Cathode Performance for Sodium-Ion Batteries: A Metaheuristic Approach to Multi-Element Doping Design.

OP4 phase P2/O3 phase Z phase biphasic in situ X‐ray diffraction layered oxide phase transformation sodium‐ion batteries sustainable cathode

Journal

Small (Weinheim an der Bergstrasse, Germany)
ISSN: 1613-6829
Titre abrégé: Small
Pays: Germany
ID NLM: 101235338

Informations de publication

Date de publication:
11 Jun 2024
Historique:
revised: 05 05 2024
received: 01 04 2024
medline: 11 6 2024
pubmed: 11 6 2024
entrez: 11 6 2024
Statut: aheadofprint

Résumé

Sodium-ion batteries (SIBs) have emerged as a compelling alternative to lithium-ion batteries (LIBs), exhibiting comparable electrochemical performance while capitalizing on the abundant availability of sodium resources. In SIBs, P2/O3 biphasic cathodes, despite their high energy, require furthur improvements in stability to meet current energy demands. This study introduces a systematic methodology that leverages the meta-heuristically assisted NSGA-II algorithm to optimize multi-element doping in electrode materials, aiming to transcend conventional trial-and-error methods and enhance cathode capacity by the synergistic integration of P2 and O3 phases. A comprehensive phase analysis of the meta-heuristically designed cathode material Na

Identifiants

pubmed: 38860560
doi: 10.1002/smll.202402585
doi:

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Pagination

e2402585

Subventions

Organisme : National Research Foundation of Korea
Organisme : MSIT
ID : 2022M3H4A3088069
Organisme : Technology Innovation Program (Alchemist Project, Al based supercritical materials discovery)
ID : 20012196

Informations de copyright

© 2024 Wiley‐VCH GmbH.

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Auteurs

Anil K Paidi (AK)

PLS-II Beamline Department, Pohang Accelerator Laboratory, POSTECH, Pohang, 37673, Republic of Korea.

Woon Bae Park (WB)

Department of Printed Electronics Engineering, Sunchon National University, Chonnam, 57922, Republic of Korea.

Vinod K Paidi (VK)

European Synchrotron Radiation Facility, 71, Avenue des Martyrs, Grenoble, 38043, France.

Jinhyeok Lee (J)

Faculty of Nanotechnology and Advanced Materials Engineering, Sejong University, Seoul, 05006, Republic of Korea.

Kug-Seung Lee (KS)

PLS-II Beamline Department, Pohang Accelerator Laboratory, POSTECH, Pohang, 37673, Republic of Korea.

Hyungju Ahn (H)

PLS-II Beamline Department, Pohang Accelerator Laboratory, POSTECH, Pohang, 37673, Republic of Korea.

Maxim Avdeev (M)

Australian Nuclear Science and Technology Organization (ANSTO), New Illawarra Road, Lucas Heights, New South Wales, 2234, Australia.

Keun Hwa Chae (KH)

Advanced Analysis Center, Korea Institute of Science and Technology, 5 Hwarang-ro 14-gil, Seongbuk-gu, Seoul, 02792, Republic of Korea.

Myoungho Pyo (M)

Department of Printed Electronics Engineering, Sunchon National University, Chonnam, 57922, Republic of Korea.

Junxiu Wu (J)

College of Chemical and Biological Engineering, Zhejiang University, Hangzhou, Zhejiang, 310027, China.

Kee-Sun Sohn (KS)

Faculty of Nanotechnology and Advanced Materials Engineering, Sejong University, Seoul, 05006, Republic of Korea.

Docheon Ahn (D)

PLS-II Beamline Department, Pohang Accelerator Laboratory, POSTECH, Pohang, 37673, Republic of Korea.

Jun Lu (J)

College of Chemical and Biological Engineering, Zhejiang University, Hangzhou, Zhejiang, 310027, China.

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