Occurrence of a "forever chemical" in the atmosphere above pristine Amazon Forest.

Aerosol Emerging pollutants LC-MS PFAS PFOA Perfluorooctanoic acid

Journal

The Science of the total environment
ISSN: 1879-1026
Titre abrégé: Sci Total Environ
Pays: Netherlands
ID NLM: 0330500

Informations de publication

Date de publication:
10 Jun 2024
Historique:
received: 15 03 2024
revised: 16 05 2024
accepted: 09 06 2024
medline: 13 6 2024
pubmed: 13 6 2024
entrez: 12 6 2024
Statut: aheadofprint

Résumé

Per- and polyfluoroalkyl substances (PFAS), often referred to as "forever chemicals", are a class of man-made, extremely stable chemicals, which are widely used in industrial and commercial applications. Exposure to some PFAS is now known to be detrimental to human health. By virtue of PFAS long residence times, they are widely detected in the environment, including remote locations such as the Arctics, where the origin of the PFAS is poorly understood. It has been suggested that PFAS may be transported through contaminated waters, leading to accumulation in coastal areas, where they can be aerosolised via sea spray, thereby extending their geographical distribution far beyond their original source regions. The aim of this work is to investigate, for the first time, whether "forever chemicals" could be transported to areas considered to be pristine, far from coastal sites. This study was performed at the Amazonian Tall Tower Observatory (ATTO), a unique remote site situated in the middle of the Amazon rainforest, where a restricted PFAS, perfluorooctanoic acid (PFOA), was observed with concentrations reaching up to 2 pg/m

Identifiants

pubmed: 38866151
pii: S0048-9697(24)04066-X
doi: 10.1016/j.scitotenv.2024.173918
pii:
doi:

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Pagination

173918

Informations de copyright

Copyright © 2024. Published by Elsevier B.V.

Auteurs

Ivan Kourtchev (I)

Centre for Agroecology Water and Resilience (CAWR), Coventry University, Wolston Lane, Ryton on Dunsmore CV8 3LG, UK. Electronic address: ivan.kourtchev@coventry.ac.uk.

Bruna G Sebben (BG)

Environmental Engineering Department, Federal University of Parana (UFPR), Curitiba, PR, Brazil.

Sebastian Brill (S)

Multiphase Chemistry Department, Max Planck Institute for Chemistry, Mainz, Germany.

Cybelli Barbosa (C)

Multiphase Chemistry Department, Max Planck Institute for Chemistry, Mainz, Germany; Division of Plant Sciences, Institute of Biology, University of Graz, Graz, Austria.

Bettina Weber (B)

Multiphase Chemistry Department, Max Planck Institute for Chemistry, Mainz, Germany; Division of Plant Sciences, Institute of Biology, University of Graz, Graz, Austria.

Rosaria R Ferreira (RR)

Amazon Tall Tower Observatory (ATTO), National Institute of Amazonian (INPA), Brazil.

Flavio Augusto Farias D'Oliveira (FAF)

Federal Institute of Pará, Physics Department (IFPA), Belém, Pará, Brazil.

Cléo Q Dias-Junior (CQ)

Federal Institute of Pará, Physics Department (IFPA), Belém, Pará, Brazil.

Olalekan A M Popoola (OAM)

Yusuf Hamied Department of Chemistry, University of Cambridge, Cambridge CB2 1EW, UK.

Jonathan Williams (J)

Multiphase Chemistry Department, Max Planck Institute for Chemistry, Mainz, Germany.

Christopher Pöhlker (C)

Multiphase Chemistry Department, Max Planck Institute for Chemistry, Mainz, Germany.

Ricardo H M Godoi (RHM)

Environmental Engineering Department, Federal University of Parana (UFPR), Curitiba, PR, Brazil.

Classifications MeSH