Synthesis and photodynamic activity of new 5-[(E)-2-(3-alkoxy-1-phenyl-1H-pyrazol-4-yl)ethenyl]-2-phenyl-3H-indoles.

cytotoxicity indole photodynamic effect pyrazole reactive oxygen species

Journal

Archiv der Pharmazie
ISSN: 1521-4184
Titre abrégé: Arch Pharm (Weinheim)
Pays: Germany
ID NLM: 0330167

Informations de publication

Date de publication:
05 Jul 2024
Historique:
revised: 31 05 2024
received: 16 04 2024
accepted: 17 06 2024
medline: 6 7 2024
pubmed: 6 7 2024
entrez: 5 7 2024
Statut: aheadofprint

Résumé

A series of new indole-pyrazole hybrids 8a-m were synthesized through the palladium-catalyzed ligandless Heck coupling reaction from easily accessible unsubstituted, methoxy- or fluoro-substituted 4-ethenyl-1H-pyrazoles and 5-bromo-3H-indoles. These compounds exerted cytotoxicity to melanoma G361 cells when irradiated with blue light (414 nm) and no cytotoxicity in the dark at concentrations up to 10 µM, prompting us to explore their photodynamic effects. The photodynamic properties of the example compound 8d were further investigated in breast cancer MCF-7 cells. Evaluation revealed comparable anticancer activities of 8d in both breast and melanoma cancer cell lines within the submicromolar range. The treatment induced a massive generation of reactive oxygen species, leading to different types of cell death depending on the compound concentration and the irradiation intensity.

Identifiants

pubmed: 38969965
doi: 10.1002/ardp.202400282
doi:

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Pagination

e2400282

Subventions

Organisme : Research Council of Lithuania
ID : S-MIP-23-51
Organisme : The project National Institute for Cancer Research, Programme EXCELES
ID : LX22NPO5102
Organisme : Doctoral Fund of Kaunas University of Technology
ID : A-410
Organisme : Palacký University Olomouc
ID : IGA_PrF_2024_005

Informations de copyright

© 2024 The Author(s). Archiv der Pharmazie published by Wiley‐VCH GmbH on behalf of Deutsche Pharmazeutische Gesellschaft.

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Auteurs

Gabrielė Varvuolytė (G)

Department of Organic Chemistry, Kaunas University of Technology, Kaunas, Lithuania.
Institute of Synthetic Chemistry, Kaunas University of Technology, Kaunas, Lithuania.

Eva Řezníčková (E)

Department of Experimental Biology, Faculty of Science, Palacký University, Olomouc, Czech Republic.

Aurimas Bieliauskas (A)

Institute of Synthetic Chemistry, Kaunas University of Technology, Kaunas, Lithuania.

Neringa Kleizienė (N)

Institute of Synthetic Chemistry, Kaunas University of Technology, Kaunas, Lithuania.

Veronika Vojáčková (V)

Department of Experimental Biology, Faculty of Science, Palacký University, Olomouc, Czech Republic.

Alena Opichalová (A)

Department of Experimental Biology, Faculty of Science, Palacký University, Olomouc, Czech Republic.

Asta Žukauskaitė (A)

Department of Chemical Biology, Faculty of Science, Palacký University, Olomouc, Czech Republic.

Vladimír Kryštof (V)

Department of Experimental Biology, Faculty of Science, Palacký University, Olomouc, Czech Republic.
Institute of Molecular and Translational Medicine, Faculty of Medicine and Dentistry, Palacký University, Olomouc, Czech Republic.

Algirdas Šačkus (A)

Department of Organic Chemistry, Kaunas University of Technology, Kaunas, Lithuania.
Institute of Synthetic Chemistry, Kaunas University of Technology, Kaunas, Lithuania.

Classifications MeSH