Machine Learning-Enabled Tomographic Imaging of Chemical Short-Range Atomic Ordering.

artificial intelligence atomic‐scale characterization high/medium‐entropy alloys local chemical ordering tomographic imaging

Journal

Advanced materials (Deerfield Beach, Fla.)
ISSN: 1521-4095
Titre abrégé: Adv Mater
Pays: Germany
ID NLM: 9885358

Informations de publication

Date de publication:
12 Aug 2024
Historique:
revised: 24 07 2024
received: 28 05 2024
medline: 13 8 2024
pubmed: 13 8 2024
entrez: 13 8 2024
Statut: aheadofprint

Résumé

In solids, chemical short-range order (CSRO) refers to the self-organization of atoms of certain species occupying specific crystal sites. CSRO is increasingly being envisaged as a lever to tailor the mechanical and functional properties of materials. Yet quantitative relationships between properties and the morphology, number density, and atomic configurations of CSRO domains remain elusive. Herein, it is showcased how machine learning-enhanced atom probe tomography (APT) can mine the near-atomically resolved APT data and jointly exploit the technique's high elemental sensitivity to provide a 3D quantitative analysis of CSRO in a CoCrNi medium-entropy alloy. Multiple CSRO configurations are revealed, with their formation supported by state-of-the-art Monte-Carlo simulations. Quantitative analysis of these CSROs allows establishing relationships between processing parameters and physical properties. The unambiguous characterization of CSRO will help refine strategies for designing advanced materials by manipulating atomic-scale architectures.

Identifiants

pubmed: 39135414
doi: 10.1002/adma.202407564
doi:

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Pagination

e2407564

Subventions

Organisme : European Research Council
ID : ERC-SHINE(771602)
Pays : International
Organisme : Natural Science Foundation of Hunan Province
ID : 2022JJ30712
Organisme : State Key Laboratory of Powder Metallurgy, Central South University
Organisme : Deutsche Forschungsgemeinschaft
ID : SPP 2006
Organisme : Deutsche Forschungsgemeinschaft
ID : DFG 5080/3-1
Organisme : Alexander von Humboldt-Stiftung
Organisme : Next Generation TATARA Project

Informations de copyright

© 2024 The Author(s). Advanced Materials published by Wiley‐VCH GmbH.

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Auteurs

Yue Li (Y)

Max-Planck-Institut für Eisenforschung GmbH, Max-Planck-Straße 1, 40237, Düsseldorf, Germany.

Timoteo Colnaghi (T)

Max Planck Computing and Data Facility, Gießenbachstraße 2, 85748, Garching, Germany.

Yilun Gong (Y)

Max-Planck-Institut für Eisenforschung GmbH, Max-Planck-Straße 1, 40237, Düsseldorf, Germany.
Department of Materials, University of Oxford, Parks Road, Oxford, OX1 3PH, UK.

Huaide Zhang (H)

Institute of Physics (IA), RWTH Aachen University, 52056, Aachen, Germany.

Yuan Yu (Y)

Institute of Physics (IA), RWTH Aachen University, 52056, Aachen, Germany.

Ye Wei (Y)

Ecole Polytechnique Fédérale de Lausanne, School of Engineering, Rte Cantonale, Lausanne, 1015, Switzerland.

Bin Gan (B)

Suzhou Laboratory, No.388, Ruoshui Street, SIP, Jiangsu, 215123, China.

Min Song (M)

State Key Laboratory of Powder Metallurgy, Central South University, Changsha, 410083, China.

Andreas Marek (A)

Max Planck Computing and Data Facility, Gießenbachstraße 2, 85748, Garching, Germany.

Markus Rampp (M)

Max Planck Computing and Data Facility, Gießenbachstraße 2, 85748, Garching, Germany.

Siyuan Zhang (S)

Max-Planck-Institut für Eisenforschung GmbH, Max-Planck-Straße 1, 40237, Düsseldorf, Germany.

Zongrui Pei (Z)

New York University, New York, NY, 10012, USA.

Matthias Wuttig (M)

Institute of Physics (IA), RWTH Aachen University, 52056, Aachen, Germany.

Sheuly Ghosh (S)

Max-Planck-Institut für Eisenforschung GmbH, Max-Planck-Straße 1, 40237, Düsseldorf, Germany.

Fritz Körmann (F)

Max-Planck-Institut für Eisenforschung GmbH, Max-Planck-Straße 1, 40237, Düsseldorf, Germany.
Materials Informatics, BAM Federal Institute for Materials Research and Testing, Richard-Willstätter-Str. 11, 12489, Berlin, Germany.

Jörg Neugebauer (J)

Max-Planck-Institut für Eisenforschung GmbH, Max-Planck-Straße 1, 40237, Düsseldorf, Germany.

Zhangwei Wang (Z)

State Key Laboratory of Powder Metallurgy, Central South University, Changsha, 410083, China.

Baptiste Gault (B)

Max-Planck-Institut für Eisenforschung GmbH, Max-Planck-Straße 1, 40237, Düsseldorf, Germany.
Department of Materials, Imperial College, South Kensington, London, SW7 2AZ, UK.

Classifications MeSH