Robust Sequence Design Space for the Isothermal Exponential Amplification of Short Oligonucleotides.

enzymes isothermal amplification molecular evolution nucleic acids oligonucleotides

Journal

Small (Weinheim an der Bergstrasse, Germany)
ISSN: 1613-6829
Titre abrégé: Small
Pays: Germany
ID NLM: 101235338

Informations de publication

Date de publication:
24 Aug 2024
Historique:
revised: 04 08 2024
received: 27 06 2024
medline: 24 8 2024
pubmed: 24 8 2024
entrez: 24 8 2024
Statut: aheadofprint

Résumé

Advances in isothermal amplification techniques have accelerated development in biosensing applications and the design of complex molecular devices. The exponential amplification reaction technique, or EXPAR, is uniquely positioned to process molecular information from short oligonucleotide strands (≈10 nucleotides length) typically encountered in molecular computing or microRNA detection. Despite its conceptual simplicity (requiring only a template strand and two enzymes), the issue of nonspecific background amplification has hindered broader adoption. In this work, a new system configuration is established at 37 °C to achieve significantly improved performance. Critical sequence motifs responsible for the excellent signal-to-background profile are identified and generalized as a universal adapter design framework. Orthogonal template sequences generated from the framework are implemented for a triplex reaction and successfully evaluated mixtures of multiple-target inputs in a single-step, one-pot format without the need for exogenous agents.

Identifiants

pubmed: 39180448
doi: 10.1002/smll.202405250
doi:

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Pagination

e2405250

Subventions

Organisme : Singapore Ministry of Education Academic Research Fund Tier 1
ID : A-0009534-01-00
Organisme : Singapore Ministry of Education Academic Research Fund Tier 2
ID : MOE-T2EP50120-0018

Informations de copyright

© 2024 The Author(s). Small published by Wiley‐VCH GmbH.

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Auteurs

Yan Shan Ang (YS)

Department of Chemical & Biomolecular Engineering, National University of Singapore, Singapore, 117585, Singapore.

Lin-Yue Lanry Yung (LL)

Department of Chemical & Biomolecular Engineering, National University of Singapore, Singapore, 117585, Singapore.

Classifications MeSH