A cell state-specific metabolic vulnerability to GPX4-dependent ferroptosis in glioblastoma.

Astrocytic Ferroptosis Glioma Mitochondrial-metabolism Quiescent

Journal

The EMBO journal
ISSN: 1460-2075
Titre abrégé: EMBO J
Pays: England
ID NLM: 8208664

Informations de publication

Date de publication:
27 Aug 2024
Historique:
received: 23 04 2024
accepted: 01 07 2024
revised: 12 06 2024
medline: 28 8 2024
pubmed: 28 8 2024
entrez: 27 8 2024
Statut: aheadofprint

Résumé

Glioma cells hijack developmental programs to control cell state. Here, we uncover a glioma cell state-specific metabolic liability that can be therapeutically targeted. To model cell conditions at brain tumor inception, we generated genetically engineered murine gliomas, with deletion of p53 alone (p53) or with constitutively active Notch signaling (N1IC), a pathway critical in controlling astrocyte differentiation during brain development. N1IC tumors harbored quiescent astrocyte-like transformed cell populations while p53 tumors were predominantly comprised of proliferating progenitor-like cell states. Further, N1IC transformed cells exhibited increased mitochondrial lipid peroxidation, high ROS production and depletion of reduced glutathione. This altered mitochondrial phenotype rendered the astrocyte-like, quiescent populations more sensitive to pharmacologic or genetic inhibition of the lipid hydroperoxidase GPX4 and induction of ferroptosis. Treatment of patient-derived early-passage cell lines and glioma slice cultures generated from surgical samples with a GPX4 inhibitor induced selective depletion of quiescent astrocyte-like glioma cell populations with similar metabolic profiles. Collectively, these findings reveal a specific therapeutic vulnerability to ferroptosis linked to mitochondrial redox imbalance in a subpopulation of quiescent astrocyte-like glioma cells resistant to standard forms of treatment.

Identifiants

pubmed: 39192032
doi: 10.1038/s44318-024-00176-4
pii: 10.1038/s44318-024-00176-4
doi:

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Subventions

Organisme : HHS | NIH | National Institute of Neurological Disorders and Stroke (NINDS)
ID : R01NS103473
Organisme : HHS | NIH | National Institute of Neurological Disorders and Stroke (NINDS)
ID : R01NS103473
Organisme : HHS | NIH | National Institute of Neurological Disorders and Stroke (NINDS)
ID : R01NS103473
Organisme : HHS | National Institutes of Health (NIH)
ID : R35CA209896
Organisme : HHS | National Institutes of Health (NIH)
ID : R01HL112626
Organisme : HHS | NIH | National Cancer Institute (NCI)
ID : P30CA013696

Informations de copyright

© 2024. The Author(s).

Références

Aibar S, Gonzalez-Blas CB, Moerman T, Huynh-Thu VA, Imrichova H, Hulselmans G, Rambow F, Marine JC, Geurts P, Aerts J et al (2017) SCENIC: single-cell regulatory network inference and clustering. Nat Methods 14:1083–1086
pubmed: 28991892 pmcid: 5937676 doi: 10.1038/nmeth.4463
Al-Dalahmah O, Argenziano MG, Kannan A, Mahajan A, Furnari J, Paryani F, Boyett D, Save A, Humala N, Khan F et al (2023) Re-convolving the compositional landscape of primary and recurrent glioblastoma reveals prognostic and targetable tissue states. Nat Commun 14:2586
pubmed: 37142563 pmcid: 10160047 doi: 10.1038/s41467-023-38186-1
Artegiani B, Lyubimova A, Muraro M, van Es JH, van Oudenaarden A, Clevers H (2017) A single-cell RNA sequencing study reveals cellular and molecular dynamics of the hippocampal neurogenic niche. Cell Rep 21:3271–3284
pubmed: 29241552 doi: 10.1016/j.celrep.2017.11.050
Barthel FP, Johnson KC, Varn FS, Moskalik AD, Tanner G, Kocakavuk E, Anderson KJ, Abiola O, Aldape K, Alfaro KD et al (2019) Longitudinal molecular trajectories of diffuse glioma in adults. Nature 576:112–120
pubmed: 31748746 pmcid: 6897368 doi: 10.1038/s41586-019-1775-1
Benner EJ, Luciano D, Jo R, Abdi K, Paez-Gonzalez P, Sheng H, Warner DS, Liu C, Eroglu C, Kuo CT (2013) Protective astrogenesis from the SVZ niche after injury is controlled by Notch modulator Thbs4. Nature 497:369–373
pubmed: 23615612 pmcid: 3667629 doi: 10.1038/nature12069
Bonnay F, Veloso A, Steinmann V, Kocher T, Abdusselamoglu MD, Bajaj S, Rivelles E, Landskron L, Esterbauer H, Zinzen RP et al (2020) Oxidative metabolism drives immortalization of neural stem cells during tumorigenesis. Cell 182:1490–1507.e1419
pubmed: 32916131 doi: 10.1016/j.cell.2020.07.039
Buonamici S, Trimarchi T, Ruocco MG, Reavie L, Cathelin S, Mar BG, Klinakis A, Lukyanov Y, Tseng JC, Sen F et al (2009) CCR7 signalling as an essential regulator of CNS infiltration in T-cell leukaemia. Nature 459:1000–1004
pubmed: 19536265 pmcid: 3750496 doi: 10.1038/nature08020
Butler A, Hoffman P, Smibert P, Papalexi E, Satija R (2018) Integrating single-cell transcriptomic data across different conditions, technologies, and species. Nat Biotechnol 36:411–420
pubmed: 29608179 pmcid: 6700744 doi: 10.1038/nbt.4096
Chaligne R, Gaiti F, Silverbush D, Schiffman JS, Weisman HR, Kluegel L, Gritsch S, Deochand SD, Gonzalez Castro LN, Richman AR et al (2021) Epigenetic encoding, heritability and plasticity of glioma transcriptional cell states. Nat Genet 53:1469–1479
pubmed: 34594037 pmcid: 8675181 doi: 10.1038/s41588-021-00927-7
Chen J, Li Y, Yu TS, McKay RM, Burns DK, Kernie SG, Parada LF (2012) A restricted cell population propagates glioblastoma growth after chemotherapy. Nature 488:522–526
pubmed: 22854781 pmcid: 3427400 doi: 10.1038/nature11287
Chu B, Kon N, Chen D, Li T, Liu T, Jiang L, Song S, Tavana O, Gu W (2019) ALOX12 is required for p53-mediated tumour suppression through a distinct ferroptosis pathway. Nat Cell Biol 21:579–591
pubmed: 30962574 pmcid: 6624840 doi: 10.1038/s41556-019-0305-6
Couturier CP, Ayyadhury S, Le PU, Nadaf J, Monlong J, Riva G, Allache R, Baig S, Yan X, Bourgey M et al (2020) Single-cell RNA-seq reveals that glioblastoma recapitulates a normal neurodevelopmental hierarchy. Nat Commun 11:3406
pubmed: 32641768 pmcid: 7343844 doi: 10.1038/s41467-020-17186-5
Daugherty DJ, Chechneva O, Mayrhofer F, Deng W (2016) The hGFAP-driven conditional TSPO knockout is protective in a mouse model of multiple sclerosis. Sci Rep 6:22556
pubmed: 26925573 pmcid: 4772008 doi: 10.1038/srep22556
Dixon SJ, Lemberg KM, Lamprecht MR, Skouta R, Zaitsev EM, Gleason CE, Patel DN, Bauer AJ, Cantley AM, Yang WS et al (2012) Ferroptosis: an iron-dependent form of nonapoptotic cell death. Cell 149:1060–1072
pubmed: 22632970 pmcid: 3367386 doi: 10.1016/j.cell.2012.03.042
Dray N, Mancini L, Binshtok U, Cheysson F, Supatto W, Mahou P, Bedu S, Ortica S, Than-Trong E, Krecsmarik M et al (2021) Dynamic spatiotemporal coordination of neural stem cell fate decisions occurs through local feedback in the adult vertebrate brain. Cell Stem Cell 28:1457–1472.e1412
pubmed: 33823144 pmcid: 8363814 doi: 10.1016/j.stem.2021.03.014
Engler A, Rolando C, Giachino C, Saotome I, Erni A, Brien C, Zhang R, Zimber-Strobl U, Radtke F, Artavanis-Tsakonas S et al (2018) Notch2 signaling maintains NSC quiescence in the murine ventricular-subventricular zone. Cell Rep 22:992–1002
pubmed: 29386140 doi: 10.1016/j.celrep.2017.12.094
Eyler CE, Matsunaga H, Hovestadt V, Vantine SJ, van Galen P, Bernstein BE (2020) Single-cell lineage analysis reveals genetic and epigenetic interplay in glioblastoma drug resistance. Genome Biol 21:174
pubmed: 32669109 pmcid: 7364565 doi: 10.1186/s13059-020-02085-1
Fack F, Tardito S, Hochart G, Oudin A, Zheng L, Fritah S, Golebiewska A, Nazarov PV, Bernard A, Hau AC et al (2017) Altered metabolic landscape in IDH-mutant gliomas affects phospholipid, energy, and oxidative stress pathways. EMBO Mol Med 9:1681–1695
pubmed: 29054837 pmcid: 5709746 doi: 10.15252/emmm.201707729
Feng H, Schorpp K, Jin J, Yozwiak CE, Hoffstrom BG, Decker AM, Rajbhandari P, Stokes ME, Bender HG, Csuka JM et al (2020) Transferrin receptor is a specific ferroptosis marker. Cell Rep 30:3411–3423.e3417
pubmed: 32160546 pmcid: 7172030 doi: 10.1016/j.celrep.2020.02.049
Fitzner D, Bader JM, Penkert H, Bergner CG, Su M, Weil MT, Surma MA, Mann M, Klose C, Simons M (2020) Cell-type- and brain-region-resolved mouse brain lipidome. Cell Rep 32:108132
pubmed: 32937123 doi: 10.1016/j.celrep.2020.108132
Gao M, Yi J, Zhu J, Minikes AM, Monian P, Thompson CB, Jiang X (2019) Role of mitochondria in ferroptosis. Mol Cell 73:354–363.e353
pubmed: 30581146 doi: 10.1016/j.molcel.2018.10.042
Garofano L, Migliozzi S, Oh YT, D’Angelo F, Najac RD, Ko A, Frangaj B, Caruso FP, Yu K, Yuan J et al (2021) Pathway-based classification of glioblastoma uncovers a mitochondrial subtype with therapeutic vulnerabilities. Nat Cancer 2:141–156
pubmed: 33681822 pmcid: 7935068 doi: 10.1038/s43018-020-00159-4
Gatliff J, East DA, Singh A, Alvarez MS, Frison M, Matic I, Ferraina C, Sampson N, Turkheimer F, Campanella M (2017) A role for TSPO in mitochondrial Ca(2+) homeostasis and redox stress signaling. Cell Death Dis 8:e2896
pubmed: 28640253 pmcid: 5520880 doi: 10.1038/cddis.2017.186
Giachino C, Boulay JL, Ivanek R, Alvarado A, Tostado C, Lugert S, Tchorz J, Coban M, Mariani L, Bettler B et al (2015) A tumor suppressor function for notch signaling in forebrain tumor subtypes. Cancer Cell 28:730–742
pubmed: 26669487 doi: 10.1016/j.ccell.2015.10.008
Gill BJ, Pisapia DJ, Malone HR, Goldstein H, Lei L, Sonabend A, Yun J, Samanamud J, Sims JS, Banu M et al (2014) MRI-localized biopsies reveal subtype-specific differences in molecular and cellular composition at the margins of glioblastoma. Proc Natl Acad Sci USA 111:12550–12555
pubmed: 25114226 pmcid: 4151734 doi: 10.1073/pnas.1405839111
Griffiths JA, Richard AC, Bach K, Lun ATL, Marioni JC (2018) Detection and removal of barcode swapping in single-cell RNA-seq data. Nat Commun 9:2667
pubmed: 29991676 pmcid: 6039488 doi: 10.1038/s41467-018-05083-x
Gu Z, Eils R, Schlesner M (2016) Complex heatmaps reveal patterns and correlations in multidimensional genomic data. Bioinformatics 32:2847–2849
pubmed: 27207943 doi: 10.1093/bioinformatics/btw313
Hande KR (1998) Etoposide: four decades of development of a topoisomerase II inhibitor. Eur J Cancer 34:1514–1521
pubmed: 9893622 doi: 10.1016/S0959-8049(98)00228-7
Hangauer MJ, Viswanathan VS, Ryan MJ, Bole D, Eaton JK, Matov A, Galeas J, Dhruv HD, Berens ME, Schreiber SL et al (2017) Drug-tolerant persister cancer cells are vulnerable to GPX4 inhibition. Nature 551:247–250
pubmed: 29088702 pmcid: 5933935 doi: 10.1038/nature24297
Hao Y, Hao S, Andersen-Nissen E, Mauck 3rd WM, Zheng S, Butler A, Lee MJ, Wilk AJ, Darby C, Zager M et al (2021) Integrated analysis of multimodal single-cell data. Cell 184:3573–3587.e3529
pubmed: 34062119 pmcid: 8238499 doi: 10.1016/j.cell.2021.04.048
Hoang-Minh LB, Siebzehnrubl FA, Yang C, Suzuki-Hatano S, Dajac K, Loche T, Andrews N, Schmoll Massari M, Patel J, Amin K et al (2018) Infiltrative and drug-resistant slow-cycling cells support metabolic heterogeneity in glioblastoma. EMBO J 37:e98772
pubmed: 30322894 pmcid: 6276884 doi: 10.15252/embj.201798772
Ingold I, Berndt C, Schmitt S, Doll S, Poschmann G, Buday K, Roveri A, Peng X, Porto Freitas F, Seibt T et al (2018) Selenium utilization by GPX4 is required to prevent hydroperoxide-induced ferroptosis. Cell 172:409–422.e421
pubmed: 29290465 doi: 10.1016/j.cell.2017.11.048
Jiang L, Kon N, Li T, Wang SJ, Su T, Hibshoosh H, Baer R, Gu W (2015) Ferroptosis as a p53-mediated activity during tumour suppression. Nature 520:57–62
pubmed: 25799988 pmcid: 4455927 doi: 10.1038/nature14344
Jiang X, Stockwell BR, Conrad M (2021) Ferroptosis: mechanisms, biology and role in disease. Nat Rev Mol Cell Biol 22:266–282
pubmed: 33495651 pmcid: 8142022 doi: 10.1038/s41580-020-00324-8
Johnson KC, Anderson KJ, Courtois ET, Gujar AD, Barthel FP, Varn FS, Luo D, Seignon M, Yi E, Kim H et al (2021) Single-cell multimodal glioma analyses identify epigenetic regulators of cellular plasticity and environmental stress response. Nat Genet 53:1456–1468
pubmed: 34594038 pmcid: 8570135 doi: 10.1038/s41588-021-00926-8
Jung E, Osswald M, Ratliff M, Dogan H, Xie R, Weil S, Hoffmann DC, Kurz FT, Kessler T, Heiland S et al (2021) Tumor cell plasticity, heterogeneity, and resistance in crucial microenvironmental niches in glioma. Nat Commun 12:1014
pubmed: 33579922 pmcid: 7881116 doi: 10.1038/s41467-021-21117-3
Kardash E, Bandemer J, Raz E (2011) Imaging protein activity in live embryos using fluorescence resonance energy transfer biosensors. Nat Protoc 6:1835–1846
Karpel-Massler G, Ishida CT, Bianchetti E, Zhang Y, Shu C, Tsujiuchi T, Banu MA, Garcia F, Roth KA, Bruce JN et al (2017) Induction of synthetic lethality in IDH1-mutated gliomas through inhibition of Bcl-xL. Nat Commun 8:1067
pubmed: 29057925 pmcid: 5651864 doi: 10.1038/s41467-017-00984-9
Killoy KM, Harlan BA, Pehar M, Vargas MR (2020) FABP7 upregulation induces a neurotoxic phenotype in astrocytes. Glia 68:2693–2704
pubmed: 32619303 pmcid: 7573932 doi: 10.1002/glia.23879
LeBlanc VG, Trinh DL, Aslanpour S, Hughes M, Livingstone D, Jin D, Ahn BY, Blough MD, Cairncross JG, Chan JA et al (2022) Single-cell landscapes of primary glioblastomas and matched explants and cell lines show variable retention of inter- and intratumor heterogeneity. Cancer Cell 40:379–392.e379
pubmed: 35303420 doi: 10.1016/j.ccell.2022.02.016
Lei L, Sonabend AM, Guarnieri P, Soderquist C, Ludwig T, Rosenfeld S, Bruce JN, Canoll P (2011) Glioblastoma models reveal the connection between adult glial progenitors and the proneural phenotype. PLoS ONE 6:e20041
pubmed: 21625383 pmcid: 3100315 doi: 10.1371/journal.pone.0020041
Levine JH, Simonds EF, Bendall SC, Davis KL, Amir EAD, Tadmor MD, Litvin O, Fienberg HG, Jager A, Zunder ER et al (2015) Data-driven phenotypic dissection of AML reveals progenitor-like cells that correlate with prognosis. Cell 162:184–197
pubmed: 26095251 pmcid: 4508757 doi: 10.1016/j.cell.2015.05.047
Levitin HM, Yuan J, Cheng YL, Ruiz FJ, Bush EC, Bruce JN, Canoll P, Iavarone A, Lasorella A, Blei DM et al (2019) De novo gene signature identification from single-cell RNA-seq with hierarchical Poisson factorization. Mol Syst Biol 15:e8557
pubmed: 30796088 pmcid: 6386217 doi: 10.15252/msb.20188557
Liau BB, Sievers C, Donohue LK, Gillespie SM, Flavahan WA, Miller TE, Venteicher AS, Hebert CH, Carey CD, Rodig SJ et al (2017) Adaptive chromatin remodeling drives glioblastoma stem cell plasticity and drug tolerance. Cell Stem Cell 20:233–246.e237
pubmed: 27989769 doi: 10.1016/j.stem.2016.11.003
Liberzon A, Subramanian A, Pinchback R, Thorvaldsdottir H, Tamayo P, Mesirov JP (2011) Molecular signatures database (MSigDB) 3.0. Bioinformatics 27:1739–1740
pubmed: 21546393 pmcid: 3106198 doi: 10.1093/bioinformatics/btr260
Liu I, Jiang L, Samuelsson ER, Marco Salas S, Beck A, Hack OA, Jeong D, Shaw ML, Englinger B, LaBelle J et al (2022) The landscape of tumor cell states and spatial organization in H3-K27M mutant diffuse midline glioma across age and location. Nat Genet 54:1881–1894
pubmed: 36471067 pmcid: 9729116 doi: 10.1038/s41588-022-01236-3
Llorens-Bobadilla E, Zhao S, Baser A, Saiz-Castro G, Zwadlo K, Martin-Villalba A (2015) Single-cell transcriptomics reveals a population of dormant neural stem cells that become activated upon brain injury. Cell Stem Cell 17:329–340
pubmed: 26235341 doi: 10.1016/j.stem.2015.07.002
Lun AT, Bach K, Marioni JC (2016) Pooling across cells to normalize single-cell RNA sequencing data with many zero counts. Genome Biol 17:75
pubmed: 27122128 doi: 10.1186/s13059-016-0947-7
Lun ATL, Riesenfeld S, Andrews T, Dao TP, Gomes T, participants in the 1st Human Cell Atlas J, Marioni JC (2019) EmptyDrops: distinguishing cells from empty droplets in droplet-based single-cell RNA sequencing data. Genome Biol 20:63
pubmed: 30902100 pmcid: 6431044 doi: 10.1186/s13059-019-1662-y
Lyamzaev KG, Panteleeva AA, Simonyan RA, Avetisyan AV, Chernyak BV (2023) Mitochondrial lipid peroxidation is responsible for ferroptosis. Cells 12:611
pubmed: 36831278 pmcid: 9954536 doi: 10.3390/cells12040611
Mbah NE, Myers AL, Chung C, Thompson JK, Hong HS, Sajjakulnukit P, Nwosu ZC, Shan M, Sweha SR, Maydan DD et al (2022) Therapeutic targeting of differentiation state-dependent metabolic vulnerabilities in DIPG. Preprint at https://doi.org/10.1101/2022.03.01.482555
Milenkovic VM, Slim D, Bader S, Koch V, Heinl ES, Alvarez-Carbonell D, Nothdurfter C, Rupprecht R, Wetzel CH (2019) CRISPR-Cas9 mediated TSPO gene knockout alters respiration and cellular metabolism in human primary microglia cells. Int J Mol Sci 20:3359
pubmed: 31323920 pmcid: 6651328 doi: 10.3390/ijms20133359
Mizrak D, Bayin NS, Yuan J, Liu Z, Suciu RM, Niphakis MJ, Ngo N, Lum KM, Cravatt BF, Joyner AL et al (2020) Single-cell profiling and SCOPE-seq reveal lineage dynamics of adult ventricular-subventricular zone neurogenesis and NOTUM as a key regulator. Cell Rep 31:107805
pubmed: 32579931 pmcid: 7396151 doi: 10.1016/j.celrep.2020.107805
Mizrak D, Levitin HM, Delgado AC, Crotet V, Yuan J, Chaker Z, Silva-Vargas V, Sims PA, Doetsch F (2019) Single-cell analysis of regional differences in adult V-SVZ neural stem cell lineages. Cell Rep 26:394–406.e395
pubmed: 30625322 pmcid: 6368857 doi: 10.1016/j.celrep.2018.12.044
Molenaar MR, Jeucken A, Wassenaar TA, van de Lest CHA, Brouwers JF, Helms JB (2019) LION/web: a web-based ontology enrichment tool for lipidomic data analysis. Gigascience 8:giz061
pubmed: 31141612 pmcid: 6541037 doi: 10.1093/gigascience/giz061
Montgomery MK, Kim SH, Dovas A, Zhao HT, Goldberg AR, Xu W, Yagielski AJ, Cambareri MK, Patel KB, Mela A et al (2020) Glioma-induced alterations in neuronal activity and neurovascular coupling during disease progression. Cell Rep 31:107500
pubmed: 32294436 pmcid: 7443283 doi: 10.1016/j.celrep.2020.03.064
Neftel C, Laffy J, Filbin MG, Hara T, Shore ME, Rahme GJ, Richman AR, Silverbush D, Shaw ML, Hebert CM et al (2019) An integrative model of cellular states, plasticity, and genetics for glioblastoma. Cell 178:835–849.e821
pubmed: 31327527 pmcid: 6703186 doi: 10.1016/j.cell.2019.06.024
Nguyen TTT, Shang E, Shu C, Kim S, Mela A, Humala N, Mahajan A, Yang HW, Akman HO, Quinzii CM et al (2021) Aurora kinase A inhibition reverses the Warburg effect and elicits unique metabolic vulnerabilities in glioblastoma. Nat Commun 12:5203
pubmed: 34471141 pmcid: 8410792 doi: 10.1038/s41467-021-25501-x
Noch EK, Palma L, Yim I, Bullen N, Barnett D, Walsh A, Bhinder B, Benedetti E, Krumsiek J, Gurvitch J et al (2024) Cysteine induces mitochondrial reductive stress in glioblastoma through hydrogen peroxide production. Proc Natl Acad Sci USA 121:e2317343121
pubmed: 38359293 pmcid: 10895255 doi: 10.1073/pnas.2317343121
Ojha R, Tantray I, Rimal S, Mitra S, Cheshier S, Lu B (2022) Regulation of reverse electron transfer at mitochondrial complex I by unconventional Notch action in cancer stem cells. Dev Cell 57:260–276.e269
pubmed: 35077680 pmcid: 8852348 doi: 10.1016/j.devcel.2021.12.020
Oren Y, Tsabar M, Cuoco MS, Amir-Zilberstein L, Cabanos HF, Hutter JC, Hu B, Thakore PI, Tabaka M, Fulco CP et al (2021) Cycling cancer persister cells arise from lineages with distinct programs. Nature 596:576–582
pubmed: 34381210 pmcid: 9209846 doi: 10.1038/s41586-021-03796-6
Pine AR, Cirigliano SM, Nicholson JG, Hu Y, Linkous A, Miyaguchi K, Edwards L, Singhania R, Schwartz TH, Ramakrishna R et al (2020) Tumor microenvironment is critical for the maintenance of cellular states found in primary glioblastomas. Cancer Discov 10:964–979
pubmed: 32253265 pmcid: 10256258 doi: 10.1158/2159-8290.CD-20-0057
Puca F, Yu F, Bartolacci C, Pettazzoni P, Carugo A, Huang-Hobbs E, Liu J, Zanca C, Carbone F, Del Poggetto E et al (2021) Medium-chain acyl-coa dehydrogenase protects mitochondria from lipid peroxidation in glioblastoma. Cancer Discov 11:2904–2923
pubmed: 34039636 pmcid: 8711129 doi: 10.1158/2159-8290.CD-20-1437
Qiu B, Zandkarimi F, Bezjian CT, Reznik E, Soni RK, Gu W, Jiang X, Stockwell BR (2024) Phospholipids with two polyunsaturated fatty acyl tails promote ferroptosis. Cell 187:1177–1190.e1118
pubmed: 38366593 doi: 10.1016/j.cell.2024.01.030
Rabe M, Dumont S, Alvarez-Arenas A, Janati H, Belmonte-Beitia J, Calvo GF, Thibault-Carpentier C, Sery Q, Chauvin C, Joalland N et al (2020) Identification of a transient state during the acquisition of temozolomide resistance in glioblastoma. Cell Death Dis 11:19
pubmed: 31907355 pmcid: 6944699 doi: 10.1038/s41419-019-2200-2
Radu AG, Torch S, Fauvelle F, Pernet-Gallay K, Lucas A, Blervaque R, Delmas V, Schlattner U, Lafanechere L, Hainaut P et al (2019) LKB1 specifies neural crest cell fates through pyruvate-alanine cycling. Sci Adv 5:eaau5106
pubmed: 31328154 pmcid: 6636984 doi: 10.1126/sciadv.aau5106
Rupprecht R, Papadopoulos V, Rammes G, Baghai TC, Fan J, Akula N, Groyer G, Adams D, Schumacher M (2010) Translocator protein (18 kDa) (TSPO) as a therapeutic target for neurological and psychiatric disorders. Nat Rev Drug Discov 9:971–988
pubmed: 21119734 doi: 10.1038/nrd3295
Rusu P, Shao C, Neuerburg A, Acikgoz AA, Wu Y, Zou P, Phapale P, Shankar TS, Doring K, Dettling S et al (2019) GPD1 specifically marks dormant glioma stem cells with a distinct metabolic profile. Cell Stem Cell 25:241–257.e248
pubmed: 31303549 doi: 10.1016/j.stem.2019.06.004
Schiffman JS, D’Avino AR, Prieto T, Pang Y, Fan Y, Rajagopalan S, Potenski C, Hara T, Suvà ML, Gawad C et al (2023) Defining ancestry, heritability and plasticity of cellular phenotypes in somatic evolution. Preprint https://doi.org/10.1101/2022.12.28.522128
Shekhar K, Lapan SW, Whitney IE, Tran NM, Macosko EZ, Kowalczyk M, Adiconis X, Levin JZ, Nemesh J, Goldman M et al (2016) Comprehensive classification of retinal bipolar neurons by single-cell transcriptomics. Cell 166:1308–1323.e1330
pubmed: 27565351 pmcid: 5003425 doi: 10.1016/j.cell.2016.07.054
Shin J, Berg DA, Zhu Y, Shin JY, Song J, Bonaguidi MA, Enikolopov G, Nauen DW, Christian KM, Ming GL et al (2015) Single-cell RNA-Seq with waterfall reveals molecular cascades underlying adult neurogenesis. Cell Stem Cell 17:360–372
pubmed: 26299571 pmcid: 8638014 doi: 10.1016/j.stem.2015.07.013
Spinazzi EF, Argenziano MG, Upadhyayula PS, Banu MA, Neira JA, Higgins DMO, Wu PB, Pereira B, Mahajan A, Humala N et al (2022) Chronic convection-enhanced delivery of topotecan for patients with recurrent glioblastoma: a first-in-patient, single-centre, single-arm, phase 1b trial. Lancet Oncol 23:1409–1418
pubmed: 36243020 pmcid: 9641975 doi: 10.1016/S1470-2045(22)00599-X
Stoeckius M, Zheng S, Houck-Loomis B, Hao S, Yeung BZ, Mauck 3rd WM, Smibert P, Satija R (2018) Cell Hashing with barcoded antibodies enables multiplexing and doublet detection for single cell genomics. Genome Biol 19:224
pubmed: 30567574 pmcid: 6300015 doi: 10.1186/s13059-018-1603-1
Subramanian A, Tamayo P, Mootha VK, Mukherjee S, Ebert BL, Gillette MA, Paulovich A, Pomeroy SL, Golub TR, Lander ES et al (2005) Gene set enrichment analysis: a knowledge-based approach for interpreting genome-wide expression profiles. Proc Natl Acad Sci USA 102:15545–15550
pubmed: 16199517 pmcid: 1239896 doi: 10.1073/pnas.0506580102
Suva ML, Tirosh I (2020) The glioma stem cell model in the era of single-cell genomics. Cancer Cell 37:630–636
pubmed: 32396858 doi: 10.1016/j.ccell.2020.04.001
Torrini C, Nguyen TTT, Shu C, Mela A, Humala N, Mahajan A, Seeley EH, Zhang G, Westhoff MA, Karpel-Massler G et al (2022) Lactate is an epigenetic metabolite that drives survival in model systems of glioblastoma. Mol Cell 82:3061–3076.e3066
pubmed: 35948010 pmcid: 9391294 doi: 10.1016/j.molcel.2022.06.030
Upadhyayula PS, Higgins DM, Mela A, Banu M, Dovas A, Zandkarimi F, Patel P, Mahajan A, Humala N, Nguyen TTT et al (2023) Dietary restriction of cysteine and methionine sensitizes gliomas to ferroptosis and induces alterations in energetic metabolism. Nat Commun 14:1187
pubmed: 36864031 pmcid: 9981683 doi: 10.1038/s41467-023-36630-w
Vicente-Gutierrez C, Bonora N, Bobo-Jimenez V, Jimenez-Blasco D, Lopez-Fabuel I, Fernandez E, Josephine C, Bonvento G, Enriquez JA, Almeida A et al (2019) Astrocytic mitochondrial ROS modulate brain metabolism and mouse behaviour. Nat Metab 1:201–211
pubmed: 32694785 doi: 10.1038/s42255-018-0031-6
Viswanathan VS, Ryan MJ, Dhruv HD, Gill S, Eichhoff OM, Seashore-Ludlow B, Kaffenberger SD, Eaton JK, Shimada K, Aguirre AJ et al (2017) Dependency of a therapy-resistant state of cancer cells on a lipid peroxidase pathway. Nature 547:453–457
pubmed: 28678785 pmcid: 5667900 doi: 10.1038/nature23007
Wang L, Babikir H, Muller S, Yagnik G, Shamardani K, Catalan F, Kohanbash G, Alvarado B, Di Lullo E, Kriegstein A et al (2019) The phenotypes of proliferating glioblastoma cells reside on a single axis of variation. Cancer Discov 9:1708–1719
pubmed: 31554641 pmcid: 7161589 doi: 10.1158/2159-8290.CD-19-0329
Wang L, Jung J, Babikir H, Shamardani K, Jain S, Feng X, Gupta N, Rosi S, Chang S, Raleigh D et al (2022) A single-cell atlas of glioblastoma evolution under therapy reveals cell-intrinsic and cell-extrinsic therapeutic targets. Nat Cancer 3:1534–1552
pubmed: 36539501 pmcid: 9767870 doi: 10.1038/s43018-022-00475-x
Wang W, Cho H, Kim D, Park Y, Moon JH, Lim SJ, Yoon SM, McCane M, Aicher SA, Kim S et al (2020) PRC2 acts as a critical timer that drives oligodendrocyte fate over astrocyte identity by repressing the notch pathway. Cell Rep 32:108147
pubmed: 32937136 pmcid: 8070886 doi: 10.1016/j.celrep.2020.108147
Watson DC, Bayik D, Storevik S, Moreino SS, Sprowls SA, Han J, Augustsson MT, Lauko A, Sravya P, Rosland GV et al (2023) GAP43-dependent mitochondria transfer from astrocytes enhances glioblastoma tumorigenicity. Nat Cancer 4:648–664
pubmed: 37169842 pmcid: 10212766 doi: 10.1038/s43018-023-00556-5
Weiss-Sadan T, Ge M, Hayashi M, Gohar M, Yao CH, de Groot A, Harry S, Carlin A, Fischer H, Shi L et al (2023) NRF2 activation induces NADH-reductive stress, providing a metabolic vulnerability in lung cancer. Cell Metab 35:722
pubmed: 37019082 pmcid: 10103906 doi: 10.1016/j.cmet.2023.03.011
Weng Q, Wang J, Wang J, He D, Cheng Z, Zhang F, Verma R, Xu L, Dong X, Liao Y et al (2019) Single-cell transcriptomics uncovers glial progenitor diversity and cell fate determinants during development and gliomagenesis. Cell Stem Cell 24:707–723.e708
pubmed: 30982771 pmcid: 6669001 doi: 10.1016/j.stem.2019.03.006
Wu J, Minikes AM, Gao M, Bian H, Li Y, Stockwell BR, Chen ZN, Jiang X (2019) Intercellular interaction dictates cancer cell ferroptosis via NF2-YAP signalling. Nature 572:402–406
pubmed: 31341276 pmcid: 6697195 doi: 10.1038/s41586-019-1426-6
Xie XP, Laks DR, Sun D, Ganbold M, Wang Z, Pedraza AM, Bale T, Tabar V, Brennan C, Zhou X et al (2022) Quiescent human glioblastoma cancer stem cells drive tumor initiation, expansion, and recurrence following chemotherapy. Dev Cell 57:32–46.e38
pubmed: 35016005 pmcid: 8820651 doi: 10.1016/j.devcel.2021.12.007
Yang WS, SriRamaratnam R, Welsch ME, Shimada K, Skouta R, Viswanathan VS, Cheah JH, Clemons PA, Shamji AF, Clish CB et al (2014) Regulation of ferroptotic cancer cell death by GPX4. Cell 156:317–331
pubmed: 24439385 pmcid: 4076414 doi: 10.1016/j.cell.2013.12.010
Ye LF, Chaudhary KR, Zandkarimi F, Harken AD, Kinslow CJ, Upadhyayula PS, Dovas A, Higgins DM, Tan H, Zhang Y et al (2020) Radiation-induced lipid peroxidation triggers ferroptosis and synergizes with ferroptosis inducers. ACS Chem Biol 15:469–484
pubmed: 31899616 pmcid: 7180072 doi: 10.1021/acschembio.9b00939
Yuan J, Levitin HM, Frattini V, Bush EC, Boyett DM, Samanamud J, Ceccarelli M, Dovas A, Zanazzi G, Canoll P et al (2018) Single-cell transcriptome analysis of lineage diversity in high-grade glioma. Genome Med 10:57
pubmed: 30041684 pmcid: 6058390 doi: 10.1186/s13073-018-0567-9
Yuan J, Sims PA (2016) An automated microwell platform for large-scale single cell RNA-Seq. Sci Rep 6:33883
pubmed: 27670648 pmcid: 5037380 doi: 10.1038/srep33883
Zamboni M, Llorens-Bobadilla E, Magnusson JP, Frisen J (2020) A widespread neurogenic potential of neocortical astrocytes is induced by injury. Cell Stem Cell 27:605–617.e605
pubmed: 32758425 pmcid: 7534841 doi: 10.1016/j.stem.2020.07.006
Zhao W, Dovas A, Spinazzi EF, Levitin HM, Banu MA, Upadhyayula P, Sudhakar T, Marie T, Otten ML, Sisti MB et al (2021) Deconvolution of cell type-specific drug responses in human tumor tissue with single-cell RNA-seq. Genome Med 13:82
pubmed: 33975634 pmcid: 8114529 doi: 10.1186/s13073-021-00894-y
Zhao X, Arca DD, Lim WK, Brahmachary M, Carro MS, Ludwig T, Cardo CC, Guillemot F, Aldape K, Califano A et al (2009) The N-Myc-DLL3 cascade is suppressed by the ubiquitin ligase Huwe1 to inhibit proliferation and promote neurogenesis in the developing brain. Dev Cell 17:210–221
pubmed: 19686682 pmcid: 2769073 doi: 10.1016/j.devcel.2009.07.009

Auteurs

Matei A Banu (MA)

Department of Neurological Surgery, Columbia University Irving Medical Center, New York, NY, USA.

Athanassios Dovas (A)

Department of Pathology and Cell Biology, Columbia University Irving Medical Center, New York, NY, USA.

Michael G Argenziano (MG)

Department of Neurological Surgery, Columbia University Irving Medical Center, New York, NY, USA.

Wenting Zhao (W)

Department of System Biology, Columbia University Irving Medical Center, New York, NY, USA.

Colin P Sperring (CP)

Department of Neurological Surgery, Columbia University Irving Medical Center, New York, NY, USA.

Henar Cuervo Grajal (H)

Spanish National Center for Cardiovascular Research, Madrid, Spain.

Zhouzerui Liu (Z)

Department of System Biology, Columbia University Irving Medical Center, New York, NY, USA.

Dominique Mo Higgins (DM)

Department of Neurological Surgery, University of North Carolina School of Medicine, Chapel Hill, NC, USA.

Misha Amini (M)

Department of Neurological Surgery, Columbia University Irving Medical Center, New York, NY, USA.

Brianna Pereira (B)

Department of Pathology and Cell Biology, Columbia University Irving Medical Center, New York, NY, USA.

Ling F Ye (LF)

Department of Medicine, Columbia University Irving Medical Center, New York, NY, USA.

Aayushi Mahajan (A)

Department of Neurological Surgery, Columbia University Irving Medical Center, New York, NY, USA.
Department of Pathology and Cell Biology, Columbia University Irving Medical Center, New York, NY, USA.

Nelson Humala (N)

Department of Neurological Surgery, Columbia University Irving Medical Center, New York, NY, USA.
Department of Pathology and Cell Biology, Columbia University Irving Medical Center, New York, NY, USA.

Julia L Furnari (JL)

Department of Neurological Surgery, Columbia University Irving Medical Center, New York, NY, USA.
Department of Pathology and Cell Biology, Columbia University Irving Medical Center, New York, NY, USA.

Pavan S Upadhyayula (PS)

Department of Neurological Surgery, Columbia University Irving Medical Center, New York, NY, USA.

Fereshteh Zandkarimi (F)

Department of Biological Sciences, Department of Chemistry and Herbert Irving Comprehensive Cancer Center, Columbia University, New York, NY, USA.

Trang Tt Nguyen (TT)

Department of Pathology and Cell Biology, Columbia University Irving Medical Center, New York, NY, USA.

Damian Teasley (D)

Department of Neurological Surgery, Columbia University Irving Medical Center, New York, NY, USA.

Peter B Wu (PB)

Department of Neurological Surgery, UCLA Geffen School of Medicine, Los Angeles, CA, USA.

Li Hai (L)

Sulzberger Columbia Genome Center, Columbia University, New York, NY, USA.

Charles Karan (C)

Sulzberger Columbia Genome Center, Columbia University, New York, NY, USA.

Tyrone Dowdy (T)

NCI Neuro-oncology Branch, Bethesda, MD, USA.

Aida Razavilar (A)

Department of Pathology and Cell Biology, Columbia University Irving Medical Center, New York, NY, USA.

Markus D Siegelin (MD)

Department of Pathology and Cell Biology, Columbia University Irving Medical Center, New York, NY, USA.

Jan Kitajewski (J)

University of Illinois Cancer Center, Department of Physiology and Biophysics, University of Illinois Chicago, Chicago, IL, USA.

Mioara Larion (M)

NCI Neuro-oncology Branch, Bethesda, MD, USA.

Jeffrey N Bruce (JN)

Department of Neurological Surgery, Columbia University Irving Medical Center, New York, NY, USA.

Brent R Stockwell (BR)

Department of Biological Sciences, Department of Chemistry and Herbert Irving Comprehensive Cancer Center, Columbia University, New York, NY, USA.

Peter A Sims (PA)

Department of System Biology, Columbia University Irving Medical Center, New York, NY, USA. pas2182@cumc.columbia.edu.

Peter Canoll (P)

Department of Neurological Surgery, Columbia University Irving Medical Center, New York, NY, USA. pc561@cumc.columbia.edu.
Department of Pathology and Cell Biology, Columbia University Irving Medical Center, New York, NY, USA. pc561@cumc.columbia.edu.

Classifications MeSH