Achieving metal-like catalysis from semiconductor for on-surface synthesis.

catalysis graphene nanoribbons metal oxide on-surface synthesis semiconductor

Journal

Proceedings of the National Academy of Sciences of the United States of America
ISSN: 1091-6490
Titre abrégé: Proc Natl Acad Sci U S A
Pays: United States
ID NLM: 7505876

Informations de publication

Date de publication:
10 Sep 2024
Historique:
medline: 6 9 2024
pubmed: 6 9 2024
entrez: 6 9 2024
Statut: ppublish

Résumé

Free of posttransfer, on-surface synthesis (OSS) of single-atomic-layer nanostructures directly on semiconductors holds considerable potential for next-generation devices. However, due to the high diffusion barrier and abundant defects on semiconductor surfaces, extended and well-defined OSS on semiconductors has major difficulty. Furthermore, given semiconductors' limited thermal catalytic activity, initiating high-barrier reactions remains a significant challenge. Herein, using TiO

Identifiants

DOI: 10.1073/pnas.2408919121 PMID: 39240967
pubmed: 39240967
doi: 10.1073/pnas.2408919121
doi:

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Pagination

e2408919121

Subventions

Organisme : MOST | National Natural Science Foundation of China (NSFC)
ID : 22272041

Déclaration de conflit d'intérêts

Competing interests statement:The authors declare no competing interest.

Auteurs

Wenlong E (W)

State Key Laboratory of Molecular Reaction Dynamics, Dalian Institute of Chemical Physics, Chinese Academy of Sciences, Dalian 116023, China.
University of Chinese Academy of Sciences, Beijing 100049, China.
ORCID: 0009-0001-1836-8538

Wei Yi (W)

State Key Laboratory of Molecular Reaction Dynamics, Dalian Institute of Chemical Physics, Chinese Academy of Sciences, Dalian 116023, China.
State Key Laboratory of Urban Water Resource and Environment, School of Chemistry and Chemical Engineering, Harbin Institute of Technology, Harbin 150001, China.

Honghe Ding (H)

National Synchrotron Radiation Laboratory and Department of Chemical Physics, University of Science and Technology of China, Hefei 230029, China.
ORCID: 0009-0003-9405-0761

Junfa Zhu (J)

National Synchrotron Radiation Laboratory and Department of Chemical Physics, University of Science and Technology of China, Hefei 230029, China.

Federico Rosei (F)

Department of Chemical and Pharmaceutical Sciences, University of Trieste, Trieste 34127, Italy.

Xueming Yang (X)

State Key Laboratory of Molecular Reaction Dynamics, Dalian Institute of Chemical Physics, Chinese Academy of Sciences, Dalian 116023, China.
Department of Chemistry and Guangdong Provincial Key Laboratory of Catalytic Chemistry, Southern University of Science and Technology, Shenzhen 518055, China.
ORCID: 0000-0001-6684-9187

Miao Yu (M)

State Key Laboratory of Molecular Reaction Dynamics, Dalian Institute of Chemical Physics, Chinese Academy of Sciences, Dalian 116023, China.
State Key Laboratory of Urban Water Resource and Environment, School of Chemistry and Chemical Engineering, Harbin Institute of Technology, Harbin 150001, China.
School of Materials and Energy, University of Electronic Science and Technology, Chengdu 610000, China.
ORCID: 0000-0001-8820-9594

Classifications MeSH