Revealing the Impact of Aging on Perovskite Solar Cells Employing Nickel Phthalocyanine-Based Hole Transporting Material.
aging stability
efficiency
hole transporting material
metal phthalocyanine
perovskite solar cells
Journal
Advanced science (Weinheim, Baden-Wurttemberg, Germany)
ISSN: 2198-3844
Titre abrégé: Adv Sci (Weinh)
Pays: Germany
ID NLM: 101664569
Informations de publication
Date de publication:
16 Sep 2024
16 Sep 2024
Historique:
revised:
24
07
2024
received:
14
05
2024
medline:
17
9
2024
pubmed:
17
9
2024
entrez:
17
9
2024
Statut:
aheadofprint
Résumé
The enhancement of the photovoltaic performance upon the aging process at particular environment is often observed in perovskite solar cells (PSCs), particularly for the devices with 2,2',7,7'-tetrakis(N,N-di(4-methoxyphenyl)amino)-9,9'-spirobifluorene (spiro-OMeTAD) as hole transporting material (HTM). In this work, for the first time the effect of aging the typical n-i-p PSCs employing nickel phthalocyanine (coded as Bis-PF-Ni) solely as dopant-free HTM is investigated and as an additive in spiro-OMeTAD solution. This study reveals that the prolong aging of these devices at dry air condition (RH = 2%, 25 °C) is beneficial for the improvement of their performances. Various bulk and surface characterization techniques are utilized to understand the factors behind the spontaneous efficiency enhancement of the devices after storage. As a result, the changes in properties of the Bis-PF-Ni layer are observed and at perovskite/Bis-PF-Ni interface, which ultimately improves the charge transport and reduces non-radiative recombination. In addition, the devices with Bis-PF-Ni HTM reveal enhanced long-term ambient and thermal stability compared to the PSCs based on doped spiro-OMeTAD.
Identifiants
pubmed: 39285650
doi: 10.1002/advs.202405284
doi:
Types de publication
Journal Article
Langues
eng
Sous-ensembles de citation
IM
Pagination
e2405284Subventions
Organisme : Scientific Research Projects Coordination Unit of Sakarya University of Applied Sciences
ID : 212-2024
Organisme : Interdisciplinary Centre for Mathematical and Computational Modelling at the University of Warsaw
Organisme : Narodowe Centrum Nauki
ID : 2020/38/E/ST5/00267
Informations de copyright
© 2024 The Author(s). Advanced Science published by Wiley‐VCH GmbH.
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