RADD: A real-time FRET-based biochemical assay for DNA deaminase studies.


Journal

Methods in enzymology
ISSN: 1557-7988
Titre abrégé: Methods Enzymol
Pays: United States
ID NLM: 0212271

Informations de publication

Date de publication:
2024
Historique:
medline: 11 10 2024
pubmed: 11 10 2024
entrez: 10 10 2024
Statut: ppublish

Résumé

In recent years, the connection between APOBEC3 cytosine deaminases and cancer mutagenesis has become ever more apparent. This growing awareness and lack of inhibitory drugs has created a distinct need for biochemical tools that can be used to identify and characterize potential inhibitors of this family of enzymes. In response to this challenge, we have developed a Real-time APOBEC3-mediated DNA Deamination (RADD) assay. The RADD assay provides a rapid, real-time fluorescence readout of APOBEC3 DNA deamination and serves as a crucial addition to the existing APOBEC3 biochemical and cellular toolkit. This method improves upon contemporary DNA deamination assays by offering a more rapid and quantifiable readout as well as providing a platform that is readily adaptable to a high-throughput format for inhibitor discovery. In this chapter we provide a detailed guide for the usage of the RADD assay for the characterization of APOBEC3 enzymes and potential inhibitors.

Identifiants

pubmed: 39389668
pii: S0076-6879(24)00409-9
doi: 10.1016/bs.mie.2024.08.001
pii:
doi:

Substances chimiques

DNA 9007-49-2
Cytidine Deaminase EC 3.5.4.5
Enzyme Inhibitors 0
APOBEC Deaminases EC 3.5.4.5

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Pagination

311-345

Informations de copyright

Copyright © 2024. Published by Elsevier Inc.

Auteurs

Christopher A Belica (CA)

Department of Biochemistry, Molecular Biology and Biophysics, University of Minnesota, Minneapolis, MN, United States; Institute for Molecular Virology, University of Minnesota, Minneapolis, MN, United States; Masonic Cancer Center, University of Minnesota, Minneapolis, MN, United States. Electronic address: belic028@umn.edu.

Patricia C Hernandez (PC)

Department of Biochemistry, Molecular Biology and Biophysics, University of Minnesota, Minneapolis, MN, United States; Institute for Molecular Virology, University of Minnesota, Minneapolis, MN, United States; Masonic Cancer Center, University of Minnesota, Minneapolis, MN, United States.

Michael A Carpenter (MA)

Department of Biochemistry and Structural Biology, University of Texas Health San Antonio, San Antonio, TX, United States; Howard Hughes Medical Institute, University of Texas Health San Antonio, San Antonio, TX, United States.

Yanjun Chen (Y)

Department of Biochemistry and Structural Biology, University of Texas Health San Antonio, San Antonio, TX, United States.

William L Brown (WL)

Department of Biochemistry, Molecular Biology and Biophysics, University of Minnesota, Minneapolis, MN, United States; Institute for Molecular Virology, University of Minnesota, Minneapolis, MN, United States; Masonic Cancer Center, University of Minnesota, Minneapolis, MN, United States.

Reuben S Harris (RS)

Department of Biochemistry and Structural Biology, University of Texas Health San Antonio, San Antonio, TX, United States; Howard Hughes Medical Institute, University of Texas Health San Antonio, San Antonio, TX, United States.

Hideki Aihara (H)

Department of Biochemistry, Molecular Biology and Biophysics, University of Minnesota, Minneapolis, MN, United States; Institute for Molecular Virology, University of Minnesota, Minneapolis, MN, United States; Masonic Cancer Center, University of Minnesota, Minneapolis, MN, United States. Electronic address: aihar001@umn.edu.

Articles similaires

[Redispensing of expensive oral anticancer medicines: a practical application].

Lisanne N van Merendonk, Kübra Akgöl, Bastiaan Nuijen
1.00
Humans Antineoplastic Agents Administration, Oral Drug Costs Counterfeit Drugs

Smoking Cessation and Incident Cardiovascular Disease.

Jun Hwan Cho, Seung Yong Shin, Hoseob Kim et al.
1.00
Humans Male Smoking Cessation Cardiovascular Diseases Female
Humans United States Aged Cross-Sectional Studies Medicare Part C
1.00
Humans Yoga Low Back Pain Female Male

Classifications MeSH