From Corn Starch to Nanostructured Magnetic Laser-Induced Graphene Nanocomposite.

biodegradables bioderived core–shell nanoparticles iron‐catalytic laser‐induced graphene magnetic starch

Journal

Small (Weinheim an der Bergstrasse, Germany)
ISSN: 1613-6829
Titre abrégé: Small
Pays: Germany
ID NLM: 101235338

Informations de publication

Date de publication:
18 Oct 2024
Historique:
revised: 02 10 2024
received: 26 06 2024
medline: 18 10 2024
pubmed: 18 10 2024
entrez: 18 10 2024
Statut: aheadofprint

Résumé

Laser-Induced Graphene (LIG) is a 3D, conductive, porous material with a high surface area, produced by laser irradiation of synthetic polymers with high thermal stability. Recently, the focus has shifted toward sustainable bioderived and biodegradable precursors, such as lignocellulosic materials. Despite starch being an abundant and cost-effective biopolymer, direct laser scribing on starch-derived precursors has not yet been explored. This study demonstrates that corn starch bioplastic (SP) can be converted into LIG through iron-catalyzed laser-induced pyrolysis, using Fe(NO₃)₃ as an additive. The impact of iron additive concentration on LIG formation and on its properties is investigated, with only certain concentrations yielding reliable and reproducible results. The investigation of LIG's crystal structure reveals magnetic and non-magnetic iron phases: γ-Fe₂O₃, Fe₃C, and Fe(C). The LIG nanocomposite exhibits soft magnetic properties, with a coercive field of H

Identifiants

pubmed: 39420870
doi: 10.1002/smll.202405252
doi:

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Pagination

e2405252

Subventions

Organisme : Ministero dell'Istruzione, dell'Università e della Ricerca
ID : CCI 2014IT16M2OP005
Organisme : H2020 Excellent Science
ID : 899349

Informations de copyright

© 2024 The Author(s). Small published by Wiley‐VCH GmbH.

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Auteurs

Sreenadh Thaikkattu Sankaran (ST)

The Biorobotics Institute, Scuola Superiore Sant'Anna, Viale Rinaldo Piaggio 34, Pontedera, 56025, Italy.
Department of Excellence in Robotics & AI, Scuola Superiore Sant'Anna, Piazza Martiri della Libertà 33, Pisa, 56127, Italy.

Alexander Dallinger (A)

Institute of Solid State Physics, NAWI Graz, Graz University of Technology, Petersgasse 16, Graz, 8010, Austria.

Anna Chiara Bressi (AC)

The Biorobotics Institute, Scuola Superiore Sant'Anna, Viale Rinaldo Piaggio 34, Pontedera, 56025, Italy.
Department of Excellence in Robotics & AI, Scuola Superiore Sant'Anna, Piazza Martiri della Libertà 33, Pisa, 56127, Italy.

Attilio Marino (A)

Smart Bio-Interfaces, Istituto Italiano di Tecnologia, Viale Rinaldo Piaggio 34, Pontedera, 56025, Italy.

Gianni Ciofani (G)

Smart Bio-Interfaces, Istituto Italiano di Tecnologia, Viale Rinaldo Piaggio 34, Pontedera, 56025, Italy.

Aleksandra Szkudlarek (A)

Academic Centre for Materials and Nanotechnology, AGH University of Krakow, av. Mickiewicza 30, Krakow, 30-059, Poland.

Vitaliy Bilovol (V)

Academic Centre for Materials and Nanotechnology, AGH University of Krakow, av. Mickiewicza 30, Krakow, 30-059, Poland.

Krystian Sokolowski (K)

Academic Centre for Materials and Nanotechnology, AGH University of Krakow, av. Mickiewicza 30, Krakow, 30-059, Poland.

Birgit Kunert (B)

Institute of Solid State Physics, NAWI Graz, Graz University of Technology, Petersgasse 16, Graz, 8010, Austria.

Hana Kristin Hampel (HK)

Institute of Experimental Physics, NAWI Graz, Graz University of Technology, Petersgasse 16, Graz, 8010, Austria.

Hilda Gomez Bernal (HG)

The Biorobotics Institute, Scuola Superiore Sant'Anna, Viale Rinaldo Piaggio 34, Pontedera, 56025, Italy.

Francesco Greco (F)

The Biorobotics Institute, Scuola Superiore Sant'Anna, Viale Rinaldo Piaggio 34, Pontedera, 56025, Italy.
Department of Excellence in Robotics & AI, Scuola Superiore Sant'Anna, Piazza Martiri della Libertà 33, Pisa, 56127, Italy.
Institute of Solid State Physics, NAWI Graz, Graz University of Technology, Petersgasse 16, Graz, 8010, Austria.
Interdisciplinary Center on Sustainability and Climate, Scuola Superiore Sant'Anna, Piazza Martiri della Libertà 33, Pisa, 56127, Italy.

Classifications MeSH