Sensitivity of Capacity Fade in Vanadium Redox Flow Battery to Electrolyte Impurity Content.
Capacity decay
Impurity ions
Vanadium
Vanadium electrolyte
Vanadium redox flow battery
Journal
ChemPlusChem
ISSN: 2192-6506
Titre abrégé: Chempluschem
Pays: Germany
ID NLM: 101580948
Informations de publication
Date de publication:
21 Oct 2024
21 Oct 2024
Historique:
revised:
14
08
2024
received:
30
05
2024
medline:
21
10
2024
pubmed:
21
10
2024
entrez:
21
10
2024
Statut:
aheadofprint
Résumé
The gradual capacity decrease of vanadium redox flow battery (VRFB) over long-term charge-discharge cycling is determined by electrolyte degradation. While it was initially believed that this degradation was solely caused by crossover, recent research suggests that oxidative imbalance induced by hydrogen evolution reaction (HER) also plays a significant role. In this work by using vanadium pentoxides with different impurities content, we prepared three grades of vanadium electrolyte. By measuring electrochemical properties on carbon felt electrode in three-electrode cell and VRFB membrane-electrode assembly we evaluate the influence of impurity content on battery polarization and rate of side reactions which is indicated by the increase of average oxidation state (AOS) during charge-discharge tests and varies from 0.061 to 0.027 day
Identifiants
pubmed: 39431899
doi: 10.1002/cplu.202400372
doi:
Types de publication
Journal Article
Langues
eng
Sous-ensembles de citation
IM
Pagination
e202400372Subventions
Organisme : Russian Science Foundation
ID : 21-73-30029
Informations de copyright
© 2024 Wiley-VCH GmbH.
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