Breast cancer secretes anti-ferroptotic MUFAs and depends on selenoprotein synthesis for metastasis.

Breast Cancer Ferroptosis Lipid Metabolism Metastasis Selenium Metabolism

Journal

EMBO molecular medicine
ISSN: 1757-4684
Titre abrégé: EMBO Mol Med
Pays: Germany
ID NLM: 101487380

Informations de publication

Date de publication:
21 Oct 2024
Historique:
received: 23 06 2023
accepted: 04 09 2024
revised: 23 08 2024
medline: 22 10 2024
pubmed: 22 10 2024
entrez: 21 10 2024
Statut: aheadofprint

Résumé

The limited availability of therapeutic options for patients with triple-negative breast cancer (TNBC) contributes to the high rate of metastatic recurrence and poor prognosis. Ferroptosis is a type of cell death caused by iron-dependent lipid peroxidation and counteracted by the antioxidant activity of the selenoprotein GPX4. Here, we show that TNBC cells secrete an anti-ferroptotic factor in the extracellular environment when cultured at high cell densities but are primed to ferroptosis when forming colonies at low density. We found that secretion of the anti-ferroptotic factors, identified as monounsaturated fatty acid (MUFA) containing lipids, and the vulnerability to ferroptosis of single cells depends on the low expression of stearyl-CoA desaturase (SCD) that is proportional to cell density. Finally, we show that the inhibition of Sec-tRNAsec biosynthesis, an essential step for selenoprotein production, causes ferroptosis and impairs the lung seeding of circulating TNBC cells that are no longer protected by the MUFA-rich environment of the primary tumour.

Identifiants

pubmed: 39433871
doi: 10.1038/s44321-024-00142-x
pii: 10.1038/s44321-024-00142-x
doi:

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Subventions

Organisme : Cancer Research UK (CRUK)
ID : A31287
Organisme : Cancer Research UK (CRUK)
ID : A29800
Organisme : Cancer Research UK (CRUK)
ID : A29799
Organisme : Cancer Research UK (CRUK)
ID : A23982
Organisme : Breast Cancer Now (BCN)
ID : 2018NovPR102

Informations de copyright

© 2024. The Author(s).

Références

Aceto N, Bardia A, Miyamoto DT, Donaldson MC, Wittner BS, Spencer JA, Yu M, Pely A, Engstrom A, Zhu H et al (2014) Circulating tumor cell clusters are oligoclonal precursors of breast cancer metastasis. Cell 158:1110–1122
doi: 10.1016/j.cell.2014.07.013 pmcid: 4149753 pubmed: 25171411
Alborzinia H, Chen Z, Yildiz U, Freitas FP, Vogel FCE, Varga JP, Batani J, Bartenhagen C, Schmitz W, Büchel G et al (2023) LRP8‐mediated selenocysteine uptake is a targetable vulnerability in MYCN‐amplified neuroblastoma. EMBO Mol Med 15(8):e18014
doi: 10.15252/emmm.202318014 pmcid: 10405063 pubmed: 37435859
Altea-Manzano P, Doglioni G, Liu Y, Cuadros AM, Nolan E, Fernández-García J, Wu Q, Planque M, Laue KJ, Cidre-Aranaz F et al (2023) A palmitate-rich metastatic niche enables metastasis growth via p65 acetylation resulting in pro-metastatic NF-κB signaling. Nat Cancer 4(3):344–364
doi: 10.1038/s43018-023-00513-2 pmcid: 7615234 pubmed: 36732635
Bersuker K, Hendricks JM, Li Z, Magtanong L, Ford B, Tang PH, Roberts MA, Tong B, Maimone TJ, Zoncu R et al (2019) The CoQ oxidoreductase FSP1 acts parallel to GPX4 to inhibit ferroptosis. Nature 575:688–692
doi: 10.1038/s41586-019-1705-2 pmcid: 6883167 pubmed: 31634900
Burk RF, Hill KE (2015) Regulation of Selenium Metabolism and Transport. Annu Rev Nutr 35:109–134
Carlisle AE, Lee N, Matthew-Onabanjo AN, Spears ME, Park SJ, Youkana D, Doshi MB, Peppers A, Li R, Joseph AB et al (2020) Selenium detoxification is required for cancer-cell survival. Nat Metab 2:603–611
doi: 10.1038/s42255-020-0224-7 pmcid: 7455022 pubmed: 32694795
Chambers MC, MacLean B, Burke R, Amodei D, Ruderman DL, Neumann S, Gatto L, Fischer B, Pratt B, Egertson J et al (2012) A cross-platform toolkit for mass spectrometry and proteomics. Nat Biotechnol 30:918–920. https://doi.org/10.1038/nbt.2377
doi: 10.1038/nbt.2377 pmcid: 3471674 pubmed: 23051804
Charalabopoulos K, Kotsalos A, Batistatou A, Charalabopoulos A, Vezyraki P, Peschos D, Kalfakakou V, Evangelou A (2006) Selenium in serum and neoplastic tissue in breast cancer: correlation with CEA. Br J Cancer 95:674–676
doi: 10.1038/sj.bjc.6603292 pmcid: 2360505 pubmed: 16880784
Chen Y-C, Prabhu KS, Mastro AM (2013) Is selenium a potential treatment for cancer metastasis? Nutrients 5:1149–1168
doi: 10.3390/nu5041149 pmcid: 3705340 pubmed: 23567478
Chen Z, Yan Y, Qi C, Liu J, Li L, Wang J (2021) The role of ferroptosis in cardiovascular disease and its therapeutic significance. Front Cardiovasc Med 8:733229
doi: 10.3389/fcvm.2021.733229 pmcid: 8576275 pubmed: 34765653
Dierge E, Debock E, Guilbaud C, Corbet C, Mignolet E, Mignard L, Bastien E, Dessy C, Larondelle Y, Feron O (2021) Peroxidation of n-3 and n-6 polyunsaturated fatty acids in the acidic tumor environment leads to ferroptosis-mediated anticancer effects. Cell Metab 33:1701–1715.e5
doi: 10.1016/j.cmet.2021.05.016 pubmed: 34118189
Doll S, Proneth B, Tyurina YY, Panzilius E, Kobayashi S, Ingold I, Irmler M, Beckers J, Aichler M, Walch A et al (2017) ACSL4 dictates ferroptosis sensitivity by shaping cellular lipid composition. Nat Chem Biol 13:91–98
doi: 10.1038/nchembio.2239 pubmed: 27842070
Eagle K, Jiang Y, Shi X, Li M, Obholzer NP, Hu T, Perez MW, Koren JV, Kitano A, Yi JS et al (2022) An oncogenic enhancer encodes selective selenium dependency in AML. Cell Stem Cell 29:386–399.e7
doi: 10.1016/j.stem.2022.01.003 pmcid: 8903199 pubmed: 35108519
Freitas FP, Alborzinia H, dos Santos AF, Nepachalovich P, Pedrera L, Zilka O, Inague A, Klein C, Aroua N, Kaushal K et al (2024) 7-Dehydrocholesterol is an endogenous suppressor of ferroptosis. Nature 626:401–410
doi: 10.1038/s41586-023-06878-9 pubmed: 38297129
Gkountela S, Castro-Giner F, Szczerba BM, Vetter M, Landin J, Scherrer R, Krol I, Scheidmann MC, Beisel C, Stirnimann CU et al (2019) Circulating tumor cell clustering shapes DNA methylation to enable metastasis seeding. Cell 176:98–112.e14
doi: 10.1016/j.cell.2018.11.046 pmcid: 6363966 pubmed: 30633912
Hernandez-Fernaud JR, Ruengeler E, Casazza A, Neilson LJ, Pulleine E, Santi A, Ismail S, Lilla S, Dhayade S, MacPherson IR et al (2017) Secreted CLIC3 drives cancer progression through its glutathione-dependent oxidoreductase activity. Nat Commun 8:14206
doi: 10.1038/ncomms14206 pmcid: 5316871 pubmed: 28198360
Hutchins PD, Russell JD, Coon JJ (2018) LipiDex: an integrated software package for high-confidence lipid identification. Cell Syst 6:621–625.e5
doi: 10.1016/j.cels.2018.03.011 pmcid: 5967991 pubmed: 29705063
Hutchins PD, Russell JD, Coon JJ (2019) Mapping lipid fragmentation for tailored mass spectral libraries. J Am Soc Mass Spectrom 30:659–668
doi: 10.1007/s13361-018-02125-y pmcid: 6447430 pubmed: 30756325
Kojima Y, Acar A, Eaton EN, Mellody KT, Scheel C, Ben-Porath I, Onder TT, Wang ZC, Richardson AL, Weinberg RA et al (2010) Autocrine TGF-β and stromal cell-derived factor-1 (SDF-1) signaling drives the evolution of tumor-promoting mammary stromal myofibroblasts. Proc Natl Acad Sci USA 107:20009–20014
doi: 10.1073/pnas.1013805107 pmcid: 2993333 pubmed: 21041659
Labunskyy VM, Hatfield DL, Gladyshev VN (2014) Selenoproteins: molecular pathways and physiological roles. Physiol Rev 94:739–777
doi: 10.1152/physrev.00039.2013 pmcid: 4101630 pubmed: 24987004
Li Y, Ran Q, Duan Q, Jin J, Wang Y, Yu L, Wang C, Zhu Z, Chen X, Weng L et al (2024) 7-Dehydrocholesterol dictates ferroptosis sensitivity. Nature 626:411–418
doi: 10.1038/s41586-023-06983-9 pmcid: 11298758 pubmed: 38297130
Lorito N, Subbiani A, Smiriglia A, Bacci M, Bonechi F, Tronci L, Romano E, Corrado A, Longo DL, Iozzo M et al (2024) FADS1/2 control lipid metabolism and ferroptosis susceptibility in triple-negative breast cancer. Embo Mol Med 16: 1533–1559
Magtanong L, Ko PJ, To M, Cao JY, Forcina GC, Tarangelo A, Ward CC, Cho K, Patti GJ, Nomura DK et al (2019) Exogenous monounsaturated fatty acids promote a ferroptosis-resistant cell state. Cell Chem Biol 26:420–432.e9
doi: 10.1016/j.chembiol.2018.11.016 pmcid: 6430697 pubmed: 30686757
Mao C, Liu X, Zhang Y, Lei G, Yan Y, Lee H, Koppula P, Wu S, Zhuang L, Fang B et al (2021) DHODH-mediated ferroptosis defence is a targetable vulnerability in cancer. Nature 593:586–590
doi: 10.1038/s41586-021-03539-7 pmcid: 8895686 pubmed: 33981038
Matyash V, Liebisch G, Kurzchalia TV, Shevchenko A, Schwudke D (2008) Lipid extraction by methyl-terf-butyl ether for high-throughput lipidomics. J Lipid Res 49:1137–1146
doi: 10.1194/jlr.D700041-JLR200 pmcid: 2311442 pubmed: 18281723
Mishima E, Ito J, Wu Z, Nakamura T, Wahida A, Doll S, Tonnus W, Nepachalovich P, Eggenhofer E, Aldrovandi M et al (2022) A non-canonical vitamin K cycle is a potent ferroptosis suppressor. Nature 608:778–783
doi: 10.1038/s41586-022-05022-3 pmcid: 9402432 pubmed: 35922516
National Institutes of Health—Office of Dietary Supplements (2023) Selenium—fact sheet for health professionals. https://ods.od.nih.gov/factsheets/Selenium-HealthProfessional/
Panzilius E, Holstein F, Dehairs J, Planque M, Von C, Koenig A, Doll S, Bannier-hélaouët M, Hilary M, Hauck SM et al (2018) Cell density-dependent ferroptosis in breast cancer is induced by accumulation of polyunsaturated fatty acid-enriched triacylglycerides. Preprint at https://www.biorxiv.org/content/10.1101/417949v2
Qiu B, Zandkarimi F, Bezjian CT, Reznik E, Soni RK, Gu W, Jiang X, Stockwell BR (2024) Phospholipids with two polyunsaturated fatty acyl tails promote ferroptosis. Cell 187(5):1177–1190.e18
doi: 10.1016/j.cell.2024.01.030 pubmed: 38366593
Sahai E, Astsaturov I, Cukierman E, DeNardo DG, Egeblad M, Evans RM, Fearon D, Greten FR, Hingorani SR, Hunter T et al (2020) A framework for advancing our understanding of cancer-associated fibroblasts. Nat Rev Cancer 20:174–186. https://doi.org/10.1038/s41568-019-0238-1
doi: 10.1038/s41568-019-0238-1 pmcid: 7046529 pubmed: 31980749
Sherrer RL, O’Donoghue P, Söll D (2008) Characterization and evolutionary history of an archaeal kinase involved in selenocysteinyl-tRNA formation. Nucleic Acids Res 36:1247–1259
doi: 10.1093/nar/gkm1134 pmcid: 2275090 pubmed: 18174226
Song X, Liu J, Kuang F, Chen X, Zeh HJ, Kang R, Kroemer G, Xie Y, Tang D (2021) PDK4 dictates metabolic resistance to ferroptosis by suppressing pyruvate oxidation and fatty acid synthesis. Cell Rep 34:108767
doi: 10.1016/j.celrep.2021.108767 pubmed: 33626342
Soula M, Weber RA, Zilka O, Alwaseem H, La K, Yen F, Molina H, Garcia-Bermudez J, Pratt DA, Birsoy K (2020) Metabolic determinants of cancer cell sensitivity to canonical ferroptosis inducers. Nat Chem Biol 16:1351–1360
doi: 10.1038/s41589-020-0613-y pmcid: 8299533 pubmed: 32778843
Szczerba BM, Castro-Giner F, Vetter M, Krol I, Gkountela S, Landin J, Scheidmann MC, Donato C, Scherrer R, Singer J et al (2019) Neutrophils escort circulating tumour cells to enable cell cycle progression. Nature 566:553–557
doi: 10.1038/s41586-019-0915-y pubmed: 30728496
Terry AR, Nogueira V, Rho H, Ramakrishnan G, Li J, Kang S, Pathmasiri KC, Bhat SA, Jiang L, Kuchay S et al (2023) CD36 maintains lipid homeostasis via selective uptake of monounsaturated fatty acids during matrix detachment and tumor progression. Cell Metab 35:2060–2076.e9
doi: 10.1016/j.cmet.2023.09.012 pubmed: 37852255
Tesfay L, Paul BT, Konstorum A, Deng Z, Cox AO, Lee J, Furdui CM, Hegde P, Torti FM, Torti SV (2019) Stearoyl-CoA desaturase 1 protects ovarian cancer cells from ferroptotic cell death. Cancer Res 79:5355–5366
doi: 10.1158/0008-5472.CAN-19-0369 pmcid: 6801059 pubmed: 31270077
Ubellacker JM, Tasdogan A, Ramesh V, Shen B, Mitchell EC, Martin-Sandoval MS, Gu Z, McCormick ML, Durham AB, Spitz DR et al (2020) Lymph protects metastasizing melanoma cells from ferroptosis. Nature 585:113–118
doi: 10.1038/s41586-020-2623-z pmcid: 7484468 pubmed: 32814895
Ursini F, Maiorino M, Gregolin C (1985) The selenoenzyme phospholipid hydroperoxide glutathione peroxidase. Biochim Biophys Acta 839(1):62–70
doi: 10.1016/0304-4165(85)90182-5 pubmed: 3978121
Vande Voorde J, Ackermann T, Pfetzer N, Sumpton D, Mackay G, Kalna G, Nixon C, Blyth K, Gottlieb E, Tardito S (2019) Improving the metabolic fidelity of cancer models with a physiological cell culture medium. Sci Adv 5:eaau7314
doi: 10.1126/sciadv.aau7314 pmcid: 6314821 pubmed: 30613774
Vinceti M, Dennert G, Crespi CM, Zwahlen M, Brinkman M, Zeegers MPA, Horneber M, D’Amico R, del Giovane C (2014) Selenium for preventing cancer. Cochrane Database Syst Rev https://doi.org/10.1002/14651858.CD005195.pub3
Wu J, Minikes AM, Gao M, Bian H, Li Y, Stockwell BR, Chen ZN, Jiang X (2019) Intercellular interaction dictates cancer cell ferroptosis via NF2–YAP signalling. Nature 572:402–406
doi: 10.1038/s41586-019-1426-6 pmcid: 6697195 pubmed: 31341276
Xie Y, Wang B, Zhao Y, Tao Z, Wang Y, Chen G, Hu X (2022) Mammary adipocytes protect triple-negative breast cancer cells from ferroptosis. J Hematol Oncol https://doi.org/10.1186/s13045-022-01297-1
Yan H fa, Zou T, Tuo QZ, Xu S, Li H, Belaidi AA, Lei P (2021) Ferroptosis: mechanisms and links with diseases. Signal Transduct Target Ther https://doi.org/10.1038/s41392-020-00428-9
Yang F, Xiao Y, Ding JH, Jin X, Ma D, Li DQ, Shi JX, Huang W, Wang YP, Jiang YZ et al (2023) Ferroptosis heterogeneity in triple-negative breast cancer reveals an innovative immunotherapy combination strategy. Cell Metab 35:84–100.e8
doi: 10.1016/j.cmet.2022.09.021 pubmed: 36257316
Yang WS, Sriramaratnam R, Welsch ME, Shimada K, Skouta R, Viswanathan VS, Cheah JH, Clemons PA, Shamji AF, Clish CB et al (2014) Regulation of ferroptotic cancer cell death by GPX4. Cell 156:317–331
doi: 10.1016/j.cell.2013.12.010 pmcid: 4076414 pubmed: 24439385
Yang WS, Stockwell BR (2016) Ferroptosis: death by lipid peroxidation. Trends Cell Biol 26:165–176
doi: 10.1016/j.tcb.2015.10.014 pubmed: 26653790
Yu M, Bardia A, Aceto N, Bersani F, Madden MW, Donaldson MC, Desai R, Zhu H, Comaills V, Zheng Z et al (2014) Ex vivo culture of circulating breast tumor cells for individualized testing of drug susceptibility. Science 345:216–220
doi: 10.1126/science.1253533 pmcid: 4358808 pubmed: 25013076
Zhao L, Wu X, Li T, Luo J, Dong D (2020) CtcRbase: the gene expression database of circulating tumor cells and microemboli. Database 2020:baaa020
doi: 10.1093/database/baaa020 pmcid: 7158883 pubmed: 32294193
Zheng J, Conrad M (2020) The metabolic underpinnings of ferroptosis. Cell Metab 32:920–937
doi: 10.1016/j.cmet.2020.10.011 pubmed: 33217331

Auteurs

Tobias Ackermann (T)

Cancer Research UK Scotland Institute, Garscube Estate, Switchback Road, Glasgow, G61 1BD, UK.
School of Cancer Sciences, University of Glasgow, Glasgow, G611QH, UK.

Engy Shokry (E)

Cancer Research UK Scotland Institute, Garscube Estate, Switchback Road, Glasgow, G61 1BD, UK.

Ruhi Deshmukh (R)

Cancer Research UK Scotland Institute, Garscube Estate, Switchback Road, Glasgow, G61 1BD, UK.

Jayanthi Anand (J)

Cancer Research UK Scotland Institute, Garscube Estate, Switchback Road, Glasgow, G61 1BD, UK.

Laura C A Galbraith (LCA)

Cancer Research UK Scotland Institute, Garscube Estate, Switchback Road, Glasgow, G61 1BD, UK.

Louise Mitchell (L)

Cancer Research UK Scotland Institute, Garscube Estate, Switchback Road, Glasgow, G61 1BD, UK.

Giovanny Rodriguez-Blanco (G)

Cancer Research UK Scotland Institute, Garscube Estate, Switchback Road, Glasgow, G61 1BD, UK.

Victor H Villar (VH)

Cancer Research UK Scotland Institute, Garscube Estate, Switchback Road, Glasgow, G61 1BD, UK.
School of Medicine, University of St Andrews, St. Andrews, KY16 9TF, UK.

Britt Amber Sterken (BA)

Cancer Research UK Scotland Institute, Garscube Estate, Switchback Road, Glasgow, G61 1BD, UK.

Colin Nixon (C)

Cancer Research UK Scotland Institute, Garscube Estate, Switchback Road, Glasgow, G61 1BD, UK.

Sara Zanivan (S)

Cancer Research UK Scotland Institute, Garscube Estate, Switchback Road, Glasgow, G61 1BD, UK.
School of Cancer Sciences, University of Glasgow, Glasgow, G611QH, UK.

Karen Blyth (K)

Cancer Research UK Scotland Institute, Garscube Estate, Switchback Road, Glasgow, G61 1BD, UK.
School of Cancer Sciences, University of Glasgow, Glasgow, G611QH, UK.

David Sumpton (D)

Cancer Research UK Scotland Institute, Garscube Estate, Switchback Road, Glasgow, G61 1BD, UK.

Saverio Tardito (S)

Cancer Research UK Scotland Institute, Garscube Estate, Switchback Road, Glasgow, G61 1BD, UK. saverio.tardito@meduniwien.ac.at.
School of Cancer Sciences, University of Glasgow, Glasgow, G611QH, UK. saverio.tardito@meduniwien.ac.at.
Center for Cancer Research, Medical University of Vienna, Comprehensive Cancer Center, Vienna, 1090, Austria. saverio.tardito@meduniwien.ac.at.

Classifications MeSH