Synthetic Periodontal Guided Tissue Regeneration Membrane with Self-Assembling Biphasic Structure and Temperature-Sensitive Shape Maintenance.

bone membrane network polymer periodontal ligament periodontal regeneration tissue engineering

Journal

Advanced healthcare materials
ISSN: 2192-2659
Titre abrégé: Adv Healthc Mater
Pays: Germany
ID NLM: 101581613

Informations de publication

Date de publication:
23 Oct 2024
Historique:
revised: 03 10 2024
received: 10 06 2024
medline: 24 10 2024
pubmed: 24 10 2024
entrez: 24 10 2024
Statut: aheadofprint

Résumé

Periodontal disease poses significant challenges to the long-term stability of oral health by destroying the supporting structures of teeth. Guided tissue regeneration techniques, particularly barrier membranes, enable local regeneration by providing an isolated, protected compartment for osseous wound healing while excluding epithelial tissue. Here, this study reports on a thermosensitive periodontal membrane (TSPM) technology designed to overcome the mechanical limitations of current membranes through a semi-interpenetrating network of high molecular weight poly(L-lactic acid) (PLLA) and in situ-polymerized mesh of poly(ε-caprolactone)diacrylate (PCL-DA), and poly lactide-co-glycolide diacrylate (PLGA-DA). An optimized composition allows facile reshaping at greater than 52 °C and rigid shape maintenance at physiological temperature. Its unique bilayer morphology is achieved through self-assembly and thermally-induced phase separation, resulting in distinct yet continuous smooth and nanofibrous compartments adequate for epithelial occlusion and regeneration. Incorporating PLGA-DA enhances the membrane's hydrophilicity and degradation properties, facilitating a more rapid and controlled degradation and therapeutic delivery. This study demonstrates its ability to promote local regeneration by serving as a barrier membrane and simultaneously as a scaffolding matrix in a rat orthotopic periodontal defect model. The TSPM outperformed a clinically available material (Epi-Guide) to facilitate robust alveolar bone and periodontal ligament regeneration at 4 and 8 weeks.

Identifiants

pubmed: 39444056
doi: 10.1002/adhm.202402137
doi:

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Pagination

e2402137

Subventions

Organisme : NIH HHS
ID : NIDCR R01-DE027662
Pays : United States
Organisme : NIDCR NIH HHS
ID : DE031476
Pays : United States

Informations de copyright

© 2024 The Author(s). Advanced Healthcare Materials published by Wiley‐VCH GmbH.

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Auteurs

W Benton Swanson (WB)

Department of Biologic and Materials Science, School of Dentistry, University of Michigan, Ann Arbor, MI, 48109, USA.

Seth M Woodbury (SM)

Department of Biologic and Materials Science, School of Dentistry, University of Michigan, Ann Arbor, MI, 48109, USA.
Department of Chemistry, College of Literature, Science and the Arts, University of Michigan, Ann Arbor, MI, 48109, USA.
Department of Physics, College of Literature, Science and the Arts, University of Michigan, Ann Arbor, MI, 48109, USA.

Renan Dal-Fabbro (R)

Department of Cariology, Restorative Sciences and Endodontics, School of Dentistry, University of Michigan, Ann Arbor, MI, 48109, USA.

Lindsey Douglas (L)

Department of Chemistry, College of Literature, Science and the Arts, University of Michigan, Ann Arbor, MI, 48109, USA.

Jackson Albright (J)

Department of Biomedical Engineering, College of Engineering, University of Michigan, Ann Arbor, MI, 48109, USA.

Miranda Eberle (M)

Department of Chemistry, College of Literature, Science and the Arts, University of Michigan, Ann Arbor, MI, 48109, USA.

David Niemann (D)

Department of Chemistry, College of Literature, Science and the Arts, University of Michigan, Ann Arbor, MI, 48109, USA.

Jinping Xu (J)

Department of Cariology, Restorative Sciences and Endodontics, School of Dentistry, University of Michigan, Ann Arbor, MI, 48109, USA.

Marco C Bottino (MC)

Department of Cariology, Restorative Sciences and Endodontics, School of Dentistry, University of Michigan, Ann Arbor, MI, 48109, USA.
Department of Biomedical Engineering, College of Engineering, University of Michigan, Ann Arbor, MI, 48109, USA.

Yuji Mishina (Y)

Department of Biologic and Materials Science, School of Dentistry, University of Michigan, Ann Arbor, MI, 48109, USA.

Classifications MeSH