Chemo-enzymatic synthesis of p-nitrophenyl β-D-galactofuranosyl disaccharides from Aspergillus sp. fungal-type galactomannan.


Journal

Carbohydrate research
ISSN: 1873-426X
Titre abrégé: Carbohydr Res
Pays: Netherlands
ID NLM: 0043535

Informations de publication

Date de publication:
01 Feb 2019
Historique:
received: 18 12 2018
revised: 10 01 2019
accepted: 10 01 2019
pubmed: 19 1 2019
medline: 6 5 2019
entrez: 19 1 2019
Statut: ppublish

Résumé

β-d-Galactofuranose (Galf) is a component of polysaccharides and glycoconjugates. There are few reports about the involvement of galactofuranosyltransferases and galactofuranosidases (Galf-ases) in the synthesis and degradation of galactofuranose-containing glycans. The cell walls of filamentous fungi in the genus Aspergillus include galactofuranose-containing polysaccharides and glycoconjugates, such as O-glycans, N-glycans, and fungal-type galactomannan, which are important for cell wall integrity. In this study, we investigated the synthesis of p-nitrophenyl β-d-galactofuranoside and its disaccharides by chemo-enzymatic methods including use of galactosidase. The key step was selective removal of the concomitant pyranoside by enzymatic hydrolysis to purify p-nitrophenyl β-d-galactofuranoside, a promising substrate for β-d-galactofuranosidase from Streptomyces species.

Identifiants

pubmed: 30658252
pii: S0008-6215(18)30736-5
doi: 10.1016/j.carres.2019.01.005
pii:
doi:

Substances chimiques

Disaccharides 0
Mannans 0
galactomannan 11078-30-1
Galactosidases EC 3.2.1.-
Galactose X2RN3Q8DNE

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Pagination

99-103

Informations de copyright

Copyright © 2019 Elsevier Ltd. All rights reserved.

Auteurs

Ryo Ota (R)

Graduate School of Environmental and Life Science, Okayama University, Tsushima-naka 1-1-1, Okayama, 700-8530, Japan.

Yumi Okamoto (Y)

Graduate School of Environmental and Life Science, Okayama University, Tsushima-naka 1-1-1, Okayama, 700-8530, Japan.

Christopher J Vavricka (CJ)

Graduate School of Science, Technology and Innovation, Kobe University, 1-1 Rokkodai, Nada, Kobe, 657-8501, Japan.

Takuji Oka (T)

Department of Applied Microbial Technology, Faculty of Biotechnology and Life Science, Sojo University, Ikeda, 4-22-1, Kumamoto 860-0082, Japan.

Emiko Matsunaga (E)

Department of Bioscience and Biotechnology, Faculty of Agriculture, Kyushu University, Hakozaki 6-10-1, Fukuoka, 812-8581, Japan.

Kaoru Takegawa (K)

Department of Bioscience and Biotechnology, Faculty of Agriculture, Kyushu University, Hakozaki 6-10-1, Fukuoka, 812-8581, Japan.

Hiromasa Kiyota (H)

Graduate School of Environmental and Life Science, Okayama University, Tsushima-naka 1-1-1, Okayama, 700-8530, Japan.

Minoru Izumi (M)

Graduate School of Environmental and Life Science, Okayama University, Tsushima-naka 1-1-1, Okayama, 700-8530, Japan. Electronic address: mizumi@okayama-u.ac.jp.

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Classifications MeSH