S-adenosylmethionine biosynthesis is a targetable metabolic vulnerability of cancer stem cells.


Journal

Breast cancer research and treatment
ISSN: 1573-7217
Titre abrégé: Breast Cancer Res Treat
Pays: Netherlands
ID NLM: 8111104

Informations de publication

Date de publication:
May 2019
Historique:
received: 19 09 2018
accepted: 22 01 2019
pubmed: 4 2 2019
medline: 21 8 2019
entrez: 4 2 2019
Statut: ppublish

Résumé

Many transformed cells and embryonic stem cells are dependent on the biosynthesis of the universal methyl-donor S-adenosylmethionine (SAM) from methionine by the enzyme MAT2A to maintain their epigenome. We hypothesized that cancer stem cells (CSCs) rely on SAM biosynthesis and that the combination of methionine depletion and MAT2A inhibition would eradicate CSCs. Human triple (ER/PR/HER2)-negative breast carcinoma (TNBC) cell lines were cultured as CSC-enriched mammospheres in control or methionine-free media. MAT2A was inhibited with siRNAs or cycloleucine. The effects of methionine restriction and/or MAT2A inhibition on the formation of mammospheres, the expression of CSC markers (CD44 Methionine restriction inhibited mammosphere formation and reduced the CD44 Our findings point to SAM biosynthesis as a unique metabolic vulnerability of CSCs that can be targeted by combining methionine depletion with MAT2A inhibition to eradicate drug-resistant CSCs.

Identifiants

pubmed: 30712196
doi: 10.1007/s10549-019-05146-7
pii: 10.1007/s10549-019-05146-7
pmc: PMC6494685
mid: NIHMS1520613
doi:

Substances chimiques

CD24 Antigen 0
Histones 0
Hyaluronan Receptors 0
S-Adenosylmethionine 7LP2MPO46S
Methionine AE28F7PNPL
MAT2A protein, human EC 2.5.1.6
Methionine Adenosyltransferase EC 2.5.1.6

Types de publication

Journal Article

Langues

eng

Pagination

39-50

Subventions

Organisme : National Institute of General Medical Sciences
ID : P41GM108538
Organisme : Morgridge Institute
ID : (JJC)
Organisme : NCI NIH HHS
ID : P30 CA014520
Pays : United States
Organisme : Breast Cancer Research Foundation
ID : (VLC)
Organisme : V Foundation for Cancer Research
ID : (VLC)
Organisme : National Cancer Institute
ID : P30CA14520
Organisme : University of Wisconsin Carbone Cancer Center
ID : Pilot Project
Organisme : NIGMS NIH HHS
ID : P41 GM108538
Pays : United States
Organisme : Wisconsin Partnership Program
ID : (VLC)
Organisme : Sidney Kimmel Foundation for Cancer Research
ID : (PWL)

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Auteurs

Elena Strekalova (E)

Department of Medicine, University of Wisconsin Carbone Cancer Center, University of Wisconsin School of Medicine and Public Health, Madison, WI, USA.

Dmitry Malin (D)

Department of Medicine, University of Wisconsin Carbone Cancer Center, University of Wisconsin School of Medicine and Public Health, Madison, WI, USA.

Erin M M Weisenhorn (EMM)

Department of Biomolecular Chemistry, University of Wisconsin Carbone Cancer Center, University of Wisconsin School of Medicine and Public Health, Madison, WI, USA.

Jason D Russell (JD)

Morgridge Institute for Research, Madison, WI, USA.
Genome Center of Wisconsin, University of Wisconsin-Madison, Madison, WI, USA.

Dominik Hoelper (D)

Department of Biomolecular Chemistry, University of Wisconsin Carbone Cancer Center, University of Wisconsin School of Medicine and Public Health, Madison, WI, USA.

Aayushi Jain (A)

Department of Biomolecular Chemistry, University of Wisconsin Carbone Cancer Center, University of Wisconsin School of Medicine and Public Health, Madison, WI, USA.

Joshua J Coon (JJ)

Department of Biomolecular Chemistry, University of Wisconsin Carbone Cancer Center, University of Wisconsin School of Medicine and Public Health, Madison, WI, USA.
Morgridge Institute for Research, Madison, WI, USA.
Genome Center of Wisconsin, University of Wisconsin-Madison, Madison, WI, USA.
Department of Chemistry, University of Wisconsin-Madison, Madison, WI, USA.

Peter W Lewis (PW)

Department of Biomolecular Chemistry, University of Wisconsin Carbone Cancer Center, University of Wisconsin School of Medicine and Public Health, Madison, WI, USA.

Vincent L Cryns (VL)

Department of Medicine, University of Wisconsin Carbone Cancer Center, University of Wisconsin School of Medicine and Public Health, Madison, WI, USA. vlcryns@medicine.wisc.edu.
Department of Medicine, University of Wisconsin Carbone Cancer Center, University of Wisconsin School of Medicine and Public Health, MFCB 4144, 1685 Highland Avenue, Madison, WI, 53705, USA. vlcryns@medicine.wisc.edu.

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Classifications MeSH